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arXiv:cond-mat/0310687 · Journal of Physics B Atomic Molecular and Optical Physics

Imaging of spinor gases

Iacopo Carusotto, Erich J. Mueller

Published Mar 24, 2004• 42 citations
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Abstract

We explore the dielectric properties of spinor condensates. Gases with vector (nematic) order, such as spin-1 condensates with ferromagnetic (antiferromagnetic) interactions, display optical activity (birefringence). This optical activity/birefringence is respectively seen for light detuned from resonance by a frequency which is not too large compared with the fine/hyperfine structure. Careful tuning of the light frequency can isolate either of these two effects. These features can be used to image spin textures in clouds of spin-1 bosons, and to discern states showing different types of spin order.

DOI
10.1088/0953-4075/37/7/058

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In this thesis, we study theoretically and in experimentally the properties of spin-1 Bose-Einstein condensates with antiferromagnetic interactions realized in the ultra-cold sodium gases confined in optical dipole traps. We present in detail how to realize, diagnose and control the spinor Bose-Einstein condensates in our experiment. In order to describe the condensate, a mean-field theory is first adopted. This theory predicts a phase transition when changing the magnetic field $B$. The predictions of the mean-field theory agree very well with most of our experimental results, including the values of the critical magnetic field $B_c$, asymptotic values of $n_0$ (relative atom number in $m_F=0$ state) at large $B$ and the phase diagram of $n_0$. However, for small magnetization and small magnetic fields, we find abnormally large fluctuations (super-Poissonian) of $n_0$. In order to describe these large fluctuations, we develop a full quantum statistical description for the spinor condensate at finite temperature. To describe uncondensed thermal atoms (also present in the same trap), we use the ``semi-ideal" Hartree-Fock approximation to deal with the interactions between the condensate atoms and the thermal ones. The experimental results lead us to introduce two kinds of temperatures, the ``spin temperature" $T_s$ and the ``kinetic temperature" $T_k$ with $T_s\ll T_k$, characterizing respectively the fluctuaitons of the condensate spin and the thermal gas. We conclude that the system is reaching a quasi-equilibrium states, where different degrees of freedom reach equilibrium by separate mechanisms but where the mutual thermalization does not occur over the lifetime of the cloud.

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We explore the dielectric properties of spinor condensates. Gases with vector (nematic) order, such as spin-1 condensates with ferromagnetic (antiferromagnetic) interactions, display optical activity (birefringence). This optical activity/birefringence is respectively seen for light detuned from resonance by a frequency which is not too large compared with the fine/hyperfine structure. Careful tuning of the light frequency can isolate either of these two effects. These features can be used to image spin textures in clouds of spin-1 bosons, and to discern states showing different types of spin order.
Large spin systems can exhibit unconventional types of magnetic ordering, different from the ferromagnetic or N\'eel-like antiferromagnetic order commonly found in spin 1/2 systems. Spin-nematic phases, for instance, do not break time-reversal invariance, and their magnetic order parameter is characterized by a second-rank tensor with the symmetry of an ellipsoid. Here we show direct experimental evidence of spin-nematic ordering in a spin 1 Bose-Einstein condensate of sodium atoms with antiferromagnetic interactions. In a mean field description this order is enforced by locking the relative phase between spin components. We reveal this mechanism by studying the spin noise after a spin rotation, which is shown to contain information hidden when looking only at averages. The method should be applicable to high-spin systems in order to reveal complex magnetic phases.
Slowly rotating spin-1 Bose-Einstein condensates are studied through a variational approach based upon lowest Landau level calculus. The author finds that in a gas with ferromagnetic interactions, such as 87Rb^{87}\mathrm{Rb}87Rb, angular momentum is predominantly carried by clusters of two different types of skyrmion textures in the spin-vector order parameter. Conversely, in a gas with antiferromagnetic interactions, such as 23Na^{23}\mathrm{Na}23Na, angular momentum is carried by $\ensuremath{\pi}$ disclinations in the nematic order parameter which arises from spin fluctuations. For experimentally relevant parameters, the cores of these $\ensuremath{\pi}$ disclinations are ferromagnetic, and can be imaged with polarized light.
Spinor Bose Einstein condensates have widely been sought after as perfect emulators of condensed matter phenomena, providing widely tunable and highly controlled systems. Utilizing a novel spin sensitive phase contrast imaging technique, the vector magnetization is measured in-situ with high spatial and temporal resolution and applied to a number of experiments. Using optically trapped F = 1 87Rb spinor condensates, the equilibrium phase diagram of a spin-1 Bose gas is quantitatively explored by observing the evolution of unmagnetized spin textures and their thermal equilibrium properties. Spin domain coarsening and a strong dependence of the spin configuration on the quadratic Zeeman shift is observed, supporting the predicted mean-field equilibrium phase diagram for small values of the quadratic shift. Additionally, spinor Bose gases are demonstrated to be an effective tool in calibrating and characterizing experimental imaging systems. Sinusoidal test patterns of varying pitch are created and used to extract the modulation transfer function and quantify optical aberrations which are of immense importance in systems which claim to have high spatial resolution. Lastly we realize an optical kagome geometry in a two-dimensional optical superlattice with a scalar Bose gases. The optical superlattice can be tuned between various geometries, including kagome, one-dimensional stripe, and decorated triangular lattice. Using atom optics we characterize the various geometries and demonstrate the versatility of this optical superlattice. The kagome geometry presents a new experimental arena for studies of geometrically frustrated systems.
This chapter focuses on ultracold gases of atoms that possess internal spin structure. First, it considers spinor interactions, and then turns to trapped spinor Bose–Einstein condensates. In particular, the chapter discusses various possible mean field phases, spin textures, and topological defects. Next, it describes bosonic spinor gases in optical lattices, effective Hamiltonians, and possible quantum phases. Finally, spinor Fermi gases in optical lattices for spins larger than ½ are discussed.
In this thesis, we study theoretically and in experimentally the properties of spin-1 Bose-Einstein condensates with antiferromagnetic interactions realized in the ultra-cold sodium gases confined in optical dipole traps. We present in detail how to realize, diagnose and control the spinor Bose-Einstein condensates in our experiment. In order to describe the condensate, a mean-field theory is first adopted. This theory predicts a phase transition when changing the magnetic field BBB. The predictions of the mean-field theory agree very well with most of our experimental results, including the values of the critical magnetic field BcB_cBc​, asymptotic values of n0n_0n0​ (relative atom number in mF=0m_F=0mF​=0 state) at large BBB and the phase diagram of n0n_0n0​. However, for small magnetization and small magnetic fields, we find abnormally large fluctuations (super-Poissonian) of n0n_0n0​. In order to describe these large fluctuations, we develop a full quantum statistical description for the spinor condensate at finite temperature. To describe uncondensed thermal atoms (also present in the same trap), we use the ``semi-ideal" Hartree-Fock approximation to deal with the interactions between the condensate atoms and the thermal ones. The experimental results lead us to introduce two kinds of temperatures, the ``spin temperature" TsT_sTs​ and the ``kinetic temperature" TkT_kTk​ with Ts≪TkT_s\ll T_kTs​≪Tk​, characterizing respectively the fluctuaitons of the condensate spin and the thermal gas. We conclude that the system is reaching a quasi-equilibrium states, where different degrees of freedom reach equilibrium by separate mechanisms but where the mutual thermalization does not occur over the lifetime of the cloud.