This thesis fathoms the possibilities and limitations of measurements in quantum optics. After a short introduction to the general aspects of measurements in quantum mechanics, it presents three examples of a measurement process in concrete applications to quantum optics. For one, while operators describing quantities of interest might have a simple theoretical form, it is often hard to actually implement a measurement of their expectation values experimentally. This situation is encountered in the first part which is devoted to the measurement of quantum statistical properties of a light beam. In contrast to classical optics, these statistics are not fully determined by first- and second-order correlations. Instead, higher-order correlations, usually described by non-Hermitian operators, are necessary to characterize the quantum state completely. A particular example is the N-photon Fock state, for which only a measurement of the Nth-order correlations allows for a full characterization. Here, we present a new method how to measure an important class of Nth-order correlations for arbitrary N in a single spatial mode with two polarizations with limited experimental resources. The second part is again centered around the realization of specific measurement operators for photon correlation measurements. However, in contrast to the previous chapter, these measurements are not an end in their own, but are designed to create specific quantum states as a consequence of the measurement process: A suitable measurement of photons emitted by a number of atoms allows to transfer the atoms into long-lived entangled states. We find that with this method it is possible to entangle two remote atomic qubits to an arbitrary and well-defined degree. Furthermore, we show how to generate two families of quantum states in an arbitrary number of remote atomic qubits: one family consists of all -- symmetric and non-symmetric -- total angular momentum eigenstates in N remote qubits, the other is a family of cluster states. It is also systematically investigated whether the technique of quantum state engineering by projective measurements allows for the creation of any arbitrary state. We find explicit solutions for the case of two and three qubits, while it is shown that no solution exist for N > 6. We conclude the section by proving that with some changes in the setup, this measurement-based quantum state engineering technique allows to create the same states among the scattered photons themselves rather than among the emitting atoms. The last part is devoted to the amount of information one is able to gain about a given system when performing a measurement. The corresponding limits of information are investigated at the example of the duality that arises in a two-way interferometer between the visibility of the interference pattern and the knowledge about the path of the interfering object. We show that there exist correlations between the phase difference the interfering object acquires on its way through the interferometer and the amount of which-way information retrievable from certain observables of the which-way detector. In this way, the which-way information becomes a phase-dependent quantity. In particular, we find that for certain values of the phase shift, the amount of extractable which-way information can be larger than allowed by phase-independent measurement. This property is put to use to find the optimal observable for the which-way detector readout in dependence on the phase of the interfering object. Following this strategy, we are able to gain more which-way information than previously thought possible.
This thesis fathoms the possibilities and limitations of measurements in quantum optics. After a short introduction to the general aspects of measurements in quantum mechanics, it presents three examples of a measurement process in concrete applications to quantum optics. For one, while operators describing quantities of interest might have a simple theoretical form, it is often hard to actually implement a measurement of their expectation values experimentally. This situation is encountered in the first part which is devoted to the measurement of quantum statistical properties of a light beam. In contrast to classical optics, these statistics are not fully determined by first- and second-order correlations. Instead, higher-order correlations, usually described by non-Hermitian operators, are necessary to characterize the quantum state completely. A particular example is the N-photon Fock state, for which only a measurement of the Nth-order correlations allows for a full characterization. Here, we present a new method how to measure an important class of Nth-order correlations for arbitrary N in a single spatial mode with two polarizations with limited experimental resources. The second part is again centered around the realization of specific measurement operators for photon correlation measurements. However, in contrast to the previous chapter, these measurements are not an end in their own, but are designed to create specific quantum states as a consequence of the measurement process: A suitable measurement of photons emitted by a number of atoms allows to transfer the atoms into long-lived entangled states. We find that with this method it is possible to entangle two remote atomic qubits to an arbitrary and well-defined degree. Furthermore, we show how to generate two families of quantum states in an arbitrary number of remote atomic qubits: one family consists of all -- symmetric and non-symmetric -- total angular momentum eigenstates in N remote qubits, the other is a family of cluster states. It is also systematically investigated whether the technique of quantum state engineering by projective measurements allows for the creation of any arbitrary state. We find explicit solutions for the case of two and three qubits, while it is shown that no solution exist for N > 6. We conclude the section by proving that with some changes in the setup, this measurement-based quantum state engineering technique allows to create the same states among the scattered photons themselves rather than among the emitting atoms. The last part is devoted to the amount of information one is able to gain about a given system when performing a measurement. The corresponding limits of information are investigated at the example of the duality that arises in a two-way interferometer between the visibility of the interference pattern and the knowledge about the path of the interfering object. We show that there exist correlations between the phase difference the interfering object acquires on its way through the interferometer and the amount of which-way information retrievable from certain observables of the which-way detector. In this way, the which-way information becomes a phase-dependent quantity. In particular, we find that for certain values of the phase shift, the amount of extractable which-way information can be larger than allowed by phase-independent measurement. This property is put to use to find the optimal observable for the which-way detector readout in dependence on the phase of the interfering object. Following this strategy, we are able to gain more which-way information than previously thought possible.
