Introduction We were able to show in Chapter 3 that a medium in which we can obtain a population inversion (i.e. a situation in which the population density in the excited state is greater than that in the fundamental level) allows for optical gain of an electromagnetic wave having a frequency near to the resonant frequency of the system. By introducing feedback of the amplified signal into the medium, the system can be made to oscillate naturally, resulting in laser oscillations . To obtain this population inversion, we must introduce at least a third (and perhaps even a fourth) energy level into the system. (We saw how a two-level system under the influence of an intense pump beam will saturate with no resulting population inversion.) The aim then of this chapter is to introduce the concepts necessary to extend our two-level system into a working model capable of illustrating the phenomenon of laser oscillation. We will not spend too much time discussing atomic transition lasers as they do not figure readily in our treatment of quantum electronic properties of semiconductors. An exception will be made, however; we brush upon the particular topics of a diode pumped laser in Complement 4.E and a quantum cascade laser in Complement 13.H. Population inversion and optical amplification Population inversion We will show how population inversion can be achieved by carrier transfer from higher lying levels to the upper level of a two-level subsystem of interest.
Introduction We were able to show in Chapter 3 that a medium in which we can obtain a population inversion (i.e. a situation in which the population density in the excited state is greater than that in the fundamental level) allows for optical gain of an electromagnetic wave having a frequency near to the resonant frequency of the system. By introducing feedback of the amplified signal into the medium, the system can be made to oscillate naturally, resulting in laser oscillations . To obtain this population inversion, we must introduce at least a third (and perhaps even a fourth) energy level into the system. (We saw how a two-level system under the influence of an intense pump beam will saturate with no resulting population inversion.) The aim then of this chapter is to introduce the concepts necessary to extend our two-level system into a working model capable of illustrating the phenomenon of laser oscillation. We will not spend too much time discussing atomic transition lasers as they do not figure readily in our treatment of quantum electronic properties of semiconductors. An exception will be made, however; we brush upon the particular topics of a diode pumped laser in Complement 4.E and a quantum cascade laser in Complement 13.H. Population inversion and optical amplification Population inversion We will show how population inversion can be achieved by carrier transfer from higher lying levels to the upper level of a two-level subsystem of interest.
POPULATION RATE EQUATIONS From the discussion in the preceding chapter, it is clear that population inversion is the basic condition for an optical gain. For any system in its normal state in thermal equilibrium, a low-energy level is always more populated than a high-energy level, hence there is no population inversion. Population inversion in a system can only be accomplished through a process called pumping by actively exciting the atoms in a low-energy level to a high-energy level. If left alone, the atoms in a system relax to thermal equilibrium. Therefore, population inversion is a nonequilibrium state that cannot be sustained without active pumping. To keep a constant optical gain, continuous pumping is required to maintain population inversion. This condition is clearly consistent with the law of conservation of energy: amplification of an optical wave leads to an increase in optical energy, which is possible only if the required energy is supplied by a source. Pumping is the process that supplies energy to the gain medium for the amplification of an optical wave. There are many different pumping techniques, including optical excitation, electric current injection, electric discharge, chemical reaction, and excitation with particle beams. The use of a specific pumping technique depends on the properties of the gain medium being pumped. The lasers and optical amplifiers of particular interest in photonic systems are made of either dielectric solid-state media doped with active ions, such as Nd:YAG and Er:glass fiber, or direct-gap semiconductors, such as GaAs and InP. For a dielectric gain medium, the most commonly used pumping technique is optical pumping using either an incoherent light source, such as a flashlamp or a light-emitting diode, or a coherent light source from another laser. A semiconductor gain medium can also be optically pumped, but it is usually pumped by electric current injection. In this section, we consider the general conditions for pumping to achieve population inversion. Detailed pumping mechanisms and physical setups are not addressed here because they depend on the specific gain medium used in a particular application. The net rate of increase of the population density in a given energy level is described by a rate equation. As we shall see below, pumping for population inversion in any practical gain medium always requires the participation of more than two energy levels.
