The photon is a quantum system that is by nature robust against noise, and fast travelling, providing an ideal information carrier for quantum information science. The field of quantum information science has generated a great deal of interest for both researchers and the public due to the advantages it can have over classical technologies in areas including communication, computing and cryptography. In this thesis, I explore several different ways that photons can be used to realize quantum information advantages and enable quantum technologies, information tasks and fundamental studies of physics. A strong emphasis is placed on their practical implementation in optical experiments, where the challenges of noise, loss and device imperfections must be considered and combated. I utilize spontaneous parametric downconversion-based sources of high-quality single photons, and their polarization, path, and temporal degrees of freedom for encoding quantum information. In my first experimental project, I demonstrate the first violation of noncontextuality with time-polarization intraparticle entangled states encoded in a single photon by implementing a powerful interference-based measurement technique for photonic states. I perform a test of noncontextuality, acquiring a parameter |SCHSH| = 2.744 ± 0.006, which violates the classical bound of 2 by over 110 standard deviations, rigorously certifying both entanglement and contextuality of the system. We propose a new approach for preparing and measuring high-dimensional time-bin states, that overcomes many of the limitations of previous techniques, and demonstrate it for time-bin qubits and qutrits. In the next experimental project, I investigate the topic of universal cloning in quantum steering-with cloning and steering being two fundamental aspects of quantum physics deeply involved in the security of quantum protocols. I report the first experimental demonstration of cloned quantum steering, showing a simultaneous violation in a steering test by two clones made from one part of an entangled pair of photons. This provides a conclusive result on the question of whether the cloning of quantum steering is possible. We also present theoretical results that clarify our understanding of cloned steering for qubits: we find a no-go theorem where quantum steering can only be copied by a qubit universal cloning machine for 2 and 3 clones, and a monogamy relation where for N clones, steering is only possible if a minimum of N + 1 measurements are performed on each clone. I discuss the field of random number generation, and study how quantum physics allows for certifiably unpredictable random sequences, without needing complete trust in all of the physical devices, offering high levels of security over classical approaches. I report the first discrete-variable detection-loophole-free implementation of one-sided device-independent randomness expansion of certified random bits, based on the quantum steering task. These results illustrate an approach to secure randomness with greater tolerance to noise and loss compared to Bell test-based protocols. The final experimental project looks at quantum autoencoders, which are a quantum machine learning tool that we investigate for the purpose of denoising quantum states. I model and simulate a denoising quantum autoencoder which compresses ququarts into a qubit space and reconstructs noise-reduced ququart states. I construct an experimental apparatus that implements this device, and demonstrate quantum state tomography of ququart states, and the training of the autoencoder.
The photon is a quantum system that is by nature robust against noise, and fast travelling, providing an ideal information carrier for quantum information science. The field of quantum information science has generated a great deal of interest for both researchers and the public due to the advantages it can have over classical technologies in areas including communication, computing and cryptography. In this thesis, I explore several different ways that photons can be used to realize quantum information advantages and enable quantum technologies, information tasks and fundamental studies of physics. A strong emphasis is placed on their practical implementation in optical experiments, where the challenges of noise, loss and device imperfections must be considered and combated. I utilize spontaneous parametric downconversion-based sources of high-quality single photons, and their polarization, path, and temporal degrees of freedom for encoding quantum information. In my first experimental project, I demonstrate the first violation of noncontextuality with time-polarization intraparticle entangled states encoded in a single photon by implementing a powerful interference-based measurement technique for photonic states. I perform a test of noncontextuality, acquiring a parameter |SCHSH| = 2.744 ± 0.006, which violates the classical bound of 2 by over 110 standard deviations, rigorously certifying both entanglement and contextuality of the system. We propose a new approach for preparing and measuring high-dimensional time-bin states, that overcomes many of the limitations of previous techniques, and demonstrate it for time-bin qubits and qutrits. In the next experimental project, I investigate the topic of universal cloning in quantum steering-with cloning and steering being two fundamental aspects of quantum physics deeply involved in the security of quantum protocols. I report the first experimental demonstration of cloned quantum steering, showing a simultaneous violation in a steering test by two clones made from one part of an entangled pair of photons. This provides a conclusive result on the question of whether the cloning of quantum steering is possible. We also present theoretical results that clarify our understanding of cloned steering for qubits: we find a no-go theorem where quantum steering can only be copied by a qubit universal cloning machine for 2 and 3 clones, and a monogamy relation where for N clones, steering is only possible if a minimum of N + 1 measurements are performed on each clone. I discuss the field of random number generation, and study how quantum physics allows for certifiably unpredictable random sequences, without needing complete trust in all of the physical devices, offering high levels of security over classical approaches. I report the first discrete-variable detection-loophole-free implementation of one-sided device-independent randomness expansion of certified random bits, based on the quantum steering task. These results illustrate an approach to secure randomness with greater tolerance to noise and loss compared to Bell test-based protocols. The final experimental project looks at quantum autoencoders, which are a quantum machine learning tool that we investigate for the purpose of denoising quantum states. I model and simulate a denoising quantum autoencoder which compresses ququarts into a qubit space and reconstructs noise-reduced ququart states. I construct an experimental apparatus that implements this device, and demonstrate quantum state tomography of ququart states, and the training of the autoencoder.
