This thesis examines the integration of two disparate technologies in order to perform experiments in single photon quantum optics with low loss. Many technologies and experiments in quantum optics, communication, or computing require a certain fraction of the photons involved to be received at the end of the experiment, and in many cases the required efficiency has not yet been reached. This includes the famous Einstein, Podolsky, and Rosen gedanken-experiment, now implemented in the laboratory, demonstrating the existence of entanglement to unconvinced observers. Also included is the nonlocality test of John Bell, as well as technological problems such as device-independent quantum key distribution. In this thesis I perform these experiments in the high-efficiency regime. This programme requires the integration of two lines of research: improving sources of single photons, and improving detectors thereof. Until recently detector research was focussed on development, with improvements being sought for their own sake, working towards the ultimate goal of perfect photon detection. Recent years have seen these devices move into quantum photonics laboratories, allowing for previously impossible experiments to be undertaken. In this thesis, I combine high-efficiency, number-resolving, detectors with a high-efficiency entangled photon pair source, based on another line of research going back decades: the use of spontaneous parametric down-conversion to create single-photon-like modes of light, and the entanglement of the output modes in a useful way. For small demonstrations, such as the experiments mentioned above, this can emulate a single photon with enough fidelity, and low enough loss, to successfully perform the procedure. Here I push both of these technologies, and the problems of combining them, as far as I can, and solve the problems inherent with any marriage of disparate devices. I also examine the relative performance of two different steering inequalities, one linear and one quadratic, in the presence of noise, analysing my experimental data with each of them. I perform a detection- loophole free demonstration of EPR steering, violating the local bound by 200s, setting a then world record for efficiency at 62.5%.
This thesis examines the integration of two disparate technologies in order to perform experiments in single photon quantum optics with low loss. Many technologies and experiments in quantum optics, communication, or computing require a certain fraction of the photons involved to be received at the end of the experiment, and in many cases the required efficiency has not yet been reached. This includes the famous Einstein, Podolsky, and Rosen gedanken-experiment, now implemented in the laboratory, demonstrating the existence of entanglement to unconvinced observers. Also included is the nonlocality test of John Bell, as well as technological problems such as device-independent quantum key distribution. In this thesis I perform these experiments in the high-efficiency regime. This programme requires the integration of two lines of research: improving sources of single photons, and improving detectors thereof. Until recently detector research was focussed on development, with improvements being sought for their own sake, working towards the ultimate goal of perfect photon detection. Recent years have seen these devices move into quantum photonics laboratories, allowing for previously impossible experiments to be undertaken. In this thesis, I combine high-efficiency, number-resolving, detectors with a high-efficiency entangled photon pair source, based on another line of research going back decades: the use of spontaneous parametric down-conversion to create single-photon-like modes of light, and the entanglement of the output modes in a useful way. For small demonstrations, such as the experiments mentioned above, this can emulate a single photon with enough fidelity, and low enough loss, to successfully perform the procedure. Here I push both of these technologies, and the problems of combining them, as far as I can, and solve the problems inherent with any marriage of disparate devices. I also examine the relative performance of two different steering inequalities, one linear and one quadratic, in the presence of noise, analysing my experimental data with each of them. I perform a detection- loophole free demonstration of EPR steering, violating the local bound by 200s, setting a then world record for efficiency at 62.5%.
