In this thesis, I present experimental and theoretical work which assesses and develops a range of tools that are required for performing quantum information processing, particularly in photonic systems. I investigate the three degrees of freedom of a single photon—its polarisation, spatialmomentum and time-frequency distributions. For polarisation, I show that using wave plates to implement arbitrary, single-qubit rotations is more complicated than is commonly appreciated. In the spatial-momentum and time-frequency domains, I develop ways to perform tomographic analysis of quantum states, and I report the first demonstrations of these techniques. In the time-frequency domain, the tomography technique utilises entanglement in the photon polarisation as a resource to store and provide access to the time-frequency information. In my first two experiments, I use spontaneous parametric down-conversion to produce entanglement between pairs of single photons in all three degrees of freedom. I demonstrate the first characterisation of entanglement in spatial modes and the time-frequency domain, the first quantitative measurement of entangled qutrit states, and the highest quality entangled states yet measured in both polarisation and spatial modes. I also report the first realisation of complete hyperentanglement, and a full, black-box tomography of a 36-dimensional two-photon state—the largest system to be characterised in this way to date. In my final experiment, I model and implement a new architecture for a controlled-Z gate which is much simpler to align than previous implementations. This gate requires only one non-classical interference condition, the visibility of which is the main limitation to its performance. I show that the gate operates effectively as a means of both creating entanglement and discriminating between the four elements in a basis of maximally entangled, Bell-type states. Indeed, its observed performance as a Bell analyser would be sufficient to build a quantum state teleporter which would guarantee that the recipient would be left with a better copy of an unknown input state than any eavesdropper. In a series of numerical simulations, I investigate some of the practicalities that arise when using tomographic reconstruction techniques, including how to estimate errors, which measurements to make and what is actually the optimal reconstruction. In particular, I show that tomographies perform better when based on the results from over-complete sets of measurements. Finally, I discuss the important issue of how to compare two processes, particularly when trying to assess the quality of a measured process by comparing it to some expected ideal. Judging possible candidate measures against a set of experimentally and theoretically motivated
In this thesis, I present experimental and theoretical work which assesses and develops a range of tools that are required for performing quantum information processing, particularly in photonic systems. I investigate the three degrees of freedom of a single photon—its polarisation, spatialmomentum and time-frequency distributions. For polarisation, I show that using wave plates to implement arbitrary, single-qubit rotations is more complicated than is commonly appreciated. In the spatial-momentum and time-frequency domains, I develop ways to perform tomographic analysis of quantum states, and I report the first demonstrations of these techniques. In the time-frequency domain, the tomography technique utilises entanglement in the photon polarisation as a resource to store and provide access to the time-frequency information. In my first two experiments, I use spontaneous parametric down-conversion to produce entanglement between pairs of single photons in all three degrees of freedom. I demonstrate the first characterisation of entanglement in spatial modes and the time-frequency domain, the first quantitative measurement of entangled qutrit states, and the highest quality entangled states yet measured in both polarisation and spatial modes. I also report the first realisation of complete hyperentanglement, and a full, black-box tomography of a 36-dimensional two-photon state—the largest system to be characterised in this way to date. In my final experiment, I model and implement a new architecture for a controlled-Z gate which is much simpler to align than previous implementations. This gate requires only one non-classical interference condition, the visibility of which is the main limitation to its performance. I show that the gate operates effectively as a means of both creating entanglement and discriminating between the four elements in a basis of maximally entangled, Bell-type states. Indeed, its observed performance as a Bell analyser would be sufficient to build a quantum state teleporter which would guarantee that the recipient would be left with a better copy of an unknown input state than any eavesdropper. In a series of numerical simulations, I investigate some of the practicalities that arise when using tomographic reconstruction techniques, including how to estimate errors, which measurements to make and what is actually the optimal reconstruction. In particular, I show that tomographies perform better when based on the results from over-complete sets of measurements. Finally, I discuss the important issue of how to compare two processes, particularly when trying to assess the quality of a measured process by comparing it to some expected ideal. Judging possible candidate measures against a set of experimentally and theoretically motivated