In this thesis, I present experimental and theoretical work which assesses and develops a range of tools that are required for performing quantum information processing, particularly in photonic systems. I investigate the three degrees of freedom of a single photon—its polarisation, spatialmomentum and time-frequency distributions. For polarisation, I show that using wave plates to implement arbitrary, single-qubit rotations is more complicated than is commonly appreciated. In the spatial-momentum and time-frequency domains, I develop ways to perform tomographic analysis of quantum states, and I report the first demonstrations of these techniques. In the time-frequency domain, the tomography technique utilises entanglement in the photon polarisation as a resource to store and provide access to the time-frequency information. In my first two experiments, I use spontaneous parametric down-conversion to produce entanglement between pairs of single photons in all three degrees of freedom. I demonstrate the first characterisation of entanglement in spatial modes and the time-frequency domain, the first quantitative measurement of entangled qutrit states, and the highest quality entangled states yet measured in both polarisation and spatial modes. I also report the first realisation of complete hyperentanglement, and a full, black-box tomography of a 36-dimensional two-photon state—the largest system to be characterised in this way to date. In my final experiment, I model and implement a new architecture for a controlled-Z gate which is much simpler to align than previous implementations. This gate requires only one non-classical interference condition, the visibility of which is the main limitation to its performance. I show that the gate operates effectively as a means of both creating entanglement and discriminating between the four elements in a basis of maximally entangled, Bell-type states. Indeed, its observed performance as a Bell analyser would be sufficient to build a quantum state teleporter which would guarantee that the recipient would be left with a better copy of an unknown input state than any eavesdropper. In a series of numerical simulations, I investigate some of the practicalities that arise when using tomographic reconstruction techniques, including how to estimate errors, which measurements to make and what is actually the optimal reconstruction. In particular, I show that tomographies perform better when based on the results from over-complete sets of measurements. Finally, I discuss the important issue of how to compare two processes, particularly when trying to assess the quality of a measured process by comparing it to some expected ideal. Judging possible candidate measures against a set of experimentally and theoretically motivated
In the case of mixed states ρAB of the composite system A ⊗ B, the previous relation generalizes to ρAB = ∑ k pkρ A k ⊗ρk , where pk are probabilities and ρk ’s (ρk ’s) are generic density matrix of the system A (B). The entanglement derives from “subtle” nonlocal correlations between the parts of a quantum system and combines three basic structural elements of quantum theory: the superposition principle, the quantum non-separability property and the exponential scaling of the state space with the number of partitions. This unique resource can be used to perform computational and cryptographic tasks otherwise impossible with classical systems. An entangled state shared by two or more separated parties is a valuable resource for fundamental quantum protocols, such as quantum teleportation [2], quantum computing [3] and quantum cryptography. By using entangled states we can deeply investigate the nonlocal properties of the quantum world. In fact, an entangled system exhibits correlations between two (or more) parties, which cannot be reproduced by a classical theory or, in general, by a Local Hidden Variables Theory (LHVT). Quantum optics represents an excellent experimental test bench for various novel concepts introduced within the framework of quantum information theory. Quantum states of photons, generally produced by a probabilistic process, namely spontaneous parametric down conversion (SPDC), may be easily and accurately manipulated using linear and nonlinear optical devices and measured by efficient single-photon detectors. Photonic qubits represent the typical carrier of quantum information and can be distributed over long distances, either in free-space or in low-loss optical fibers. Two-particle experiments correspond to operate with qubits belonging to a (2 × 2) Hilbert space. Many quantum information tasks and fundamental tests of quantum mechanics, such as the simulation of properties of quantum systems, the realization of quantum algorithms of increasing complexity and the investigation of the quantum world at a mesoscopic level, deal with a large number of qubits. In order to take full advantage of the possibilities offered by quantum mechanics, more qubits must be added to a quantum state. Two approaches may be followed to increase the number of qubits. The first one consists of increasing the number of entangled particles. In this way, multi-qubit entangled states are created by distributing the qubits between the particles so that each particle carries one qubit. A second strategy consists of encoding more than one qubit in each particle, by exploiting different degrees of freedom (DOFs) of the photon such as the polarization, the path, the emission time, the orbital angular momentum. This has been used to create two-photon fourand six-qubit states and up to five-photon ten-qubit graph states. The entanglement of two particles in different DOFs corresponds to socalled hyperentanglement. It is worth noting that multi-qubit hyperentanglement allows to achieve higher