When an atomic system interacts with light, it can amplify the electromagnetic radiation when gain exceeds loss. This requires that transitions from the upper level to the lower level prevail over the transitions from the lower level to the upper level. If one deals with a two-level system, the only way to obtain amplification is to create a state of population inversion, i.e. the upper level must be more densely populated that the lower level. "Lasing without inversion" may be possible when part of the atoms are trapped, which removes them from the subspace of states with which the upper level can have transitions. This chapter determines to what extent population inversion is necessary to achieve amplification. Independently, amplification without inversion and lasing without inversion were predicted by Harris using a different type of atomic interference. The amplification threshold has a number of features that are reminiscent of the laser threshold.
This chapter begins with a heuristic derivation of atomic population rate equations which include changes to level populations due to stimulated transitions as well as level relaxations and pump. These equations are used to study the saturation of population inversion with increasing light intensity and its dependence on the type of gain medium (three-level gain media vs. four-level gain media), lineshape and nature of line broadening (homogeneous vs inhomogeneous broadening). How saturation affects lineshape and thus gain and absorption giving rise to phenomena like power broadening and spectral hole burning is also discussed. The chapter summarizes the equations of motion for atomic polarization, inversion and the cavity field describing their nonlinear dynamical coupling. These equations, known as the Maxwell-Bloch equations, provide a complete description of atom-field interaction in a laser. Approximations of these equations, including the rate equation approximation, to deal with different laser classes are briefly described. These will be used in the next few chapters to explore and understand the rich and varied behavior of lasers. The chapter ends with a summary of select gain media for different types of commonly used lasers.
Introduction When an electromagnetic wave propagates through amedium stimulated emissions increase the intensity of the wave, while absorptions diminish it. The overall intensity will increase if the number of stimulated emissions can be made larger than the number of absorptions. If we can create such a situation then we have built an amplifier that operates through the mechanism of stimulated emission. This laser amplifier , in common with electronic amplifiers, has useful gain only over a particular frequency bandwidth. Its operating frequency range will be determined by the lineshape of the transition, and we expect the frequency width of its useful operating range to be of the same order as the width of the lineshape. It is very important to consider how this frequencywidth is related to the various mechanisms by which transitions between different energy states of a particle are smeared out over a range of frequencies. This line broadening affects in a fundamental way not only the frequency bandwidth of the amplifier, but also its gain. A laser amplifier can be turned into an oscillator by supplying an appropriate amount of positive feedback. The level of oscillation will stabilize because the amplifier saturates. Laser amplifiers fall into two categories, which saturate in different ways. A homogeneously broadened amplifier consists of a number of amplifying particles that are essentially equivalent, whereas an inhomogeneously broadened amplifier contains amplifying particles with a distribution of amplification characteristics. Homogeneous line broadening All energy states, except the lowest energy state of a particle (the ground state) cover a range of possible energies.
A three-level system which radiates at both intermediate transition frequencies is considered to be coherently pumped at a frequency near the two-photon resonance frequency. A sharply resonant rise in the second- and third-level population is found for slight detuning of the pump from two-photon resonance. Population inversion in either transition is shown to be possible, depending on the pertinent parameters. This effect furnishes a novel method of population inversion at a frequency higher than the pump frequency. Keywords include: Laser, Laser-type devices, Coherent pumping, Three-level systems, and Quantum electronics.
Considerable attention has been directed recently to the study of lasing without the need of population inversion. The optical coherence and quantum interference associated with the light amplification may lead to interesting statistical properties in inversionless lasers. Here we analyze a laser model that consists of an ensemble of closed multi-level (three or four levels) atoms driven by a single coherent field. Unlike conventional lasers where population inversion is maintained and kept at the threshold value for arbitrary laser output, the multi-level laser analyzed here can start lasing from population inversion and evolves from population inversion into non-inversion with the increasing atomic pumping. In other words, the system makes transition from light amplification by population inversion into light amplification by coherence. On the other hand, the system can be also made to start lasing without population inversion in any state basis. In both cases, initial inversion and non-inversion, which are controlled by the ratio of spontaneous decay rates, the laser well above threshold is always maintained by lasing without inversion (light amplification by coherence), and the laser intensity fluctuations may drop below the shot noise limit. Two factors contribute to the noise reduction: first, the disappearance of the population inversion leads to the depleted atomic population in the upper lasing state, which reduces the spontaneous emission noises; second, the fast coherent cycling of electrons between excited states leads to the highly regulated absorption and emission processes. We found that the combination of these two mechanisms can lead to the noise reduction in the laser output more than 50% below the shot-noise limit.