Entangled photons are at the heart of experimental quantum physics. They were used for the first fundamental tests of quantum theory, and became a basic building block for many novel quantum protocols, such as quantum cryptography, dense coding or teleportation. Therefore, the efficient generation of entangled photons, as well as their distribution and accurate analysis are of paramount importance, particularly with regard to the practicability of many applications of quantum communication. This thesis deals largely with the problem of efficient generation of photonic entanglement with the principal aim of developing a bright source of polarization-entangled photon pairs, which meets the requirements for reliable and economic operation of quantum communication prototypes and demonstrators. Our approach uses a correlated photon-pair emission in nonlinear process of spontaneous parametric down-conversion pumped by light coming from a compact and cheap blue laser diode. Two alternative source configurations are examined within the thesis. The first makes use of a well established concept of degenerate non-collinear emission from a single type-II nonlinear crystal and the second relies on a novel method where the emissions from two adjacent type-I phase-matched nonlinear crystals operated in collinear non-degenerate regime are coherently overlapped. The latter approach showed to be more effective, yielding a total detected rate of almost 10^6 pairs/s at >98 % quantum interference visibility of polarization correlations. This performance, together with the almost free of alignment operation of the system, suggest that it is an especially promising candidate for many future practical applications, including quantum cryptography, detector calibration or use in undergraduate lab courses. The second issue addressed within the thesis is the simplification and practical implementation of quantum-assisted solutions to multiparty communication tasks. While the recent rapid progress in the development of bright entangled photon-pair sources has been followed with ample experimental reports on two-party quantum communication tasks, the practical implementations of tasks for more than two parties have been held back, so far. This is mainly due to the requirement of multiparty entangled states, which are very difficult to be produced with current methods and moreover suffer from a high noise. We show that entanglement is not the only non-classical resource endowing the quantum multiparty information processing its power. Instead, only the sequential communication and transformation of a single qubit can be sufficient to accomplish certain tasks. This we prove for two distinct communication tasks, secret sharing and communication complexity. Whereas the goal of the first is to split a cryptographic key among several parties in a way that its reconstruction requires their collaboration, the latter aims at reducing the amount of communication during distributed computational tasks. Importantly, our qubit-assisted solutions to the problems are feasible with state-of-the-art technology. This we clearly demonstrate in the laboratory implementation for 6 and 5 parties, respectively, which is to the best of our knowledge the highest number of actively performing parties in a quantum protocol ever implemented. Thus, by successfully solving and implementing a cryptographic task as well as a task originating in computer science, we clearly illustrate the potential to introduce multiparty communication problems into real life.
The scope of this thesis is to explore different ways of bringing the phenomenon of quantum entanglement to our classical world. A first manner is to make entanglement an element of everyone's cultural background. I show that nontrivial quantum nonlocality tests can be performed with do-it-yourself optical sources. Furthermore, entanglement can be brought to the real world as a technological resource for improving everyday activities, like communication. Sources of entangled photons, suited to long distance quantum communication, need to be developed. I present a source of entangled photons realized via Spontaneous Parametric Down Conversion in an integrated cavity-waveguide. I show how this kind of sources can be engineered. I also report the realization of low-loss sources for the implementation of an experiment of faithful entanglement swapping adopting a nonlinear interaction between two single photons. Last, one can also attempt to physically generate and observe entanglement at macroscopic scales. I analyze the possibility of cloning a photon of an entangled pair and detecting the amplified state with human eyes. Bringing entanglement to scales one can see allows one to investigate ways of measuring light in the quantum-to-classical regime. I report the experimental demonstration of a method, based on optimal quantum cloning, for measuring low optical radiances in an absolute way. Moreover, I present the realization of photon number resolving detectors at infrared wavelengths and room temperature operation.