This thesis summarizes investigations on quantum correlations in the fluorescence light of single trapped atoms. The results found have applications in the broad field of quantum information science: it is shown how to overcome classical imaging boundaries using a new developed scheme of quantum imaging, how to project and engineer correlated quantum states in the ground states of multi-level atoms by detecting their fluorescence light and how to prove the quantum nature of these correlations using fundamental tests of quantum information science. Without the need of further introduction to these topics it is interesting to note at this early point that all correlations observed are indeed of quantum nature and show in particular entanglement features, while initially the system under consideration is entirely uncorrelated and the only intervention comes along with the measurement process itself. Therefore, this thesis is embedded into a current field of research activities in the area of quantum information science which is commonly referred to as measurement-induced entanglement. In the first part of this thesis, the correlated photon signal as measured in the fluorescence light of single-photon emitters is at the focus of investigations. It is shown that this correlated signal can be used to overcome classical signals in terms of resolution when applied to image processing. In the second part, the fluorescence signal of a system of multi-level atoms is used to project correlated quantum states into the long-lived ground levels of the atoms. Hereby, a broad variety of entangled quantum states can be generated, ranging from symmetric states like the W-states and GHZ-states to arbitrary total angular momentum eigenstates. Finally, the last part of this thesis takes a closer look at the fundamental physical processes inherent in all schemes and applications investigated throughout the thesis. There, amongst others we investigate Bell-type inequalities that are able to prove the quantum nature of the correlations.
This thesis intends to familiarize the reader with the concepts of photon statistics and correlations in quantum optics. Developing light sources that emit quantum states is central for the realization of quantum technologies. One important step in characterizing these sources is the measurement of field fluctuations and correlations, by coincidence measurements. The expectation value of a coincidence measurement, a simultaneous measurement of two intensities (or, more general, four fields), is represented by the fourth-order correlation function. The value of the correlation function, at zero delay between the detection of two photons, reveals important properties of the state to which they belonged, for example the fluctuations of the photon number. Since predictability is important for many applications, light sources emitting single photons are also characterized by the indistinguishability of consecutively emitted photons, or of two photons from separate emitters. In paper I we investigate blinking behaviour in quantum emitters, and its effect on the interference pattern and photon statistics with photons from two separate emitters. Blinking refers to an emitters transition into a non-emitting state, and subsequent transition back to an emitting state. We show that blinking can not be treated as linear loss, when measuring the fourth-order correlation function for two emitters in a Hong-Ou-Mandel setup. In general, a measurement of the fourth-order correlation function is robust to loss, which makes it a very practical tool. However, the relation between recorded coincidence counts and the correlation function is only direct in the limit of zero detection efficiency, and depends on the detection system. In paper II, we show that by adding a variable attenuation in the beam path, we can trace back to the ''true'' value of the correlation function at zero quantum efficiency. This method improves accuracy in correlation measurements by decreasing a systematic error at the expense of an increased statistical error, which is easier to handle, extending the use of coincidence methods to classical and non-classical multi-photon states.
In these notes, based on lectures given as part of the Les Houches summer school on Quantum Optics and Nanophotonics in August, 2013, I have tried to give a brief survey of some important approaches and modern tendencies in quantum measurement. I wish it to be clear from the outset that I shy explicitly away from the "quantum measurement problem," and that the present treatment aims to elucidate the theory and practice of various ways in which measurements can, in light of quantum mechanics, be carried out; and various formalisms for describing them. While the treatment is by necessity largely theoretical, the emphasis is meant to be on an experimental "perspective" on measurement -- that is, to place the priority on the possibility of gaining information through some process, and then attempting to model that process mathematically and consider its ramifications, rather than stressing a particular mathematical definition as the {\it sine qua non} of measurement. The textbook definition of measurement as being a particular set of mathematical operations carried out on particular sorts of operators has been so well drilled into us that many have the unfortunate tendency of saying "that experiment can't be described by projections onto the eigenstates of a Hermitian operator, so it is not really a measurement," when of course any practitioner of an experimental science such as physics should instead say "that experiment allowed us to measure something, and if the standard theory of measurement does not describe it, the standard theory of measurement is incomplete." Idealisations are important, but when the real world breaks the approximations made in the theory, it is the theory which must be fixed, and not the real world.
