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IEEE Transactions on Ultrasonics Ferroelectrics and Frequency Control

Characterization of Frequency-Doubled 1.5-$\mu$ m Lasers for High-Performance Rb Clocks

Nil Almat, William Moreno, Matthieu Pellaton, Florian Gruet, C. Affolderbach, G. Mileti

Published Jan 15, 2018• 9 citations
Publisher

Abstract

We report on the characterization of two fiber-coupled 1.5-μm diode lasers, frequency-doubled and stabilized to Rubidium (Rb) atomic resonances at 780 nm. Such laser systems are of interest in view of their implementation in Rb vapor-cell atomic clocks, as an alternative to lasers emitting directly at 780 nm. The spectral properties and the instabilities of the frequency-doubled lasers are evaluated against a state-of-the-art compact Rb-stabilized laser system based on a distributed-feedback laser diode emitting at 780 nm. All three lasers are frequency stabilized using essentially identical Doppler-free spectroscopy schemes. The long-term optical power fluctuations at 780 nm are measured, simultaneously with the frequency instability measurements done by three beat notes established between the three lasers. One of the frequency-doubled laser systems shows at 780 nm excellent spectral properties. Its relative intensity noise-12Hz-1is one order of magnitude lower than the reference 780-nm laser, and the frequency noise6Hz2/Hz is limited by the laser current source. Its optical frequency instability is-12at τ = 1 s, limited by the reference laser, and better than 1 × 10-11at all timescales up to one day. We also evaluate the impact of the laser spectral properties and instabilities on the Rb atomic clock performance, in particular taking into account the light-shift effect. Optical power instabilities on long-term timescales, largely originating from the frequency-doubling stage, are identified as a limitation in view of high-performance Rb atomic clocks.