The nascent field of quantum information offers the promise of dramatic speed increases for certain types of computation and logical protocols which are classically impossible. The phenomenon of nonlocality is fundamental to this study, and polarization-entangled photons o er a clean, bright, and stable system for its experimental investigation. This thesis investigates, both experimentally and theoretically, the creation, manipulation, and measurement of polarization-entangled photon pairs. Our entangled photon pairs are created through spontaneous parametric down-conversion within a pair of adjacent, orthogonally oriented nonlinear crystals. The quality and brightness of this source is then dramatically improved through the use of birefringent crystals which compensate for an angle-dependent phase shift. The use of these compensation crystals has allowed measured count rates of two million pairs per second with 97.7% fidelity (with a maximally entangled state) or alternately, ten thousand pairs per second with 99.5% fidelity. By manipulating these entangled states, it is possible to study both how they change and how they can be used. We discuss the theory of state manipulation and the experimental implementation of extremely precise single-qubit operations. To study the operations themselves, we use quantum process tomography to characterize them and have successfully implemented the first experimental realization of ancilla-assisted process tomography. To study decoherence, we implemented the first experimental decoherence-free subspace. By using techniques developed during these investigations, we are able to transform our source of entangled photons into a source of any two-photon polarization state, mixed or pure. Developing new techniques for state creation and manipulation is possible because of simultaneous development in state measurement. In addition to detailing both a theoretical analysis and experimental instructions for state tomography, we experimentally and theoretically compared state tomography with tests of local realism (Bell inequalities) and entanglement witnesses (an entanglement detection technique). In the process, we have measured the largest violations of local realism to date, both statistical (over 2400-sigma) and absolute (S = 2:826 ± 0:005 -- within 0:2% of a maximal violation).
This thesis describes experimental generation, manipulation and measurement of quantum information using photon pairs emitted in bulk crystals. Multi-photon sources engineered during the course of this thesis have proven to be ideal for original contributions in the field of optical quantum information. \n \nIn the first part of this dissertation, we study nonlocality, bound entanglement and measurement-based quantum computing using entangled resources produced by our source. First, we produced and characterised three-photon GHZ polarisation states. We then experimentally violate the long-standing Svetlichny's inequality with a value of 4.51, which is greater than the classical bound by 3.6 standard deviations. Our results agree with the predictions of quantum mechanics, rule out nonlocal hidden-variable theories and certify the genuine tripartite entanglement achievable by our source. Second, with four-photon polarisation states, we demonstrate bound entanglement in Smolin states and realize all of their conceptually important characteristics. Our results highlight the difficulties to achieve the critical condition of undistillability without completely losing entanglement. We conclude the first part by simulating, for the first time, valence-bond solid states and use them as a resource for measurement-based quantum computing. Affleck-Kennedy-Lieb-Tasaki states are produced with 87% fidelity and single-qubit quantum logic gates reach an average fidelity of 92% over all input states and rotations. \n \nIn the second part of this dissertation, we explore controlled waveform manipulation at the single-photon level. Specifically, we shrink the spectral bandwidth of a single photon from 1740 GHz to 43 GHz and demonstrate tunability over a range 70 times that bandwidth. The results are a considerable addition to the field of quantum frequency conversion and have genuine potential for technological applications.
