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Physical Review A

Operation of a two-mode laser in a three-level atomic system with a common upper level

Shi-yao Chu, Da-chun Su

Published Jun 1, 1982• 24 citations
Publisher

Abstract

The quantum theory of the three-energy-level two-mode laser in which all the levels are being pumped is investigated and the master equation of the laser operation is obtained. It contains two variables, ${n}_{1}$, the photon number of the first mode, and ${n}_{2}$, the photon number of the second mode. There appear four terms in the master equation which represent two-photon processes between the two modes, the absorption of a photon from one mode, and emission of a photon to the other. They are absent in the single-mode case and in the two-mode case with pumping only to the upper level. The master equation can be represented by a diagram of probability in two dimensions which can be extended to infinity, and each arrow of it represents a term on the right-hand side of the master equation. By summing each variable (${n}_{1}$ or ${n}_{2}$) of the master equation, two equations can be obtained. Each equation contains only one variable, and can be expressed by a diagram of probability flow in one dimension. By considering the correspondence between macroscopic equilibrium and microscopic detailed balance the equations of motion in the steady state are obtained. By introducing a parameter $H$, the equation of motion is simplified and a formal solution can be deduced which is dependent on $H$. It appears that the parameter $H$ cannot be fully determined, but some properties of it can be deduced which prove that the introduction of $H$ is reasonable. The operation characteristics of the laser under different conditions are discussed on the basis of the formal solution: among them are the threshold condition, the condition for one-mode operation, and the change of the photon-statistical distribution. We especially discuss the laser output power curves under two-mode operation above threshold. The curve of one mode, which oscillates first, shows a bending-down phenomenon as the excitation increases when the other mode goes beyond its threshold as demonstrated experimentally by Otsuka. This phenomenon is explained qualitatively and is attributed to the two-photon processes between the two modes.

