This chapter begins with a heuristic derivation of atomic population rate equations which include changes to level populations due to stimulated transitions as well as level relaxations and pump. These equations are used to study the saturation of population inversion with increasing light intensity and its dependence on the type of gain medium (three-level gain media vs. four-level gain media), lineshape and nature of line broadening (homogeneous vs inhomogeneous broadening). How saturation affects lineshape and thus gain and absorption giving rise to phenomena like power broadening and spectral hole burning is also discussed. The chapter summarizes the equations of motion for atomic polarization, inversion and the cavity field describing their nonlinear dynamical coupling. These equations, known as the Maxwell-Bloch equations, provide a complete description of atom-field interaction in a laser. Approximations of these equations, including the rate equation approximation, to deal with different laser classes are briefly described. These will be used in the next few chapters to explore and understand the rich and varied behavior of lasers. The chapter ends with a summary of select gain media for different types of commonly used lasers.
This chapter begins with a heuristic derivation of atomic population rate equations which include changes to level populations due to stimulated transitions as well as level relaxations and pump. These equations are used to study the saturation of population inversion with increasing light intensity and its dependence on the type of gain medium (three-level gain media vs. four-level gain media), lineshape and nature of line broadening (homogeneous vs inhomogeneous broadening). How saturation affects lineshape and thus gain and absorption giving rise to phenomena like power broadening and spectral hole burning is also discussed. The chapter summarizes the equations of motion for atomic polarization, inversion and the cavity field describing their nonlinear dynamical coupling. These equations, known as the Maxwell-Bloch equations, provide a complete description of atom-field interaction in a laser. Approximations of these equations, including the rate equation approximation, to deal with different laser classes are briefly described. These will be used in the next few chapters to explore and understand the rich and varied behavior of lasers. The chapter ends with a summary of select gain media for different types of commonly used lasers.
Using Lamb's model, we analyze the effects of gain saturation by strong traveling-wave fields in dilute laser media. Using approximate solutions of an integral equation for the population inversion density (PID), the index of refraction and incremental gain are studied for arbitrarily strong fields. Effects of atomic motion are included for a Maxwellian velocity distribution, but pressure effects are neglected. The case of a monochromatic field leads to the saturation results of Gordon, White, and Rigden, which are studied as a function of frequency. For a small ratio of natural to Doppler linewidths, there is a transition from inhomogeneous to homogeneous broadening for sufficiently strong fields. An effect of particular interest is the generation of waves at $2{\ensuremath{\omega}}_{1}\ensuremath{-}{\ensuremath{\omega}}_{2}$, $2{\ensuremath{\omega}}_{2}\ensuremath{-}{\ensuremath{\omega}}_{1}$, and higher order sidebands by two strong input signals at ${\ensuremath{\omega}}_{1}$ and ${\ensuremath{\omega}}_{2}$. The source of the parametric gain at these frequencies is the time-dependent gain saturation due to the presence of multiple strong fields. For ${\ensuremath{\omega}}_{1}\ensuremath{-}{\ensuremath{\omega}}_{2}$ small compared to the decay rates ${\ensuremath{\gamma}}_{a}$ and ${\ensuremath{\gamma}}_{b}$ of the laser levels, the gain at these intermodulation sidebands is computed as a function of the field strengths. The limiting cases of homogeneous and inhomogeneous (due to atomic motion) broadening are studied in detail. These two cases give essentially the same results, for a given unsaturated gain. Numerical results indicate that a first-order side-band intensity at least 10% as large as that of the inducing fields can be easily observed in practice. The integral equation for the PID is converted into an infinite set of linear algebraic equations for a typical solid-state laser. The conditions under which this set of equations can be limited to a finite number is discussed, and the dependence of the sideband gain on ${\ensuremath{\omega}}_{1}\ensuremath{-}{\ensuremath{\omega}}_{2}$ is calculated. For large ${\ensuremath{\omega}}_{1}\ensuremath{-}{\ensuremath{\omega}}_{2}$, the gain at the mth sideband decreases as ${({\ensuremath{\omega}}_{1}\ensuremath{-}{\ensuremath{\omega}}_{2})}^{\ensuremath{-}m}$.
