In Chapter 1, we introduced the standard rate equations (SRE) for a laser containing two-level atoms between which stimulated emission is possible. But real lasers exhibit much more complicated energy level schemes. Throughout this chapter, we consider several models in which the light–matter interaction is described by population equations for all the levels involved in the laser operation. Although they are mathematically more complicated, we shall investigate these equations in the same way as in Chapter 1, i.e. by formulating dimensionless equations and by analyzing the stability properties of the steady states. The basic ingredients of the SRE model used up to here, namely pumping and relaxation processes, play key roles in the efficiency of lasers. But already during the pioneering days of the laser, it appeared important to investigate three- and four-level models in order to obtain more reliable information on quantities such as the power conversion efficiency or the response time. The common extensions of the two-level SRE typically consider an open two-level system, or three- or four-level systems, depending on the nature of the active medium. Restriction to as few as four levels is again a crude simplification of the complex population dynamics occurring in most lasers. But it is rather surprising to see how good these simple kinetic models are. As we demonstrate by studying specific examples, the solution of the three- or four-level rate equations differs only slightly from the solution of the SRE.
In Chapter 1, we introduced the standard rate equations (SRE) for a laser containing two-level atoms between which stimulated emission is possible. But real lasers exhibit much more complicated energy level schemes. Throughout this chapter, we consider several models in which the light–matter interaction is described by population equations for all the levels involved in the laser operation. Although they are mathematically more complicated, we shall investigate these equations in the same way as in Chapter 1, i.e. by formulating dimensionless equations and by analyzing the stability properties of the steady states. The basic ingredients of the SRE model used up to here, namely pumping and relaxation processes, play key roles in the efficiency of lasers. But already during the pioneering days of the laser, it appeared important to investigate three- and four-level models in order to obtain more reliable information on quantities such as the power conversion efficiency or the response time. The common extensions of the two-level SRE typically consider an open two-level system, or three- or four-level systems, depending on the nature of the active medium. Restriction to as few as four levels is again a crude simplification of the complex population dynamics occurring in most lasers. But it is rather surprising to see how good these simple kinetic models are. As we demonstrate by studying specific examples, the solution of the three- or four-level rate equations differs only slightly from the solution of the SRE.
Modeling lasers may be realized with different levels of sophistication. Rigorously it requires a full quantum treatment but many laser dynamical properties may be captured by semiclassical or even purely classical approaches. In this book we deliberately chose the simplest point of view, i.e. purely classical equations, and try to extract analytically as much information as possible. The basic framework of our approach is provided by the rate equations . In their simplest version, they apply to an idealized active system consisting of only two energy levels coupled to a reservoir. They were introduced as soon as the laser was discovered to explain (regular or irregular, damped or undamped) intensity spikes commonly seen with solid state lasers (for a historical review, see the introduction in). These rate equations are discussed and sometimes derived from a semiclassical theory in textbooks on lasers. They capture the essential features of the response of a single-mode laser and they may be modified to account for specific effects such as the modulation of a parameter or optical feedback. The most basic processes involved in laser operation are schematically represented in Figure 1.1. N 1 and N 2 denote the number of atoms in the ground and excited levels, respectively. The process of light–matter interaction is restricted to stimulated emission and absorption.
This chapter begins with a heuristic derivation of atomic population rate equations which include changes to level populations due to stimulated transitions as well as level relaxations and pump. These equations are used to study the saturation of population inversion with increasing light intensity and its dependence on the type of gain medium (three-level gain media vs. four-level gain media), lineshape and nature of line broadening (homogeneous vs inhomogeneous broadening). How saturation affects lineshape and thus gain and absorption giving rise to phenomena like power broadening and spectral hole burning is also discussed. The chapter summarizes the equations of motion for atomic polarization, inversion and the cavity field describing their nonlinear dynamical coupling. These equations, known as the Maxwell-Bloch equations, provide a complete description of atom-field interaction in a laser. Approximations of these equations, including the rate equation approximation, to deal with different laser classes are briefly described. These will be used in the next few chapters to explore and understand the rich and varied behavior of lasers. The chapter ends with a summary of select gain media for different types of commonly used lasers.