In this thesis we examine a variety of question regarding several quantum information-theoretic concepts as they manifest in the context of relativistic quantum fields. In particular, we study the qualitative and quantitative structure of entanglement (as well as more generalized quantum correlations) in field theory. Primarily we study the nature of vacuum entanglement, but consider spatial correlations in more general field states as well. We also discuss several novel aspects of particle creation phenomena, which generally go hand in hand with the presence of field entanglement. Such investigations are important from two perspectives. First, we gain enlightening new insight into the nature of quantum fields and, therefore, into the fundamental constituents of the matter contained in our universe. Second, we are able to consider the possibility of utilizing the relativistic nature of quantum fields as a resource for quantum technological tasks such as entanglement distribution, information processing, and metrology. \n \nAs a general guiding principle, here we approach such questions from an operational perspective. That is, we focus less on the mathematical facts derivable from a given theory and instead attempt to answer in what concretely physical ways such facts manifest themselves. For example, in what ways can vacuum entanglement actually be experimentally detected and measured, at least in principle? Such an approach allows us to circumvent otherwise problematic interpretational issues. It also lends itself more naturally to the proposal of real world experiments regarding, and utilizations of, the physics being investigated. In this thesis we utilize two models of detection as applied to field theory. \n \nThe first is one that we will develop from scratch and use to great effect in a number of studies; this is the non-perturbative oscillator detector. In this context, a ``detector" is simply some quantum system that is allowed to interact in some way with a quantum field. The response of this system then gives us information about the field properties. Typically such studies are done perturbatively, which presents several severe limitations on what may be investigated. We develop an alternative model, in which the detector is identified as a quantum harmonic oscillator, that allows non-perturbative solutions. We go on to apply this model to a variety of studies. We start by the examining the Unruh effect in a cavity setting. Not only are we able to examine the thermalization behavior of such a detector (which is stronger than what can be achieved perturbatively), we also demonstrate that the Unruh response is largely independent of the cavity boundary conditions, indicating a surprising amount of generality and universality to the phenomenon. We also consider the spacelike extraction of spatial entanglement by a set of such detectors. This includes the harvesting of genuine tripartite entanglement out of the vacuum, as well as the observation that the extractable quantum discord (a generalized measure of quantum correlations) can be greatly amplified by thermal fluctuations in the field, in opposite behavior to entanglement. This calls into question the nature of quantum discord, but also suggests at the possibility of actually using environmental noise as a quantum computational resource. Next, we use the oscillator detector model to great effect by proposing a method of reliably and sustainably generating and distributing entanglement via a cavity field. This protocol is inherently non-perturbative, and we refer to it as entanglement farming. Lastly, we modify the farming scenario to discover a very sensitive resonance effect that generates a large difference in the protocol output due to a minute change in system parameters, including the length of cavity being used. We put this forth as a potential method of quantum seismic metrology. \n \nThe second model that we will consider simply involves performing projective measurements onto a given set of field modes. We will find, however, that such an approach allows us to solve previously intractable problems. In particular, we apply this procedure to the physically sensible choice of localized, positive frequency field modes. Using this model we perform two different studies. In the first, we consider the response of an observer accelerating not through the vacuum state but rather a thermal state. Such a setting has not been (properly) studied previously, due to the computational challenges involved. By applying the localized projective measurement model we are able determine that such an observer sees both an Unruh response from acceleration and a response from the field thermality and that, critically, these responses are distinguishable. We then go on to examine the degradation of quantum correlations between two observers due to the acceleration of one of the observers. This is a prototypical scenario of interest and, by applying realistic measurement assumptions, we obtain results qualitatively different from many previous works on the issue. \n \nIn addition to these models, we question the nature of vacuum entanglement and particle creation by considering an operationally straightforward procedure that greatly demystifies these phenomena and puts them on to solid, physically concrete grounds. This operation is that of very quickly introducing a boundary condition onto one's field, for example by creating a mirror. The real particles generated in this process will then be quantum entangled with each other, even if they are created at spatially separate locations, and this entanglement derives exactly from the previously present vacuum entanglement. Not only does this realization provide an operationally satisfying interpretation of vacuum entanglement, it also suggests a straightforward procedure for its experimental verification. \n \nIn all of this, the computational framework that we will rely upon is that of Gaussian quantum mechanics. This is a restriction of continuous variable quantum mechanics that, while limited in its applicability, provides extremely powerful computational tools in the cases that it may be used. The scenarios of interest in this thesis fall within this category and lend themselves naturally to a Gaussian approach. With this we are able to perform, near trivially, many otherwise intractable studies.