Using Lamb's model, we analyze the effects of gain saturation by strong traveling-wave fields in dilute laser media. Using approximate solutions of an integral equation for the population inversion density (PID), the index of refraction and incremental gain are studied for arbitrarily strong fields. Effects of atomic motion are included for a Maxwellian velocity distribution, but pressure effects are neglected. The case of a monochromatic field leads to the saturation results of Gordon, White, and Rigden, which are studied as a function of frequency. For a small ratio of natural to Doppler linewidths, there is a transition from inhomogeneous to homogeneous broadening for sufficiently strong fields. An effect of particular interest is the generation of waves at $2{\ensuremath{\omega}}_{1}\ensuremath{-}{\ensuremath{\omega}}_{2}$, $2{\ensuremath{\omega}}_{2}\ensuremath{-}{\ensuremath{\omega}}_{1}$, and higher order sidebands by two strong input signals at ${\ensuremath{\omega}}_{1}$ and ${\ensuremath{\omega}}_{2}$. The source of the parametric gain at these frequencies is the time-dependent gain saturation due to the presence of multiple strong fields. For ${\ensuremath{\omega}}_{1}\ensuremath{-}{\ensuremath{\omega}}_{2}$ small compared to the decay rates ${\ensuremath{\gamma}}_{a}$ and ${\ensuremath{\gamma}}_{b}$ of the laser levels, the gain at these intermodulation sidebands is computed as a function of the field strengths. The limiting cases of homogeneous and inhomogeneous (due to atomic motion) broadening are studied in detail. These two cases give essentially the same results, for a given unsaturated gain. Numerical results indicate that a first-order side-band intensity at least 10% as large as that of the inducing fields can be easily observed in practice. The integral equation for the PID is converted into an infinite set of linear algebraic equations for a typical solid-state laser. The conditions under which this set of equations can be limited to a finite number is discussed, and the dependence of the sideband gain on ${\ensuremath{\omega}}_{1}\ensuremath{-}{\ensuremath{\omega}}_{2}$ is calculated. For large ${\ensuremath{\omega}}_{1}\ensuremath{-}{\ensuremath{\omega}}_{2}$, the gain at the mth sideband decreases as ${({\ensuremath{\omega}}_{1}\ensuremath{-}{\ensuremath{\omega}}_{2})}^{\ensuremath{-}m}$.
POPULATION RATE EQUATIONS From the discussion in the preceding chapter, it is clear that population inversion is the basic condition for an optical gain. For any system in its normal state in thermal equilibrium, a low-energy level is always more populated than a high-energy level, hence there is no population inversion. Population inversion in a system can only be accomplished through a process called pumping by actively exciting the atoms in a low-energy level to a high-energy level. If left alone, the atoms in a system relax to thermal equilibrium. Therefore, population inversion is a nonequilibrium state that cannot be sustained without active pumping. To keep a constant optical gain, continuous pumping is required to maintain population inversion. This condition is clearly consistent with the law of conservation of energy: amplification of an optical wave leads to an increase in optical energy, which is possible only if the required energy is supplied by a source. Pumping is the process that supplies energy to the gain medium for the amplification of an optical wave. There are many different pumping techniques, including optical excitation, electric current injection, electric discharge, chemical reaction, and excitation with particle beams. The use of a specific pumping technique depends on the properties of the gain medium being pumped. The lasers and optical amplifiers of particular interest in photonic systems are made of either dielectric solid-state media doped with active ions, such as Nd:YAG and Er:glass fiber, or direct-gap semiconductors, such as GaAs and InP. For a dielectric gain medium, the most commonly used pumping technique is optical pumping using either an incoherent light source, such as a flashlamp or a light-emitting diode, or a coherent light source from another laser. A semiconductor gain medium can also be optically pumped, but it is usually pumped by electric current injection. In this section, we consider the general conditions for pumping to achieve population inversion. Detailed pumping mechanisms and physical setups are not addressed here because they depend on the specific gain medium used in a particular application. The net rate of increase of the population density in a given energy level is described by a rate equation. As we shall see below, pumping for population inversion in any practical gain medium always requires the participation of more than two energy levels.
