Quantum communication attempts to harness the unique rules of quantum mechanics to perform communication tasks that are difficult or impossible using classical rules. To realize these benefits, information must be carried on quantum systems. Photons make excellent carriers because they interact very little with the environment, move quickly, and can naturally store quantum information in their polarization. However, it is notoriously difficult to detect a single photon without destroying it. Standard detectors simply absorb the photon, losing the quantum information. This is a critical outstanding problem in quantum communication, as advanced protocols need to know exactly when a photon has arrived at a receiver after transmission through the atmosphere or an optical fibre before performing further quantum-information-processing tasks. Certifying a photon’s presence is of particular interest in tests of Bell’s inequalities, which have only recently been performed without loopholes arising from photon loss, and in device-independent quantum cryptography, which relies on such Bell tests for security. \n \nIn this thesis, I first present work on directly reducing losses in a successful loophole-free Bell test. This is an extremely difficult task that cannot be extended for long-distance communication. Therefore I then focus on ways to circumvent loss by detecting photons without destroying them while preserving their quantum information. First I analyze theoretically a way to herald photons using only linear-optical elements (beam splitters and phase shifters) and extra ancilla photons. Similar but older methods have been demonstrated experimentally by other groups, and my improvements will help future advanced quantum communication protocols. \n \nThe main experiment in this thesis certifies the presence of a photon in a rather simple way: split the photon into two using a nonlinear optical crystal, then detect one of the pair to herald the other. I show in this first proof-of-principle experiment that photonic qubit precertification indeed preserves qubit states, with up to (92.3 ± 0.6)% fidelity and rates of 1100 events per hour. With reductions in detector dark counts, precertification could outperform direct transmission, even with extremely lossy fibre links. \n \nFinally, I present two sources of photons based on nonlinearities in optical fibres. One of the limitations of the photon splitting scheme for heralding is the low success probability due to the very low likelihood of splitting a photon in two. In these fibre photon sources I investigate increasing the splitting likelihood in four-wave mixing through advanced materials and fibre designs. I use polarization-maintaining fibres to generate entangled photon pairs as a prerequisite to precertification, with (92.2 ± 0.2)% fidelity to a maximally-entangled state. Then I show that one type of highly nonlinear chalcogenide glass, never before used for photon pair generation, could outperform standard nonlinear crystals by two orders of magnitude, with calculated conversion efficiency up to 10^-3. To approach the single photon regime, I generate photon pairs in chalcogenide microwires with pump powers as low as 480 nW and verify their timing correlations. \n \nThese advances demonstrate the capability of nondestructive precertification of photons to allow advanced quantum communications protocols even over long distance, and could lead to the first implementations of fully device-independent quantum cryptography.
Quantum communication attempts to harness the unique rules of quantum mechanics to perform communication tasks that are difficult or impossible using classical rules. To realize these benefits, information must be carried on quantum systems. Photons make excellent carriers because they interact very little with the environment, move quickly, and can naturally store quantum information in their polarization. However, it is notoriously difficult to detect a single photon without destroying it. Standard detectors simply absorb the photon, losing the quantum information. This is a critical outstanding problem in quantum communication, as advanced protocols need to know exactly when a photon has arrived at a receiver after transmission through the atmosphere or an optical fibre before performing further quantum-information-processing tasks. Certifying a photon’s presence is of particular interest in tests of Bell’s inequalities, which have only recently been performed without loopholes arising from photon loss, and in device-independent quantum cryptography, which relies on such Bell tests for security. \n \nIn this thesis, I first present work on directly reducing losses in a successful loophole-free Bell test. This is an extremely difficult task that cannot be extended for long-distance communication. Therefore I then focus on ways to circumvent loss by detecting photons without destroying them while preserving their quantum information. First I analyze theoretically a way to herald photons using only linear-optical elements (beam splitters and phase shifters) and extra ancilla photons. Similar but older methods have been demonstrated experimentally by other groups, and my improvements will help future advanced quantum communication protocols. \n \nThe main experiment in this thesis certifies the presence of a photon in a rather simple way: split the photon into two using a nonlinear optical crystal, then detect one of the pair to herald the other. I show in this first proof-of-principle experiment that photonic qubit precertification indeed preserves qubit states, with up to (92.3 ± 0.6)% fidelity and rates of 1100 events per hour. With reductions in detector dark counts, precertification could outperform direct transmission, even with extremely lossy fibre links. \n \nFinally, I present two sources of photons based on nonlinearities in optical fibres. One of the limitations of the photon splitting scheme for heralding is the low success probability due to the very low likelihood of splitting a photon in two. In these fibre photon sources I investigate increasing the splitting likelihood in four-wave mixing through advanced materials and fibre designs. I use polarization-maintaining fibres to generate entangled photon pairs as a prerequisite to precertification, with (92.2 ± 0.2)% fidelity to a maximally-entangled state. Then I show that one type of highly nonlinear chalcogenide glass, never before used for photon pair generation, could outperform standard nonlinear crystals by two orders of magnitude, with calculated conversion efficiency up to 10^-3. To approach the single photon regime, I generate photon pairs in chalcogenide microwires with pump powers as low as 480 nW and verify their timing correlations. \n \nThese advances demonstrate the capability of nondestructive precertification of photons to allow advanced quantum communications protocols even over long distance, and could lead to the first implementations of fully device-independent quantum cryptography.