Quantum communication attempts to harness the unique rules of quantum mechanics to perform communication tasks that are difficult or impossible using classical rules. To realize these benefits, information must be carried on quantum systems. Photons make excellent carriers because they interact very little with the environment, move quickly, and can naturally store quantum information in their polarization. However, it is notoriously difficult to detect a single photon without destroying it. Standard detectors simply absorb the photon, losing the quantum information. This is a critical outstanding problem in quantum communication, as advanced protocols need to know exactly when a photon has arrived at a receiver after transmission through the atmosphere or an optical fibre before performing further quantum-information-processing tasks. Certifying a photon’s presence is of particular interest in tests of Bell’s inequalities, which have only recently been performed without loopholes arising from photon loss, and in device-independent quantum cryptography, which relies on such Bell tests for security. \n \nIn this thesis, I first present work on directly reducing losses in a successful loophole-free Bell test. This is an extremely difficult task that cannot be extended for long-distance communication. Therefore I then focus on ways to circumvent loss by detecting photons without destroying them while preserving their quantum information. First I analyze theoretically a way to herald photons using only linear-optical elements (beam splitters and phase shifters) and extra ancilla photons. Similar but older methods have been demonstrated experimentally by other groups, and my improvements will help future advanced quantum communication protocols. \n \nThe main experiment in this thesis certifies the presence of a photon in a rather simple way: split the photon into two using a nonlinear optical crystal, then detect one of the pair to herald the other. I show in this first proof-of-principle experiment that photonic qubit precertification indeed preserves qubit states, with up to (92.3 ± 0.6)% fidelity and rates of 1100 events per hour. With reductions in detector dark counts, precertification could outperform direct transmission, even with extremely lossy fibre links. \n \nFinally, I present two sources of photons based on nonlinearities in optical fibres. One of the limitations of the photon splitting scheme for heralding is the low success probability due to the very low likelihood of splitting a photon in two. In these fibre photon sources I investigate increasing the splitting likelihood in four-wave mixing through advanced materials and fibre designs. I use polarization-maintaining fibres to generate entangled photon pairs as a prerequisite to precertification, with (92.2 ± 0.2)% fidelity to a maximally-entangled state. Then I show that one type of highly nonlinear chalcogenide glass, never before used for photon pair generation, could outperform standard nonlinear crystals by two orders of magnitude, with calculated conversion efficiency up to 10^-3. To approach the single photon regime, I generate photon pairs in chalcogenide microwires with pump powers as low as 480 nW and verify their timing correlations. \n \nThese advances demonstrate the capability of nondestructive precertification of photons to allow advanced quantum communications protocols even over long distance, and could lead to the first implementations of fully device-independent quantum cryptography.
Shared quantum correlations find application in a wide range of modern quantum information protocols. This thesis presents several optical experiments towards the improved certification of shared quantum correlations, using photonic qubits. The first experiment demonstrates the Einstein–Podolsky–Rosen (EPR) steering effect with no detection loophole. Polarisation–entangled photon pairs generated in a Sagnac interferometer were used to test new loss–tolerant EPR steering inequalities. To test the robustness of the loss–tolerant EPR steering nequalities, a transmission loss of −4.3dB was introduced using a 1km optical fibre loop, finding inequality violations for n = 10 and n = 16 measurement settings with no detection loophole (equating to a total loss of 87%). The findings demonstrate how the new loss–tolerant protocols can be used to certify the EPR steering effect for arbitrarily high losses, and may find application in one–sided device–independent quantum key distribution protocols. The second experiment introduces EPR steering in the context of an EPR steering game. The rules of the game allow for certification of shared quantum correlations via EPR steering inequalites without requiring trust in devices or parties external to a quantum referee. In particular, the experiment successfully demonstrates EPR steering in a measurement–device independent framework; a framework which has typically been accessible only through Bell inequality violations. The findings suggest the possibility for quantum–refereed one–sided device–independent quantum key distribution protocols.