DOI
10.1109/tuffc.2018.2793419

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Characterization of Frequency-Doubled 1.5-μ\muμ m Lasers for High-Performance Rb Clocks
We report on the characterization of two fiber-coupled 1.5-μm diode lasers, frequency-doubled and stabilized to Rubidium (Rb) atomic resonances at 780 nm. Such laser systems are of interest in view of their implementation in Rb vapor-cell atomic clocks, as an alternative to lasers emitting directly at 780 nm. The spectral properties and the instabilities of the frequency-doubled lasers are evaluated against a state-of-the-art compact Rb-stabilized laser system based on a distributed-feedback laser diode emitting at 780 nm. All three lasers are frequency stabilized using essentially identical Doppler-free spectroscopy schemes. The long-term optical power fluctuations at 780 nm are measured, simultaneously with the frequency instability measurements done by three beat notes established between the three lasers. One of the frequency-doubled laser systems shows at 780 nm excellent spectral properties. Its relative intensity noise-12Hz-1is one order of magnitude lower than the reference 780-nm laser, and the frequency noise6Hz2/Hz is limited by the laser current source. Its optical frequency instability is-12at τ = 1 s, limited by the reference laser, and better than 1 × 10-11at all timescales up to one day. We also evaluate the impact of the laser spectral properties and instabilities on the Rb atomic clock performance, in particular taking into account the light-shift effect. Optical power instabilities on long-term timescales, largely originating from the frequency-doubling stage, are identified as a limitation in view of high-performance Rb atomic clocks.
We report on a narrow-linewidth diode laser source emitting at 780 nm, based on frequency doubling from 1.56 μm, which is frequency stabilized on the D2 transition line of Rubidium (Rb). This compact laser source shows a frequency stability of 2·10-12at 1 s and-12for τ up to 104s. This laser source is evaluated in a modular four-laser setup to identify and locate the sources of instabilities. In view of the lasers' applications to vapor-cell Rb atomic clocks, we also studied the various light-shift coefficients in a pulsed optically-pumped Rb clock. Finally, we evaluate the impact of the frequency and intensity instabilities of the frequency-doubled optical sources on the clock stability.
We present the development and complete spectral characterization of our compact and frequency-stabilized laser heads, to be used for rubidium atomic clocks and basic spectroscopy. The light source is a Distributed Feed-Back (DFB) laser diode emitting at 780 nm or 795 nm. The laser frequency is stabilized on a sub-Doppler absorption peak of the 87Rb atom, obtained from an evacuated rubidium cell. These laser heads, including the electronics for the light signals detection, have an overall volume of 0.63 liters. We also present a variant of the laser head into which is integrated an Acousto-Optical Modulator (AOM) that precisely detunes the laser frequency in order to minimize the AC Stark shift in Rb atomic clocks.
We describe a high-performance, compact optical frequency standard based on a microfabricated Rb vapor cell and a low-noise, external cavity diode laser operating on the Rb two-photon transition at 778 nm. The optical standard achieves an instability of 1.8 × 10 − 13 τ − 1 / 2 for times less than 100 s and a flicker noise floor of 1 × 10 − 14 out to 6000 s. At long integration times, the instability is limited by variations in optical probe power and the ac Stark shift. The retrace was measured to 5.7 × 10 − 13 after 30 h of dormancy. Such a simple, yet high-performance optical standard could be suitable as an accurate realization of the meter or, if coupled with an optical frequency comb, as a compact atomic clock comparable to a hydrogen maser.
This thesis presents experimental studies on continuous-wave (CW) laser-microwave double-resonance (DR) spectroscopy and metrology in rubidium (87Rb) vapor cells in view of new high-performance, compact Rb-cell atomic clocks. The Rb vapor cell is confined inside a magnetron-type cavity microwave resonator (MWR). The CW DR spectroscopy involves two resonant electromagnetic fields that are operated simultaneously to interrogate the atoms - the optical field to polarize the atoms by optical pumping, and the microwave field to drive the ground-state hyperfine clock transition that serves as an atomic frequency reference. Details on characterization of compact laser heads and microwave synthesizers used in this work are presented. The vapor cell standards are useful in our everyday lives for applications ranging from telecommunications, navigation, metrology etc. In view of improving the performances of the Rb cell standards, two different clock approaches were studied in detail: The first one is on use of vapor cells (1.4 cm3) whose inner walls are coated with anti-relaxation material. A first ever wall-coated cell clock was demonstrated with good short-term frequency stability. The medium- to long-term stability was found to be limited by the temperature coefficient (TC) of the coating material itself. This work gave the insight to important features to be considered in future anti-relaxation coating materials for atomic standards. The second novel approach involves using a bigger cell (12 cm3) within a newly developed, improved MWR towards a high-performance atomic standard. Adopting a larger cell gives a higher atomic Q-factor signal that improves the short-term clock stability. In this approach, the cell was filled with 87Rb and buffer gases. With this clock, we demonstrate the state-of-the-art short-term stability of <1.4×10−13 τ−1/2. Metrological quantitative measurements on parameters influencing the medium- to long-term stability were studied in view of next generation satellite navigation systems that demand a stability level of <1×10−14 at 10 4 s (equivalent to <1 ns/day). The potential of short-term stability and understanding of the limiting factors on medium- to long-term time scales demonstrated in this study pave the way for future work towards the commercialization of high-performance Rb atomic clocks for a variety of applications.
This thesis presents experimental studies on continuous-wave (CW) laser-microwave double-resonance (DR) spectroscopy and metrology in rubidium (87Rb) vapor cells in view of new high-performance, compact Rb-cell atomic clocks. The Rb vapor cell is confined inside a magnetron-type cavity microwave resonator (MWR). The CW DR spectroscopy involves two resonant electromagnetic fields that are operated simultaneously to interrogate the atoms - the optical field to polarize the atoms by optical pumping, and the microwave field to drive the ground-state hyperfine clock transition that serves as an atomic frequency reference. Details on characterization of compact laser heads and microwave synthesizers used in this work are presented. The vapor cell standards are useful in our everyday lives for applications ranging from telecommunications, navigation, metrology etc. In view of improving the performances of the Rb cell standards, two different clock approaches were studied in detail: The first one is on use of vapor cells (1.4 cm3) whose inner walls are coated with anti-relaxation material. A first ever wall-coated cell clock was demonstrated with good short-term frequency stability. The medium- to long-term stability was found to be limited by the temperature coefficient (TC) of the coating material itself. This work gave the insight to important features to be considered in future anti-relaxation coating materials for atomic standards. The second novel approach involves using a bigger cell (12 cm3) within a newly developed, improved MWR towards a high-performance atomic standard. Adopting a larger cell gives a higher atomic Q-factor signal that improves the short-term clock stability. In this approach, the cell was filled with 87Rb and buffer gases. With this clock, we demonstrate the state-of-the-art short-term stability of <1.4×10−13 τ−1/2. Metrological quantitative measurements on parameters influencing the medium- to long-term stability were studied in view of next generation satellite navigation systems that demand a stability level of <1×10−14 at 10 4 s (equivalent to <1 ns/day). The potential of short-term stability and understanding of the limiting factors on medium- to long-term time scales demonstrated in this study pave the way for future work towards the commercialization of high-performance Rb atomic clocks for a variety of applications.
Distributed feedback (DFB) laser chips have recently become available at wavelengths that match the D1 and D2 resonance transitions of alkaline atoms. We investigated the spectral properties, tuning characteristics and modulation behavior of continuous wave, single-mode DFB diodes at 778-780 nm and performed high-resolution spectroscopy of Rubidium vapor. The mode-hop free tuning range of the DFB diodes was as large as 2.4 nm (1186 GHz). The line width of the laser diodes was examined both with a heterodyne beat experiment and with high-resolution Doppler-free two photon spectroscopy, yielding a half width of 2-2.5 MHz. The saturation spectra of the D2-line of 85Rb and 87Rb were recorded with a resolution close to the natural line width. The emission frequency was actively stabilized to Doppler-free transitions with a relative accuracy of better than 4 parts in 109 using commercially available servo devices only. The output power of 80 mW was sufficient to allow for two photon spectroscopy of the 5S-5D-transition of 87Rb. We conclude that the performance of the DFB laser equals that of grating-stabilized external-cavity diode lasers (ECDLs), without the mechanical complexity of the latter systems. The DFB diode is thus well-suited to high-resolution applications in alkaline spectroscopy, including laser cooling and optical manipulation of ultra-cold atoms.