Abstract One of the biggest challenges in experimental quantum information is to sustain the fragile superposition state of a qubit1. Long lifetimes can be achieved for material qubit carriers as memories2, at least in principle, but not for propagating photons that are rapidly lost by absorption, diffraction or scattering3. The loss problem can be mitigated with a nondestructive photonic qubit detector that heralds the photon without destroying the encoded qubit. Such a detector is envisioned to facilitate protocols in which distributed tasks depend on the successful dissemination of photonic qubits4, 5, improve loss-sensitive qubit measurements6, 7 and enable certain quantum key distribution attacks8. Here we demonstrate such a detector based on a single atom in two crossed fibre-based optical resonators, one for qubit-insensitive atom–photon coupling and the other for atomic-state detection9. We achieve a nondestructive detection efficiency upon qubit survival of 79 ± 3 per cent and a photon survival probability of 31 ± 1 per cent, and we preserve the qubit information with a fidelity of 96.2 ± 0.3 per cent. To illustrate the potential of our detector, we show that it can, with the current parameters, improve the rate and fidelity of long-distance entanglement and quantum state distribution compared to previous methods, provide resource optimization via qubit amplification and enable detection-loophole-free Bell tests.
For any communication, the conveyed information must be carried by some physical system. If this system is a quantum system rather than a classical one, its behavior will be governed by the laws of quantum mechanics. Hence, the properties of quantum mechanics, such as superpositions and entanglement, are accessible, opening up new possibilities for transferring information. The exploration of these possibilities constitutes the field of quantum communication. The key ingredient in quantum communication is the qubit, a bit that can be in any superposition of 0 and 1, and that is carried by a quantum state. One possible physical realization of these quantum states is to use single photons. Hence, to explore the possibilities of optical quantum communication, photonic quantum states must be generated, transmitted, characterized, and detected with high precision. This thesis begins with the first of these steps: the implementation of single-photon sources generating photonic qubits. The sources are based on photon-pair generation in nonlinear crystals, and designed to be compatible with fiber optical communication systems. To ensure such a compatibility and to create a high-quality source, a theoretical analysis is made, optimizing the coupling of the photons into optical fibers. Based on the theoretical analysis, a heralded single-photon source and a two-crystal source of entangled photons-pairs are experimentally implemented. The source of entangled photons is further developed into a compact source with a narrow bandwidth compatible with standard telecommunication wavelength-division multiplexers, and even further developed to a more stable one-crystal source. The sources are to be used for quantum communication in general and quantum cryptography in particular. Specifically, a heralded single-photon source is implemented and then used for a full test of a decoy-state quantum cryptography protocol.
Entangled photons are at the heart of experimental quantum physics. They were used for the first fundamental tests of quantum theory, and became a basic building block for many novel quantum protocols, such as quantum cryptography, dense coding or teleportation. Therefore, the efficient generation of entangled photons, as well as their distribution and accurate analysis are of paramount importance, particularly with regard to the practicability of many applications of quantum communication. This thesis deals largely with the problem of efficient generation of photonic entanglement with the principal aim of developing a bright source of polarization-entangled photon pairs, which meets the requirements for reliable and economic operation of quantum communication prototypes and demonstrators. Our approach uses a correlated photon-pair emission in nonlinear process of spontaneous parametric down-conversion pumped by light coming from a compact and cheap blue laser diode. Two alternative source configurations are examined within the thesis. The first makes use of a well established concept of degenerate non-collinear emission from a single type-II nonlinear crystal and the second relies on a novel method where the emissions from two adjacent type-I phase-matched nonlinear crystals operated in collinear non-degenerate regime are coherently overlapped. The latter approach showed to be more effective, yielding a total detected rate of almost 10^6 pairs/s at >98 % quantum interference visibility of polarization correlations. This performance, together with the almost free of alignment operation of the system, suggest that it is an especially promising candidate for many future practical applications, including quantum cryptography, detector calibration or use in undergraduate lab courses. The second issue addressed within the thesis is the simplification and practical implementation of quantum-assisted solutions to multiparty communication tasks. While the recent rapid progress in the development of bright entangled photon-pair sources has been followed with ample experimental reports on two-party quantum communication tasks, the practical implementations of tasks for more than two parties have been held back, so far. This is mainly due to the requirement of multiparty entangled states, which are very difficult to be produced with current methods and moreover suffer from a high noise. We show that entanglement is not the only non-classical resource endowing the quantum multiparty information processing its power. Instead, only the sequential communication and transformation of a single qubit can be sufficient to accomplish certain tasks. This we prove for two distinct communication tasks, secret sharing and communication complexity. Whereas the goal of the first is to split a cryptographic key among several parties in a way that its reconstruction requires their collaboration, the latter aims at reducing the amount of communication during distributed computational tasks. Importantly, our qubit-assisted solutions to the problems are feasible with state-of-the-art technology. This we clearly demonstrate in the laboratory implementation for 6 and 5 parties, respectively, which is to the best of our knowledge the highest number of actively performing parties in a quantum protocol ever implemented. Thus, by successfully solving and implementing a cryptographic task as well as a task originating in computer science, we clearly illustrate the potential to introduce multiparty communication problems into real life.