The adiabatic elimination principle [91, 92] is universal in the area of nonlinear dissipative dynamical systems, and its importance arises from the fact that it allows one to reduce the number of the equations which govern the dynamics of the system. We introduce it at this stage in the book in order to be able to describe the optical pumping mechanisms which can be exerted to attain population inversion. However, this principle will be applied repeatedly in the following chapters for other purposes. In the first subsection we describe the principle in general, while the following subsections concern the issue of optical pumping. We show first that it is not possible to obtain population inversion between the two levels of the lasing transition if the pump involves only these two levels. Next we illustrate the three-level pumping scheme and the four-level pumping scheme. We demonstrate that, by adiabatically eliminating the probabilities of the additional energy levels, one arrives at an equation identical to Eq. (4.12), which, for appropriate ranges of values of the parameters involved in the pumping, allows one to obtain population inversion. General formulation of the principle In a dissipative dynamical system the dynamical variables undergo relaxation processes associated with suitable rate constants such as, for example, the rate γ ⊥ for the normalized atomic polarization P and the rate γ ∥ for the normalized population difference D . The inverses of these rates provide the time scales which characterize the evolution of each variable. Therefore we can distinguish a set of fast variables , which evolve over short time scales and are therefore characterized by large relaxation rates, and a set of slow variables , which display small relaxation rates. A remarkable simplification in the analysis of dynamical systems is obtained by using the technique of adiabatic elimination of fast variables, which Haken considered as a basis for the discipline which he formulated and called Synergetics [91, 92].
In the first section we discuss the stationary solutions for a laser with an injected signal, the active counterpart of the optical bistability analyzed in Chapter 11. Next, in Section 13.2 we consider another very interesting system, namely a laser with a saturable absorber, a free-running laser in which the optical cavity contains a passive medium in addition to the active medium. The single-mode model for this system can be constructed by combining the single-mode models for the free-running laser and for optical bistability. The discussion is then focussed on its stationary states. In Section 13.3 we return to the single-mode model for optical bistability and, by introducing an appropriate “cubic limit” on the parameters in play, we derive a cubic model for dispersive optical bistability with two-level atoms. The stationary equation for such a model formally coincides with that derived and discussed for a Kerr medium in Section 11.2. In the last section we start from the equations for a quadratic nonlinear medium in the degenerate configuration derived in Chapter 6 and combine them with the appropriate boundary conditions for the two field envelopes in play, assuming that the quadratic medium is contained in a ring cavity as happens in an optical parametric oscillator or in second-harmonic generation in a cavity. Next, by introducing the low-transmission limit and the single-mode limit we derive a two-mode model that describes the dynamics of a degenerate optical parametric oscillator or of second-harmonic generation in a cavity. Finally, for the case of a parametric oscillator we illustrate extensively the stationary solutions of the equations. A laser with an injected signal From a technical point of view, this system is interesting because of the possibility of stabilizing the frequency and the phase of separate lasers by taking advantage of the known affinity of nonlinear oscillators to lock onto a periodic forcing element. In 1972 Spencer and Lamb [125] predicted the possibility of bistable behavior in a laser with an injected signal before the surge of interest in optical bistability in the passive configuration.
POPULATION RATE EQUATIONS From the discussion in the preceding chapter, it is clear that population inversion is the basic condition for an optical gain. For any system in its normal state in thermal equilibrium, a low-energy level is always more populated than a high-energy level, hence there is no population inversion. Population inversion in a system can only be accomplished through a process called pumping by actively exciting the atoms in a low-energy level to a high-energy level. If left alone, the atoms in a system relax to thermal equilibrium. Therefore, population inversion is a nonequilibrium state that cannot be sustained without active pumping. To keep a constant optical gain, continuous pumping is required to maintain population inversion. This condition is clearly consistent with the law of conservation of energy: amplification of an optical wave leads to an increase in optical energy, which is possible only if the required energy is supplied by a source. Pumping is the process that supplies energy to the gain medium for the amplification of an optical wave. There are many different pumping techniques, including optical excitation, electric current injection, electric discharge, chemical reaction, and excitation with particle beams. The use of a specific pumping technique depends on the properties of the gain medium being pumped. The lasers and optical amplifiers of particular interest in photonic systems are made of either dielectric solid-state media doped with active ions, such as Nd:YAG and Er:glass fiber, or direct-gap semiconductors, such as GaAs and InP. For a dielectric gain medium, the most commonly used pumping technique is optical pumping using either an incoherent light source, such as a flashlamp or a light-emitting diode, or a coherent light source from another laser. A semiconductor gain medium can also be optically pumped, but it is usually pumped by electric current injection. In this section, we consider the general conditions for pumping to achieve population inversion. Detailed pumping mechanisms and physical setups are not addressed here because they depend on the specific gain medium used in a particular application. The net rate of increase of the population density in a given energy level is described by a rate equation. As we shall see below, pumping for population inversion in any practical gain medium always requires the participation of more than two energy levels.
The steady-state intensity distribution for a laser operating somewhat above threshold is determined by solving a master equation. The master equation describes the interaction between a single radiation mode and N two-level atoms, it contains the effects of pumping and radiation loss from the cavity, and it is applicable to both homogeneous and Doppler broadening. Forms of the master equation applicable to both three- and four-level lasers are considered. Solutions are obtained under the assumption that the distribution of atoms and radiation intensity is a bivariate Gaussian. Fluctuations in the output of giant-pulse lasers are also considered.