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arXiv:physics/0410256 · Laser Physics Letters

Rubidium spectroscopy at 778–780 nm with a distributed feedback laser diode

Sebastian Kraft, Anselm J. Deninger, Christian Trück, József Fortágh, Frank Lison, Claus Zimmermann

Published Nov 3, 2004• 37 citations
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Abstract

We have performed high resolution spectroscopy of rubidium with a single mode continuous wave distributed feedback (DFB) laser diode. The saturation spectrum of the D 2 -line of 85 Rb and 87 Rb was recorded with a resolution close to the natural line width. The emission frequency was actively stabilized to Doppler-free transitions with a relative accuracy of better than 7 parts in 10 9 using commercially available servo devices only. An output power of 80 mW was sufficient to allow for two-photon spectroscopy of the 5S-5D-transition of 87 Rb. Further, we report on the spectral properties of the DFB diode, its tuning range and its frequency modulation properties. The line width of the diode laser, determined with high resolution Doppler free two photon spectroscopy, was 4 MHz without applying any active stabilization techniques. For time scales below 5 μs the line width drops below 2 MHz.

DOI
10.1002/lapl.200410155

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We have performed high resolution spectroscopy of rubidium with a single mode continuous wave distributed feedback (DFB) laser diode. The saturation spectrum of the D 2 -line of 85 Rb and 87 Rb was recorded with a resolution close to the natural line width. The emission frequency was actively stabilized to Doppler-free transitions with a relative accuracy of better than 7 parts in 10 9 using commercially available servo devices only. An output power of 80 mW was sufficient to allow for two-photon spectroscopy of the 5S-5D-transition of 87 Rb. Further, we report on the spectral properties of the DFB diode, its tuning range and its frequency modulation properties. The line width of the diode laser, determined with high resolution Doppler free two photon spectroscopy, was 4 MHz without applying any active stabilization techniques. For time scales below 5 μs the line width drops below 2 MHz.
Distributed feedback (DFB) laser chips have recently become available at wavelengths that match the D1 and D2 resonance transitions of alkaline atoms. We investigated the spectral properties, tuning characteristics and modulation behavior of continuous wave, single-mode DFB diodes at 778-780 nm and performed high-resolution spectroscopy of Rubidium vapor. The mode-hop free tuning range of the DFB diodes was as large as 2.4 nm (1186 GHz). The line width of the laser diodes was examined both with a heterodyne beat experiment and with high-resolution Doppler-free two photon spectroscopy, yielding a half width of 2-2.5 MHz. The saturation spectra of the D2-line of 85Rb and 87Rb were recorded with a resolution close to the natural line width. The emission frequency was actively stabilized to Doppler-free transitions with a relative accuracy of better than 4 parts in 109 using commercially available servo devices only. The output power of 80 mW was sufficient to allow for two photon spectroscopy of the 5S-5D-transition of 87Rb. We conclude that the performance of the DFB laser equals that of grating-stabilized external-cavity diode lasers (ECDLs), without the mechanical complexity of the latter systems. The DFB diode is thus well-suited to high-resolution applications in alkaline spectroscopy, including laser cooling and optical manipulation of ultra-cold atoms.
Frequency-modulation (FM) spectroscopy has been performed on the D(2) transitions of rubidium atoms with an AlGaAs diode laser at 780 nm. Doppler-broadened hyperfine-structure transitions of (85)Rb and (87)Rb were resolved with no residual amplitude-modulation-induced background signal by modulating the injection current of the laser diode at a low frequency (20-50 MHz) compared with the Doppler width. To obtain Doppler-free spectra, we combined FM spectroscopy with saturation spectroscopy. The results show that the FM spectroscopy technique is sensitive and should be useful for high-resolution spectroscopy, although the resolution was instrument limited and unusual double peaks were observed.
We describe an experiment for investigating the 5S1∕2→5D5∕2 two-photon transition in rubidium using a single grating-feedback diode laser operating at 778.1nm (385THz). Continuous tuning of the laser frequency over 4GHz allows for the clear resolution of the Doppler-free spectral features and allows accurate measurement of the hyperfine ground-state splitting. A direct comparison between Doppler-broadened and Doppler-free spectral features is possible because both are distinctly evident in the two-photon spectra. By independently modifying the polarization state of the two laser fields, the impact of electric dipole selection rules on the two-photon transition spectra is investigated. This experiment is a valuable addition to the advanced undergraduate laboratory because it uses much of the same equipment as the single-photon saturated absorption spectroscopy experiment performed on the 5S1∕2→5P3∕2 transition in rubidium (λ=780.24nm) and provides students with an opportunity to investigate characteristics of atomic spectra not evident in the single-photon experiment.
We demonstrate the spectra of 87Rb 5S1/2 - 5P3/2 - 4D3/2 transitions by utilizing the double-resonance optical-pumping (DROP) and optical-optical double-resonance (OODR) techniques, respectively. The DROP spectrum, compared with the traditional OODR spectrum, show a much better signal-to-noise ratio (SNR). Paying special attention to the influence of alignment of lasers where the coupling and probe beams are counter-propagation and co-propagation on DROP spectrum, so as to further narrow the spectral width by means of electromagnetically induced transparency (EIT). When -the frequency of 1.5μm fiber-pigtailed butterfly-type distributed-feedback (DFB) diode laser is stabilized to the DROP spectrum of 87Rb 5P3/2 - 4D3/2 transition, the preliminary result of residual frequency jitter after stabilization is ~ ±1.3 MHz within 60 s.
The 5S1/2 --> 7S1/2 two-photon transition of atomic rubidium, which is 100 times weaker than the 5S-5D transition, is observed with an extended-cavity diode laser and a vapor cell. Signals with a signal-to-noise ratio of 280 are obtained with a laser power of 10 mW, and the observed linewidth is 3 MHz. The laser wavelength is 760 nm and is locked on the transitions to a stability of 2 x 10(-11). For the first time to our knowledge, the isotope shift of this transition is measured to be 130(4) MHz in atomic frequency.
Characterization of Frequency-Doubled 1.5-μ\muμ m Lasers for High-Performance Rb Clocks
We report on the characterization of two fiber-coupled 1.5-μm diode lasers, frequency-doubled and stabilized to Rubidium (Rb) atomic resonances at 780 nm. Such laser systems are of interest in view of their implementation in Rb vapor-cell atomic clocks, as an alternative to lasers emitting directly at 780 nm. The spectral properties and the instabilities of the frequency-doubled lasers are evaluated against a state-of-the-art compact Rb-stabilized laser system based on a distributed-feedback laser diode emitting at 780 nm. All three lasers are frequency stabilized using essentially identical Doppler-free spectroscopy schemes. The long-term optical power fluctuations at 780 nm are measured, simultaneously with the frequency instability measurements done by three beat notes established between the three lasers. One of the frequency-doubled laser systems shows at 780 nm excellent spectral properties. Its relative intensity noise-12Hz-1is one order of magnitude lower than the reference 780-nm laser, and the frequency noise6Hz2/Hz is limited by the laser current source. Its optical frequency instability is-12at τ = 1 s, limited by the reference laser, and better than 1 × 10-11at all timescales up to one day. We also evaluate the impact of the laser spectral properties and instabilities on the Rb atomic clock performance, in particular taking into account the light-shift effect. Optical power instabilities on long-term timescales, largely originating from the frequency-doubling stage, are identified as a limitation in view of high-performance Rb atomic clocks.