The photon is a quantum system that is by nature robust against noise, and fast travelling, providing an ideal information carrier for quantum information science. The field of quantum information science has generated a great deal of interest for both researchers and the public due to the advantages it can have over classical technologies in areas including communication, computing and cryptography. In this thesis, I explore several different ways that photons can be used to realize quantum information advantages and enable quantum technologies, information tasks and fundamental studies of physics. A strong emphasis is placed on their practical implementation in optical experiments, where the challenges of noise, loss and device imperfections must be considered and combated. I utilize spontaneous parametric downconversion-based sources of high-quality single photons, and their polarization, path, and temporal degrees of freedom for encoding quantum information. In my first experimental project, I demonstrate the first violation of noncontextuality with time-polarization intraparticle entangled states encoded in a single photon by implementing a powerful interference-based measurement technique for photonic states. I perform a test of noncontextuality, acquiring a parameter |SCHSH| = 2.744 ± 0.006, which violates the classical bound of 2 by over 110 standard deviations, rigorously certifying both entanglement and contextuality of the system. We propose a new approach for preparing and measuring high-dimensional time-bin states, that overcomes many of the limitations of previous techniques, and demonstrate it for time-bin qubits and qutrits. In the next experimental project, I investigate the topic of universal cloning in quantum steering-with cloning and steering being two fundamental aspects of quantum physics deeply involved in the security of quantum protocols. I report the first experimental demonstration of cloned quantum steering, showing a simultaneous violation in a steering test by two clones made from one part of an entangled pair of photons. This provides a conclusive result on the question of whether the cloning of quantum steering is possible. We also present theoretical results that clarify our understanding of cloned steering for qubits: we find a no-go theorem where quantum steering can only be copied by a qubit universal cloning machine for 2 and 3 clones, and a monogamy relation where for N clones, steering is only possible if a minimum of N + 1 measurements are performed on each clone. I discuss the field of random number generation, and study how quantum physics allows for certifiably unpredictable random sequences, without needing complete trust in all of the physical devices, offering high levels of security over classical approaches. I report the first discrete-variable detection-loophole-free implementation of one-sided device-independent randomness expansion of certified random bits, based on the quantum steering task. These results illustrate an approach to secure randomness with greater tolerance to noise and loss compared to Bell test-based protocols. The final experimental project looks at quantum autoencoders, which are a quantum machine learning tool that we investigate for the purpose of denoising quantum states. I model and simulate a denoising quantum autoencoder which compresses ququarts into a qubit space and reconstructs noise-reduced ququart states. I construct an experimental apparatus that implements this device, and demonstrate quantum state tomography of ququart states, and the training of the autoencoder.
In 1935 Einstein, Podolsky and Rosen used the assumption of local realism to conclude in a Gedankenexperiment with two entangled particles that quantum mechanics is not complete. For this reason EPR motivated an extension of quantum mechanics by so-called local hidden variables. Based on this idea in 1964 Bell constructed a mathematical inequality whereby experimental tests could distinguish between quantum mechanics and local-realistic theories. Many experiments have since been done that are consistent with quantum mechanics, disproving the concept of local realism. But all these tests suffered from loopholes allowing a local-realistic explanation of the experimental observations by exploiting either the low detector efficiency or the fact that the detected particles were not observed space-like separated. In this context, of special interest is entanglement between different quantum objects like atoms and photons, because it allows one to entangle distant atoms by the interference of photons. The resulting space-like separation together with the almost perfect detection efficiency of the atoms allows a first loophole-free test of Bell's inequality. The primary goal of the present thesis is the experimental realization of entanglement between a single localized atom and a single spontaneously emitted photon at a wavelength suitable for the transport over long distances. In the experiment a single optically trapped Rb87 atom is excited to a state which has two selected decay channels. In the following spontaneous decay a photon is emitted coherently with equal probability into both decay channels. This accounts for perfect correlations between the polarization state of the emitted photon and the Zeeman state of the atom after spontaneous decay. Because these decay channels are spectrally and in all other degrees of freedom indistinguishable, the spin state of the atom is entangled with the polarization state of the photon. To verify entanglement, appropriate correlation measurements in complementary bases of the photon polarization and the internal quantum state of the atom are performed. It is shown, that the generated atom-photon state yields an entanglement fidelity of 0.82. The experimental results of this work mark an important step towards the generation of entanglement between space-like separated atoms for a first loophole-free test of Bell's inequality. Furthermore entanglement between a single atom and a single photon is an important tool for new quantum communication and information applications, e.g. the remote state preparation of a single atom over large distances.