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Theoretical and experimental study of spin-1 antiferromagnetic Bose-Einstein Condensates

Shao, Lingxuan

Published Jul 4, 2014• 1 citation
OpenAlex

Abstract

In this thesis, we study theoretically and in experimentally the properties of spin-1 Bose-Einstein condensates with antiferromagnetic interactions realized in the ultra-cold sodium gases confined in optical dipole traps. We present in detail how to realize, diagnose and control the spinor Bose-Einstein condensates in our experiment. In order to describe the condensate, a mean-field theory is first adopted. This theory predicts a phase transition when changing the magnetic field $B$. The predictions of the mean-field theory agree very well with most of our experimental results, including the values of the critical magnetic field $B_c$, asymptotic values of $n_0$ (relative atom number in $m_F=0$ state) at large $B$ and the phase diagram of $n_0$. However, for small magnetization and small magnetic fields, we find abnormally large fluctuations (super-Poissonian) of $n_0$. In order to describe these large fluctuations, we develop a full quantum statistical description for the spinor condensate at finite temperature. To describe uncondensed thermal atoms (also present in the same trap), we use the ``semi-ideal" Hartree-Fock approximation to deal with the interactions between the condensate atoms and the thermal ones. The experimental results lead us to introduce two kinds of temperatures, the ``spin temperature" $T_s$ and the ``kinetic temperature" $T_k$ with $T_s\ll T_k$, characterizing respectively the fluctuaitons of the condensate spin and the thermal gas. We conclude that the system is reaching a quasi-equilibrium states, where different degrees of freedom reach equilibrium by separate mechanisms but where the mutual thermalization does not occur over the lifetime of the cloud.