The photon is a quantum system that is by nature robust against noise, and fast travelling, providing an ideal information carrier for quantum information science. The field of quantum information science has generated a great deal of interest for both researchers and the public due to the advantages it can have over classical technologies in areas including communication, computing and cryptography. In this thesis, I explore several different ways that photons can be used to realize quantum information advantages and enable quantum technologies, information tasks and fundamental studies of physics. A strong emphasis is placed on their practical implementation in optical experiments, where the challenges of noise, loss and device imperfections must be considered and combated. I utilize spontaneous parametric downconversion-based sources of high-quality single photons, and their polarization, path, and temporal degrees of freedom for encoding quantum information. In my first experimental project, I demonstrate the first violation of noncontextuality with time-polarization intraparticle entangled states encoded in a single photon by implementing a powerful interference-based measurement technique for photonic states. I perform a test of noncontextuality, acquiring a parameter |SCHSH| = 2.744 ± 0.006, which violates the classical bound of 2 by over 110 standard deviations, rigorously certifying both entanglement and contextuality of the system. We propose a new approach for preparing and measuring high-dimensional time-bin states, that overcomes many of the limitations of previous techniques, and demonstrate it for time-bin qubits and qutrits. In the next experimental project, I investigate the topic of universal cloning in quantum steering-with cloning and steering being two fundamental aspects of quantum physics deeply involved in the security of quantum protocols. I report the first experimental demonstration of cloned quantum steering, showing a simultaneous violation in a steering test by two clones made from one part of an entangled pair of photons. This provides a conclusive result on the question of whether the cloning of quantum steering is possible. We also present theoretical results that clarify our understanding of cloned steering for qubits: we find a no-go theorem where quantum steering can only be copied by a qubit universal cloning machine for 2 and 3 clones, and a monogamy relation where for N clones, steering is only possible if a minimum of N + 1 measurements are performed on each clone. I discuss the field of random number generation, and study how quantum physics allows for certifiably unpredictable random sequences, without needing complete trust in all of the physical devices, offering high levels of security over classical approaches. I report the first discrete-variable detection-loophole-free implementation of one-sided device-independent randomness expansion of certified random bits, based on the quantum steering task. These results illustrate an approach to secure randomness with greater tolerance to noise and loss compared to Bell test-based protocols. The final experimental project looks at quantum autoencoders, which are a quantum machine learning tool that we investigate for the purpose of denoising quantum states. I model and simulate a denoising quantum autoencoder which compresses ququarts into a qubit space and reconstructs noise-reduced ququart states. I construct an experimental apparatus that implements this device, and demonstrate quantum state tomography of ququart states, and the training of the autoencoder.
This thesis details two experimental tests that can be applied to particular quantum states to reveal important information. We begin by discussing the relevant background in quantum information. We introduce qubits and qudits as basic quantum states, and we discuss the evolution and measurement of quantum states. We then discuss quantum state tomography as a means by which to obtain complete information about a state, followed by a discussion of state discrimination as a means by which to determine the state given the promise that it is drawn from some known set. We then discuss relevant experimental techniques in quantum optics, including measurement, generation of entanglement, and generation of single photons from entanglement. \n \nThe first experiment we discuss deals with the causal structure of a system, which is the description of the origin of correlations between two or more states. The causal structure can be direct-cause, meaning that one state causes the other; common-cause, meaning that both states are caused by another; or hybrid-cause, which is a combination of the two. We perform the first implementation of a new type of tomography to determine the causal structure; this is called causal tomography and functions regardless of whether two qubits are related by a common state, a process, or some combination thereof. We implement a process on two entangled photons so that we can select the exact causal structure that results, which ranges continuously between direct-cause and common-cause structures. Using causal tomography, we recover causal structures that closely match expected results and demonstrate that quantum mechanics provides an advantage in causal inference. \n \nThe second experiment we discuss deals with the unambiguous discrimination of multiple quantum states. For the first time, we apply the principles of unambiguous state discrimination to high-dimensional systems. Given a state chosen randomly out of d possible states encoded in d dimensions, we implement a procedure for determining which state was chosen; this procedure in theory functions without error. We encode and detect the states in the orbital angular momentum degree of freedom up to dimension d=14. Although no experiment can provide perfectly error-free measurement due to inevitable imperfections, we obtain an error rate below the theoretical error rate of minimum-error state discrimination for dimensions up to d=12. At the time of submission of this thesis, this work has been accepted for publication in Physical Review Letters.