This thesis examines the integration of two disparate technologies in order to perform experiments in single photon quantum optics with low loss. Many technologies and experiments in quantum optics, communication, or computing require a certain fraction of the photons involved to be received at the end of the experiment, and in many cases the required efficiency has not yet been reached. This includes the famous Einstein, Podolsky, and Rosen gedanken-experiment, now implemented in the laboratory, demonstrating the existence of entanglement to unconvinced observers. Also included is the nonlocality test of John Bell, as well as technological problems such as device-independent quantum key distribution. In this thesis I perform these experiments in the high-efficiency regime. This programme requires the integration of two lines of research: improving sources of single photons, and improving detectors thereof. Until recently detector research was focussed on development, with improvements being sought for their own sake, working towards the ultimate goal of perfect photon detection. Recent years have seen these devices move into quantum photonics laboratories, allowing for previously impossible experiments to be undertaken. In this thesis, I combine high-efficiency, number-resolving, detectors with a high-efficiency entangled photon pair source, based on another line of research going back decades: the use of spontaneous parametric down-conversion to create single-photon-like modes of light, and the entanglement of the output modes in a useful way. For small demonstrations, such as the experiments mentioned above, this can emulate a single photon with enough fidelity, and low enough loss, to successfully perform the procedure. Here I push both of these technologies, and the problems of combining them, as far as I can, and solve the problems inherent with any marriage of disparate devices. I also examine the relative performance of two different steering inequalities, one linear and one quadratic, in the presence of noise, analysing my experimental data with each of them. I perform a detection- loophole free demonstration of EPR steering, violating the local bound by 200s, setting a then world record for efficiency at 62.5%.
At the heart of quantum physics lies the principle of superposition, and at the heart of information theory lies the bit. Perhaps the most useful property of quantum systems is that they can be loaded with information bits, so-called qubits, that are indefinitely both 0 and 1 until a measurement is made. Another consequence is that several qubits can become entangled, which is manifested by the non-classical correlations between such quantum systems when measured in all possible bases. Within the rapidly progressing fields of quantum information and quantum communication these quantum effects are utilized to perform tasks such as quantum computing and quantum cryptography. In this thesis we present experimental and theoretical work using single photon sources to prepare ``flying'' photonic qubits. We describe work using mainly quasi-phase-matched nonlinear crystals to generate beams of entangled photon pairs, that are either encoded in polarization at near-visible wavelengths, or in time at optical fiber telecommunication wavelengths (1550 nm). The optical fiber is the medium used for transporting the qubits over a long distance, and it is therefore essential to couple the photons well into the fibers. By focusing the beams optimally, we have investigated how this problem can meet the requirement of creating photons of a narrow frequency bandwidth and a high photon flux. Furthermore, we have generated truly single photons that are heralded by an electrical signal. As a result of modifying the statistics of such sources we have been able to show the effect of photon antibunching. In two separate works, we have implemented a quantum key distribution system based on faint laser pulses at the telecom wavelength of 1550 nm, as well as protocols based on entanglement for performing authentication of key distribution in quantum cryptography.
We present two types of photon sources designed for secure quantum communication, e.g. for quantum cryptography. Both types are based on the creation of photon pairs by spontaneous parametric downconversion in nonlinear crystals. The first is a heralded single photon source and the second is a source of polarization-entangled photon pairs. For the heralded single photon source the detection of one of the photons of a downconversion pair is used as a trigger to announce the presence of the other: the single photon. The source is characterized by a highly sub-Poisson photon number statistics making it very suitable for use in quantum cryptography protocols using single photonic qubits to create correlated information between a sender and a receiver. The entanglement source instead uses the inherent non-classical correlations between entangled qubits. We also present a hybrid-encoding where the sender uses polarization to encode information while the receiver uses time-bins. Both sources create photons with highly non-degenerate wavelengths of 810 nm and 1550 nm, taking advantage of the efficient detectors at near-infrared and the low transmission loss of optical fibers at telecommunication wavelengths.