DOI
10.1103/physreva.25.3169

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The quantum theory of the three-energy-level two-mode laser in which all the levels are being pumped is investigated and the master equation of the laser operation is obtained. It contains two variables, n1{n}_{1}n1​, the photon number of the first mode, and n2{n}_{2}n2​, the photon number of the second mode. There appear four terms in the master equation which represent two-photon processes between the two modes, the absorption of a photon from one mode, and emission of a photon to the other. They are absent in the single-mode case and in the two-mode case with pumping only to the upper level. The master equation can be represented by a diagram of probability in two dimensions which can be extended to infinity, and each arrow of it represents a term on the right-hand side of the master equation. By summing each variable (n1{n}_{1}n1​ or n2{n}_{2}n2​) of the master equation, two equations can be obtained. Each equation contains only one variable, and can be expressed by a diagram of probability flow in one dimension. By considering the correspondence between macroscopic equilibrium and microscopic detailed balance the equations of motion in the steady state are obtained. By introducing a parameter HHH, the equation of motion is simplified and a formal solution can be deduced which is dependent on HHH. It appears that the parameter HHH cannot be fully determined, but some properties of it can be deduced which prove that the introduction of HHH is reasonable. The operation characteristics of the laser under different conditions are discussed on the basis of the formal solution: among them are the threshold condition, the condition for one-mode operation, and the change of the photon-statistical distribution. We especially discuss the laser output power curves under two-mode operation above threshold. The curve of one mode, which oscillates first, shows a bending-down phenomenon as the excitation increases when the other mode goes beyond its threshold as demonstrated experimentally by Otsuka. This phenomenon is explained qualitatively and is attributed to the two-photon processes between the two modes.
The quantum theory of two-level atom single-mode laser system of Sargent, Scully and Lamb is extended to two-mode laser in a three-level atomic system with common lower level, and master equation is obtained for the system with all the three levels being pumped. There appear four terms in the master equation that are absent in the single-mode case and those interpreted as 2-photon processes play an especial role in the present case. The master equation is represented by a probability flow diagram in two-dimensions with the photon numbers n1 and n2 of the two-mode as variables. The probability flow diagram can be extended to infinity, and each arrow of it represents a term of the right hand side of master equation. By taking sum over one of the variables n1 or n2, the master equation is reduced to two equations, each of them can be represented by an one-dimensional probability flow diagram. The equation of motion under steady state is obtained by considering the correspondence between the macroscopic balance and the microscopic balance.A parameter H is introduced to reduce the equation of motion and to facilitate the mathematical procedure and a formal solution is thus obtained. Using the equation of motion and its formal solution various operation characteristics are discussed. Among them are: the threshold condition for each mode; the condition of only one mode operation; the variation of photon statistics between single-mode operation and two-mode operation and the variation of photon statistics with lower level being pumped and not pumped.
The density operator theory and method are used to extend the fully quantum-mechanical theory of the two-level single-mode laser advanced by Sargent, Scully and Lamb (1974) to the homogeneously broadened four-level atomic system so that the master equation of the three-mode laser operation for this system is obtained. The steady-state operation characteristics of the laser in different cases are discussed and compared. Especially, pictorial comparison and discussion of the quantum-statistical properties of the laser are carried out by means of numerical computation. Meanwhile some experimental results obtained by Otsuka (1978) are qualitatively explained.
A quantum theory of a two-photon laser in a three-level atomic system of the cascade type is presented starting from an original microscopic Hamiltonian. The master equation of the laser operation is derived by using the method of Scully and Lamb [Phys. Rev. A 159, 208 (1967)] for a single-mode laser containing a two-level medium. The photon-number distribution of the laser is studied in detail. The curve of the distribution may have a two-peak structure. One of the peaks located at the origin comes from the single-photon process and reflects the thermal property of the laser, while another comes from the two-photon process and reflects the coherent property of the laser. We cannot find an exact criterion for the threshold of the two-photon laser. The two-photon laser can approximately be considered as a coherent state for certain values of A/C, which can even be much smaller than the threshold for the nonresonant single-mode laser in a two-level system, but it is much larger than the threshold for the resonant one.
We have solved a master equation to obtain the diagonal elements of the density matrix for laser light. The master equation represents a generalization of a master equation derived earlier for a single radiation mode interacting with NNN stationary two-level atoms. The generalization takes into account the pumping scheme which characterizes a three-level laser. For positive temperatures and a lossless cavity, the equilibrium solution of the master equation gives the correct statistical-mechanical description of the atoms and radiation. For negative temperatures, the distribution function for the number of photons in the mode is either exponential or peaked, depending on whether the laser is operating below or above threshold. The calculated intensity fluctuations are in good agreement with semiclassical results for lasers operating slightly above threshold.
We have solved a master equation to obtain the diagonal elements of the density matrix for laser light. The master equation represents a generalization of a master equation derived earlier for a single radiation mode interacting with NNN stationary two-level atoms. The generalization takes into account the pumping scheme which characterizes a three-level laser. For positive temperatures and a lossless cavity, the equilibrium solution of the master equation gives the correct statistical-mechanical description of the atoms and radiation. For negative temperatures, the distribution function for the number of photons in the mode is either exponential or peaked, depending on whether the laser is operating below or above threshold. The calculated intensity fluctuations are in good agreement with semiclassical results for lasers operating slightly above threshold.
The fully quantum-mechanical model of a single-mode laser is examined. A previously introduced method of solution where both the pump and loss reservoirs are treated simultaneously as a weak perturbation of the atom-light system is employed. This method is similar to perturbation theory for degenerate systems in that the reservoirs remove the nonuniqueness (degeneracy) of the steady state of the unperturbed atom-light system. In the limit of weak reservoir coupling, the exact steady-state solution of the master equation is derived. This solution still contains the atomic variables explicitly and therefore remains valid even in situations where the conventional adiabatic elimination of the atomic variables is no longer possible. A compact discrete representation of the master equation in terms of atomic occupation numbers and photon numbers is developed which allows one to perform all calculations in an elementary manner, requiring only appropriate summations over photon and occupation numbers. General exact relations are obtained for the steady-state probability distribution function p(n,m)p(n,m)p(n,m) to find nnn photons in the light field and mmm atoms in the excited state. Our solution constitutes the first steady-state laser distribution function that is valid for an arbitrary number of laser atoms and in the complete region from far below to far above threshold. It provides a quantitative criterion for the range of validity of approximate methods in laser theory.