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In this thesis, we study theoretically and in experimentally the properties of spin-1 Bose-Einstein condensates with antiferromagnetic interactions realized in the ultra-cold sodium gases confined in optical dipole traps. We present in detail how to realize, diagnose and control the spinor Bose-Einstein condensates in our experiment. In order to describe the condensate, a mean-field theory is first adopted. This theory predicts a phase transition when changing the magnetic field BBB. The predictions of the mean-field theory agree very well with most of our experimental results, including the values of the critical magnetic field BcB_cBc​, asymptotic values of n0n_0n0​ (relative atom number in mF=0m_F=0mF​=0 state) at large BBB and the phase diagram of n0n_0n0​. However, for small magnetization and small magnetic fields, we find abnormally large fluctuations (super-Poissonian) of n0n_0n0​. In order to describe these large fluctuations, we develop a full quantum statistical description for the spinor condensate at finite temperature. To describe uncondensed thermal atoms (also present in the same trap), we use the semi-ideal" Hartree-Fock approximation to deal with the interactions between the condensate atoms and the thermal ones. The experimental results lead us to introduce two kinds of temperatures, the spin temperature" TsT_sTs​ and the ``kinetic temperature" TkT_kTk​ with Ts≪TkT_s\ll T_kTs​≪Tk​, characterizing respectively the fluctuaitons of the condensate spin and the thermal gas. We conclude that the system is reaching a quasi-equilibrium states, where different degrees of freedom reach equilibrium by separate mechanisms but where the mutual thermalization does not occur over the lifetime of the cloud.
Ultra-cold spinor Bose gases present rich physics due to the special combination of superfluidity and magnetism in a quantum system. This system was first realized in 1998 by confining a Bose-Einstein condensate in an all-optical trap.\nIn this thesis, we consider the fluctuations of observable quantities in a spin-1 Bose gas. Understanding how fluctuations arise due to the spin excitations of the condensate is important because it offers an insight into how measurement noise reveals the many-body physics of the system.\nTo begin, we present the mean-field and Bogoliubov theory of a uniform spin-1 Bose gas subject to a constant magnetic field, describing the condensate and its low-energy collective excitations.\nWe then develop a formalism to describe the fluctuations in a general density-like observable. We start from the two-point correlation function and cast it in the form of a generalised static structure factor determined by the three Bogoliubov quasiparticle excitation branches. We derive analytic results for the fluctuation amplitudes and the temperature-dependent static structure factors for observables of total density and the three spin densities.\nFor all four magnetic phases, we analyse the spinor order parameter and quasiparticle spectra while numerically mapping out the fluctuation amplitudes and static structure factors for the total and spin density operators.\nWe describe the fluctuations in experimental measurements made within finite cells, which is an important step to making meaningful predictions for experiments. We consider cylindrical cells and gaussian cells as two limiting cases. We apply this analysis to an experimentally realisable system of a quasi-2D spinor gas in a harmonic trap, comparing extensive numeric results with analytic limits.
In this thesis we investigate the static, dynamic, and thermodynamic properties\nof atomic spin-1 Bose gases in external magnetic fields. At low magnetic fields\nthe properties of single-component, or scalar condensates, are essentially\nunaffected but can become significantly altered for spinor Bose condensates as\nshown by our studies.\n\nWe first study the Bose-Einstein condensation of trapped spin-1 Bose gases by\nemploying the Hartree-Fock approximation and the two-fluid model within a mean\nfield approximation. Our detailed investigation reveals that the\nferromagnetically interacting spin-1 condensates exhibit triple condensations\nwhile the antiferromagnetically interacting ones show double condensations.\n\nThe ground state structure of homogeneous and trapped spin-1 Bose condensates\nwith ferromagnetic and antiferromagnetic interactions at zero temperature in\nmagnetic fields are then investigated systematically. We further illuminate the\nimportant effect of quadratic Zeeman shift which causes a preferred occupation\nof the $|m_F=0\nangle$ state through spin exchange collisions, $2|m_F=0\nangle\nleftrightarrow |m_F=1\nangle + |m_F=-1\nangle$.\n\nWe also present detailed studies of the off-equilibrium coherent dynamics of\nspin-1 Bose condensates in magnetic fields within the single spatial mode\napproximation. Dynamical instabilities of the off-equilibrium oscillations are\nshown to be responsible for the formation of multiple domains as recently\nobserved in several 87^{87}87Rb experiments.\n\nFinally, we discuss briefly excited condensate states, or soliton-like states,\nin cigar-shaped spin-1 Bose condensates with an effective quasi-1D description,\nusing the developed nonpolynomial Schr"odinger equation.