Since its inception, quantum information processing (QIP) has been branched into many new directions. As well as well-known applications such as teleportation and metrology, researchers are beginning to investigate interdisciplinary areas such as quantum machine learning. One of the interesting areas is where quantum information science meets stochastic modelling, from the field of complexity science. Recently, it has been shown theoretically that, for simulating classical systems, quantumassisted models and simulators are more efficient in terms of memory storage they require to do simulations, compared with classical computers. That is, for most systems, classical simulators demand an excessive amount of memory storage, while quantum simulators can do the same simulation with less memory. The main focus of this thesis is on experimental realisation of quantum simulators that are capable of simulating stochastic processes with a reduced amount of memory. To implement the (nearly) exact simulation of stochastic processes using quantum simulators, it is essential to have low-noise state preparation, robust unitary operations, and high-precision read-out. These requirements, and the flexibility and precision of photonic quantum optics, make photonics the ideal system for developing the science of this new quantum advantage and for making strides towards its technological realisation. In the context of stochastic simulation, I have experimentally studied three key problems that serve as stepping stones in advancing this new field. In the first experiment, an error-tolerant quantum simulator was designed, and realised to simulate a 1D Ising spin chain, using internal states that store less information than the corresponding classical approach. Furthermore, an interesting and fundamental phenomenon named the ambiguity of simplicity is witnessed. This is the inconsistency that we observe in the order of relative complexity of two systems when we change the simulators from classical to quantum. In the second experiment, a quantum simulator was built that can simulate classical processes for more than one step of the simulation at a time, storing the information from multiple steps coherently. In the third experiment, a new type of quantum memory advantage, which is based on the dimensionality of the memory register, rather than on information entropy measure, is demonstrated. This advantage is realisable in a single simulator, in contrast to previous works. Realising the dimensionality memory advantage in practical applications does not rely on running multiple simulators in parallel.In the field of optical QIP, realising an ideal single-photon source has been a longstanding challenge. In another part of my PhD, I have worked on a source that aims to tackle some of the existing issues in this context. We built a source of high-quality entangled photons with a high heralding efficiency, which has the potential to be used in multi-photon experiments. This source was also essential to demonstrate a fundamental task in quantum non-locality, one-way steering, which was performed conclusively for the first time.
Quantum communication attempts to harness the unique rules of quantum mechanics to perform communication tasks that are difficult or impossible using classical rules. To realize these benefits, information must be carried on quantum systems. Photons make excellent carriers because they interact very little with the environment, move quickly, and can naturally store quantum information in their polarization. However, it is notoriously difficult to detect a single photon without destroying it. Standard detectors simply absorb the photon, losing the quantum information. This is a critical outstanding problem in quantum communication, as advanced protocols need to know exactly when a photon has arrived at a receiver after transmission through the atmosphere or an optical fibre before performing further quantum-information-processing tasks. Certifying a photon’s presence is of particular interest in tests of Bell’s inequalities, which have only recently been performed without loopholes arising from photon loss, and in device-independent quantum cryptography, which relies on such Bell tests for security. \n \nIn this thesis, I first present work on directly reducing losses in a successful loophole-free Bell test. This is an extremely difficult task that cannot be extended for long-distance communication. Therefore I then focus on ways to circumvent loss by detecting photons without destroying them while preserving their quantum information. First I analyze theoretically a way to herald photons using only linear-optical elements (beam splitters and phase shifters) and extra ancilla photons. Similar but older methods have been demonstrated experimentally by other groups, and my improvements will help future advanced quantum communication protocols. \n \nThe main experiment in this thesis certifies the presence of a photon in a rather simple way: split the photon into two using a nonlinear optical crystal, then detect one of the pair to herald the other. I show in this first proof-of-principle experiment that photonic qubit precertification indeed preserves qubit states, with up to (92.3 ± 0.6)% fidelity and rates of 1100 events per hour. With reductions in detector dark counts, precertification could outperform direct transmission, even with extremely lossy fibre links. \n \nFinally, I present two sources of photons based on nonlinearities in optical fibres. One of the limitations of the photon splitting scheme for heralding is the low success probability due to the very low likelihood of splitting a photon in two. In these fibre photon sources I investigate increasing the splitting likelihood in four-wave mixing through advanced materials and fibre designs. I use polarization-maintaining fibres to generate entangled photon pairs as a prerequisite to precertification, with (92.2 ± 0.2)% fidelity to a maximally-entangled state. Then I show that one type of highly nonlinear chalcogenide glass, never before used for photon pair generation, could outperform standard nonlinear crystals by two orders of magnitude, with calculated conversion efficiency up to 10^-3. To approach the single photon regime, I generate photon pairs in chalcogenide microwires with pump powers as low as 480 nW and verify their timing correlations. \n \nThese advances demonstrate the capability of nondestructive precertification of photons to allow advanced quantum communications protocols even over long distance, and could lead to the first implementations of fully device-independent quantum cryptography.