In Chapter 1, we introduced the standard rate equations (SRE) for a laser containing two-level atoms between which stimulated emission is possible. But real lasers exhibit much more complicated energy level schemes. Throughout this chapter, we consider several models in which the light–matter interaction is described by population equations for all the levels involved in the laser operation. Although they are mathematically more complicated, we shall investigate these equations in the same way as in Chapter 1, i.e. by formulating dimensionless equations and by analyzing the stability properties of the steady states. The basic ingredients of the SRE model used up to here, namely pumping and relaxation processes, play key roles in the efficiency of lasers. But already during the pioneering days of the laser, it appeared important to investigate three- and four-level models in order to obtain more reliable information on quantities such as the power conversion efficiency or the response time. The common extensions of the two-level SRE typically consider an open two-level system, or three- or four-level systems, depending on the nature of the active medium. Restriction to as few as four levels is again a crude simplification of the complex population dynamics occurring in most lasers. But it is rather surprising to see how good these simple kinetic models are. As we demonstrate by studying specific examples, the solution of the three- or four-level rate equations differs only slightly from the solution of the SRE.
Using semiclassical radiation theory, a formalism similar to that used by Lamb in his Theory of an Optical Maser is developed for studying the amplification of vector traveling waves in a laser-type medium. The effect of the medium on the waves is given in terms of space (or time) dependent field amplitudes and phases and a nonlinear index of refraction. With particular emphasis on typical gaseous media, the effects of Doppler broadening are treated in detail for arbitrary ratios of natural to Doppler linewidths. Polarization and propagation vectors in various directions are considered, and the nonlinear effects are found to make an isotropic medium effectively anisotropic.
Lowest order nonlinear effects (due to a polarization cubic in the field amplitudes) are studied extensively, and the frequency dependence of several of these processes is presented in graphical form. In particular, the introduction of fields at new frequencies and polarization effects are considered. The characteristics of these nonlinear processes peculiar to Doppler broadened lines are discussed, and the processes are interpreted in terms of saturation and coherent modulation of the population inversion density.
Strong nonlinear effects are considered in a more approximate way and are found to consist of saturation of the various linear and nonlinear processes previously considered. These strong nonlinear effects should occur at low enough intensities to be easily observed in practice on a CW basis. With the present formalism, the analytical results of Gordon, White and Rigden regarding gain saturation in laser amplifiers are obtained, and the extension is made to include frequencies away from line center and the effects of multiple spectral components. Again, the introduction of fields at new frequencies is considered in detail. These results are also discussed in terms of saturation and coherent modulation of the populations and hole burning.
Introduction When an electromagnetic wave propagates through amedium stimulated emissions increase the intensity of the wave, while absorptions diminish it. The overall intensity will increase if the number of stimulated emissions can be made larger than the number of absorptions. If we can create such a situation then we have built an amplifier that operates through the mechanism of stimulated emission. This laser amplifier , in common with electronic amplifiers, has useful gain only over a particular frequency bandwidth. Its operating frequency range will be determined by the lineshape of the transition, and we expect the frequency width of its useful operating range to be of the same order as the width of the lineshape. It is very important to consider how this frequencywidth is related to the various mechanisms by which transitions between different energy states of a particle are smeared out over a range of frequencies. This line broadening affects in a fundamental way not only the frequency bandwidth of the amplifier, but also its gain. A laser amplifier can be turned into an oscillator by supplying an appropriate amount of positive feedback. The level of oscillation will stabilize because the amplifier saturates. Laser amplifiers fall into two categories, which saturate in different ways. A homogeneously broadened amplifier consists of a number of amplifying particles that are essentially equivalent, whereas an inhomogeneously broadened amplifier contains amplifying particles with a distribution of amplification characteristics. Homogeneous line broadening All energy states, except the lowest energy state of a particle (the ground state) cover a range of possible energies.