Spinor Bose-Einstein condensates under external magnetic fields exhibit well-characterized spin domains of its ground state due to spin-dependent interactions. At low temperatures, collision-induced spin-mixing instabilities may promote the condensate to dwell into metastable states occurring near the phase boundaries. In this paper, we study theoretically the metastable spin-phase diagram of a spin-1 antiferromagnetic Bose-Einstein condensate at zero and finite temperatures. The approach makes use of Hartree-Fock theory and exploits the symmetry of the Hamiltonian and of the order parameters yielding a closed system of transcendental equations for the free energy, fully avoiding the use of self-consistency methods. Our results are consistent with recent experiments and allow us to explain qualitatively the different types of observed quench dynamics. In addition, we found that similar phenomena should occur in antiferromagnetic spinor condensates with a sudden change in the temperature. It is shown also that the increase in temperature induces a traceable shift of the ferromagnetic-polar transition boundary, behavior previously not noted by self-consistent mean-field calculations.
This thesis discusses non-equilibrium phenomena in antiferromagnetic spinor quantum gases. We investigate, both experimentally and theoretically, the quench dynamics of antiferromagnetic spinor Bose-Einstein condensates in the vicinity of a zero temperature quantum phase transition. A microwave dressing field was used as a novel tool to access the polar to antiferrmagnetic quantum phase transition at the quadratic Zeeman shift, q=0. By performing instantaneous quenches across the phase transition,a dynamical instability was induced in the atomic cloud. This lead to pair formation and rapid amplification of spin +/-1 atoms through spin-mixing collisions. The spatial ordering kinetics in the vicinity of the phase transition was quantified by performing the local spin measurement. The coarsening dynamics was observed for the instability for q < 0, as it nucleated small domains that grew to the axial size of the cloud. Rich nonequilibrium behavior was observed in the form of growth and decay of both nematic and magnetic spin waves, following the quench. The spatiotemporal evolution was characterized through two particle correlations between atoms in each pair of spin states, which revealed dramatic differences between the dynamics of the spin correlations and those of the spin populations. \nFinally, we demonstrate the remarkable influence of linear Zeeman term on non-equilibrium dynamics of spinor Bose-Einstein condensates. We show that contrary to prior understanding magnetic field gradient actually suppresses the tendency of spin 0 state to separate into spin +/-1 state. This reconciles the Bogoliubov discrepancies and leads to a dramatic sharpening of the transition point, resulting in a resolution at the 1 Hz level. Our results point to the use of dynamics, rather than equilibrium quantities for high precision measurements of phase transitions in quantum gases.
Bose-Einstein condensation (BEC) is a phenomenon in which identical bosons occupy the same quantum state below a certain critical temperature. A hallmark of BEC is the coherence between particles every particle shares the same quantum wavefunction and phase. This coherence has been demonstrated for the external (motional) degrees of freedom of the atomic condensates by interfering two condensates. In this thesis, the coherence is shown to extend to the internal spin degrees of freedom of a spin-1 Bose gas evidenced by the observed coherent and reversible spin-changing collisions. The observed coherent dynamics are analogous to Josephson oscillations in weakly connected superconductors and represent a type of matter-wave four-wave mixing. Control of the coherent evolution of the system using magnetic fields is also demonstrated. The studies on spinor condensates begin by creating spinor condensates directly using all-optical approaches that were first developed in our laboratory. All-optical formation of Bose-Einstein condensates (BEC) in 1D optical lattice and single focus trap geometries are developed and presented. These techniques offer considerable flexibility and speed compared to magnetic trap approaches, and the trapping potential can be essentially spin-independent and are ideally suited for studying spinor condensates. Using condensates with well-defined initial non-equilibrium spin configuration, spin mixing of F = 1 and F = 2 spinor condensates of rubidium-87 atoms confined in an optical trap is observed. The equilibrium spin configuration in the F = 1 manifold confirms that 87Rb is ferromagnetic. The coherent spinor dynamics are demonstrated by initiating spin mixing deterministically with a non-stationary spin population configuration. Finally, the interplay between the coherent spin mixing and spatial dynamics in spin-1 condensates with ferromagnetic interactions is investigated.
In this thesis, we present some experiments realized with ultracold gases of sodium atoms, trapped at the intersect between two laser beams. At very low temperature, the discretization of energy and the indistinguishability of particles, lead to a new state of matter, a Bose-Einstein condensate. This remarkable phenomenon was initially introduced to describe an ideal gas, that is to say with no interactions between its constituents. Here, we are interested in the effects of the interactions between the atoms. More precisely, our atoms carry a spin 1, and we focus on the collective spin state, in a regime where the spatial degrees of freedom are frozen. Two important results that we present were obtained by embedding the condensate in a nearly vanishing magnetic field. In that regime, interactions dominate and favor the emergence of strongly correlated states. In a first series of experiment, the magnetic field is suddenly decreased to bring the system out-of-equilibrium. The ensuing relaxation dynamics leads to a stationnary state that can be well described by a Gibbs ensemble. In a second experiment, the field is slowly reduced, in order to follow the ground state of the system. We thereby produce a fragmented condensate, which possesses the remarkable feature of being invariant upon spin rotations. The restoration of this symmetry, always broken by single (i.e. nonfragmented) condensates, is driven by the pairing of atoms in singlet states.