We explore the concepts of coherence and entanglement as they apply to both the classical and quantum natures of light. In the classical domain, we take inspiration from the tools and concepts developed in foundational quantum mechanics and quantum information science to gain a better understanding of classical coherence theory of light with multiple degrees of freedom (DoFs). First, we use polarization and spatial parity DoFs to demonstrate the notion of classical entanglement, and show that Bell's measure can serve as a useful tool in distinguishing between classical optical coherence theory. Second, we establish a methodical yet versatile approach called 'optical coherency matrix tomography' for reconstructing the coherency matrix of an electromagnetic beam with multiple DoFs. This technique exploits the analogy between this problem in classical optics and that of tomographically reconstructing the density matrix associated with multipartite quantum states in quantum information science. Third, we report the first experimental measurements of the 4 x 4 coherency matrix associated with an electromagnetic beam in which polarization and a spatial DoF are relevant, ranging from the traditional two-point Young's double slit to spatial parity and orbital angular momentum modes. In the quantum domain, we use the modal structure of classical fields to develop qubits and structure Hilbert spaces for use in quantum information processing. Advancing to three-qubit logic gates is an important step towards the success of optical schemes for quantum computing. We experimentally implement a variety of two- and three- qubit, linear and deterministic, single-photon, controlled, quantum logic gates using polarization and spatial parity qubits. Lastly, we demonstrate the implementation of two-qubit single-photon logic using polarization and orbital angular momentum qubits.
This thesis fathoms the possibilities and limitations of measurements in quantum optics. After a short introduction to the general aspects of measurements in quantum mechanics, it presents three examples of a measurement process in concrete applications to quantum optics. For one, while operators describing quantities of interest might have a simple theoretical form, it is often hard to actually implement a measurement of their expectation values experimentally. This situation is encountered in the first part which is devoted to the measurement of quantum statistical properties of a light beam. In contrast to classical optics, these statistics are not fully determined by first- and second-order correlations. Instead, higher-order correlations, usually described by non-Hermitian operators, are necessary to characterize the quantum state completely. A particular example is the N-photon Fock state, for which only a measurement of the Nth-order correlations allows for a full characterization. Here, we present a new method how to measure an important class of Nth-order correlations for arbitrary N in a single spatial mode with two polarizations with limited experimental resources. The second part is again centered around the realization of specific measurement operators for photon correlation measurements. However, in contrast to the previous chapter, these measurements are not an end in their own, but are designed to create specific quantum states as a consequence of the measurement process: A suitable measurement of photons emitted by a number of atoms allows to transfer the atoms into long-lived entangled states. We find that with this method it is possible to entangle two remote atomic qubits to an arbitrary and well-defined degree. Furthermore, we show how to generate two families of quantum states in an arbitrary number of remote atomic qubits: one family consists of all -- symmetric and non-symmetric -- total angular momentum eigenstates in N remote qubits, the other is a family of cluster states. It is also systematically investigated whether the technique of quantum state engineering by projective measurements allows for the creation of any arbitrary state. We find explicit solutions for the case of two and three qubits, while it is shown that no solution exist for N > 6. We conclude the section by proving that with some changes in the setup, this measurement-based quantum state engineering technique allows to create the same states among the scattered photons themselves rather than among the emitting atoms. The last part is devoted to the amount of information one is able to gain about a given system when performing a measurement. The corresponding limits of information are investigated at the example of the duality that arises in a two-way interferometer between the visibility of the interference pattern and the knowledge about the path of the interfering object. We show that there exist correlations between the phase difference the interfering object acquires on its way through the interferometer and the amount of which-way information retrievable from certain observables of the which-way detector. In this way, the which-way information becomes a phase-dependent quantity. In particular, we find that for certain values of the phase shift, the amount of extractable which-way information can be larger than allowed by phase-independent measurement. This property is put to use to find the optimal observable for the which-way detector readout in dependence on the phase of the interfering object. Following this strategy, we are able to gain more which-way information than previously thought possible.