We are currently witnessing a fundamental change in the field of quantum information, whereby protocols and experiments previously performed in university labs are now being implemented in real-world scenarios, and a strong commercial push for new and reliable applications is contributing significantly in advancing fundamental research. In this thesis and related included papers, I first look at a keystone of quantum science, Bell's theorem. In particular, I will expose an issue that we call apparent signalling, which affects many current and past experiments relying on Bell tests. A statistical test of the impact of apparent signalling is described, together with experimental approaches to successfully mitigate it. Next, I consider one of the most refined ideas that recently emerged in quantum information, device-independent certification. Device-independent quantum information aims at answering the question: "Assuming we trust quantum mechanics, what can we conclude about the quantum systems or the measurement operators in a given experiment, based solely on its results, while making minimal assumptions on the physical devices used?". In my work, the problem was successfully approached in two different scenarios, one based on entangled photons and the other on prepare-and-measure experiments with single photons, with the aim of certifying informationally-complete quantum measurements. Finally, I conclude by presenting an elegant and promising approach to the experimental generation of multi-photon entanglement, which is a fundamental prerequisite in most modern quantum information protocols.
This thesis examines the integration of two disparate technologies in order to perform experiments in single photon quantum optics with low loss. Many technologies and experiments in quantum optics, communication, or computing require a certain fraction of the photons involved to be received at the end of the experiment, and in many cases the required efficiency has not yet been reached. This includes the famous Einstein, Podolsky, and Rosen gedanken-experiment, now implemented in the laboratory, demonstrating the existence of entanglement to unconvinced observers. Also included is the nonlocality test of John Bell, as well as technological problems such as device-independent quantum key distribution. In this thesis I perform these experiments in the high-efficiency regime. This programme requires the integration of two lines of research: improving sources of single photons, and improving detectors thereof. Until recently detector research was focussed on development, with improvements being sought for their own sake, working towards the ultimate goal of perfect photon detection. Recent years have seen these devices move into quantum photonics laboratories, allowing for previously impossible experiments to be undertaken. In this thesis, I combine high-efficiency, number-resolving, detectors with a high-efficiency entangled photon pair source, based on another line of research going back decades: the use of spontaneous parametric down-conversion to create single-photon-like modes of light, and the entanglement of the output modes in a useful way. For small demonstrations, such as the experiments mentioned above, this can emulate a single photon with enough fidelity, and low enough loss, to successfully perform the procedure. Here I push both of these technologies, and the problems of combining them, as far as I can, and solve the problems inherent with any marriage of disparate devices. I also examine the relative performance of two different steering inequalities, one linear and one quadratic, in the presence of noise, analysing my experimental data with each of them. I perform a detection- loophole free demonstration of EPR steering, violating the local bound by 200s, setting a then world record for efficiency at 62.5%.
Quantum information science explores the foundational aspects of quantum mechanics and its ombination with information science for new information technologies. The underlying key resource is non-classical correlations. These counter-intuitive correlations between quantum systems can be used for encoding, transmitting and measuring information in quantum information tasks. Although quantum properties can be used in a variety of systems, here we explore photons. These information carriers are fast, easy to generate and manipulate and only interact weakly with the environment. These properties make them to excellent candidates to be employed in experiments. Developing quantum technology, such as single photon sources and single photon detectors, allows us to investigate the foundational aspects of quantum mechanics in quantum information tasks. These tasks use non-classical correlations, which form a hierarchy, from Bell nonlocality to Einstein-Podolsky-Rosen (EPR) steering to quantum nonseparability. Two systems are nonlocally correlated, when measuring one system affects the measurement results on the other system, hence the name `steering. In test for non-classical correlations, we share a quantum state between two observers which are trusted or untrusted. While observers are both untrusted or trusted in entanglement witness tests and Bell inequality violations, respectively, EPR-steering is distinct from these two classes by its fundamental asymmetry: one party is trusted while the other is untrusted.
Light beams offer many degrees of freedom to be explored in discrete and continuous domains. In addition to the possibility of entangling photons in these many degrees of freedom, it makes light a very useful and versatile tool for quantum information and quantum foundation purposes. In this thesis, we endorse its importance and versatility by presenting novel contributions that further explore both discrete and continuous degrees of freedom. It begins with two experiments that use classical light and explore its analogous behavior to quantum systems. The first one is a classical optics simulation of the dynamics of a relativistic quantum particle. The second work is related to the theory of mutually unbiased measurements that are effectively discrete but constructed from continuous variables systems. In the second part of the thesis, three works are presented that use the polarization and path discrete degrees of freedom. The first one is a redefinition of the quantum nonlocal correlation called steering in the multipartite scenario, based on an inconsistency in the previous definition, namely the creation of this correlation from scratch using operations that supposedly would not be able to do so. We call this exposure of quantum steering. Steering exposure is observed with entangled photons. The other two works are related to the experimental implementation of quantum channels of qubits, one of them is a particular channel for which we test for non-Markovianity using a operational measure called conditional past-future (CPF) correlation. The thesis finishes with a proposal for an experimental realization of any quantum channel of a single qubit, where the qubit is realized by the polarization of single photons. The functioning of all optical devices used is didactically explained.