This thesis describes experimental generation, manipulation and measurement of quantum information using photon pairs emitted in bulk crystals. Multi-photon sources engineered during the course of this thesis have proven to be ideal for original contributions in the field of optical quantum information. \n \nIn the first part of this dissertation, we study nonlocality, bound entanglement and measurement-based quantum computing using entangled resources produced by our source. First, we produced and characterised three-photon GHZ polarisation states. We then experimentally violate the long-standing Svetlichny's inequality with a value of 4.51, which is greater than the classical bound by 3.6 standard deviations. Our results agree with the predictions of quantum mechanics, rule out nonlocal hidden-variable theories and certify the genuine tripartite entanglement achievable by our source. Second, with four-photon polarisation states, we demonstrate bound entanglement in Smolin states and realize all of their conceptually important characteristics. Our results highlight the difficulties to achieve the critical condition of undistillability without completely losing entanglement. We conclude the first part by simulating, for the first time, valence-bond solid states and use them as a resource for measurement-based quantum computing. Affleck-Kennedy-Lieb-Tasaki states are produced with 87% fidelity and single-qubit quantum logic gates reach an average fidelity of 92% over all input states and rotations. \n \nIn the second part of this dissertation, we explore controlled waveform manipulation at the single-photon level. Specifically, we shrink the spectral bandwidth of a single photon from 1740 GHz to 43 GHz and demonstrate tunability over a range 70 times that bandwidth. The results are a considerable addition to the field of quantum frequency conversion and have genuine potential for technological applications.
This thesis describes experimental generation, manipulation and measurement of quantum information using photon pairs emitted in bulk crystals. Multi-photon sources engineered during the course of this thesis have proven to be ideal for original contributions in the field of optical quantum information. \n \nIn the first part of this dissertation, we study nonlocality, bound entanglement and measurement-based quantum computing using entangled resources produced by our source. First, we produced and characterised three-photon GHZ polarisation states. We then experimentally violate the long-standing Svetlichny's inequality with a value of 4.51, which is greater than the classical bound by 3.6 standard deviations. Our results agree with the predictions of quantum mechanics, rule out nonlocal hidden-variable theories and certify the genuine tripartite entanglement achievable by our source. Second, with four-photon polarisation states, we demonstrate bound entanglement in Smolin states and realize all of their conceptually important characteristics. Our results highlight the difficulties to achieve the critical condition of undistillability without completely losing entanglement. We conclude the first part by simulating, for the first time, valence-bond solid states and use them as a resource for measurement-based quantum computing. Affleck-Kennedy-Lieb-Tasaki states are produced with 87% fidelity and single-qubit quantum logic gates reach an average fidelity of 92% over all input states and rotations. \n \nIn the second part of this dissertation, we explore controlled waveform manipulation at the single-photon level. Specifically, we shrink the spectral bandwidth of a single photon from 1740 GHz to 43 GHz and demonstrate tunability over a range 70 times that bandwidth. The results are a considerable addition to the field of quantum frequency conversion and have genuine potential for technological applications.
Entanglement is a key resource in many quantum information schemes and in the last years the research on multi-qubit entanglement has drawn lots of attention. In this thesis the experimental generation and characterisation of multi-qubit entanglement is presented. Specifically we have prepared entangled states of up to six qubits. The qubits were implemented in the polarisation degree of freedom of single photons. We emphasise that one type of states that we produce are rotationally invariant states, remaining unchanged under simultaneous identical unitary transformations of all their individual constituents. Such states can be applied to e.g. decoherence-free encoding, quantum communication without sharing a common reference frame, quantum telecloning, secret sharing and remote state preparation schemes. They also have properties which are interesting in studies of foundations of quantum mechanics. In the experimental implementation we use a single source of entangled photon pairs, based on parametric down-conversion, and extract the first, second and third order events. Our experimental setup is completely free from interferometric overlaps, making it robust and contributing to a high fidelity of the generated states. To our knowledge, the achieved fidelity is the highest that has been observed for six-qubit entangled states and our measurement results are in very good agreement with predictions of quantum theory. We have also performed another novel test of the foundations of quantum mechanics. It is based on an inequality that is fulfilled by any non-contextual hidden variable theory, but can be violated by quantum mechanics. This test is similar to Bell inequality tests, which rule out local hidden variable theories as possible completions of quantum mechanics. Here, however, we show that non-contextual hidden variable theories cannot explain certain experimental results, which are consistent with quantum mechanics. Hence, neither of these theories can be used to make quantum mechanics complete.
In this thesis, I present experimental and theoretical work which assesses and develops a range of tools that are required for performing quantum information processing, particularly in photonic systems. I investigate the three degrees of freedom of a single photon—its polarisation, spatialmomentum and time-frequency distributions. For polarisation, I show that using wave plates to implement arbitrary, single-qubit rotations is more complicated than is commonly appreciated. In the spatial-momentum and time-frequency domains, I develop ways to perform tomographic analysis of quantum states, and I report the first demonstrations of these techniques. In the time-frequency domain, the tomography technique utilises entanglement in the photon polarisation as a resource to store and provide access to the time-frequency information. In my first two experiments, I use spontaneous parametric down-conversion to produce entanglement between pairs of single photons in all three degrees of freedom. I demonstrate the first characterisation of entanglement in spatial modes and the time-frequency domain, the first quantitative measurement of entangled qutrit states, and the highest quality entangled states yet measured in both polarisation and spatial modes. I also report the first realisation of complete hyperentanglement, and a full, black-box tomography of a 36-dimensional two-photon state—the largest system to be characterised in this way to date. In my final experiment, I model and implement a new architecture for a controlled-Z gate which is much simpler to align than previous implementations. This gate requires only one non-classical interference condition, the visibility of which is the main limitation to its performance. I show that the gate operates effectively as a means of both creating entanglement and discriminating between the four elements in a basis of maximally entangled, Bell-type states. Indeed, its observed performance as a Bell analyser would be sufficient to build a quantum state teleporter which would guarantee that the recipient would be left with a better copy of an unknown input state than any eavesdropper. In a series of numerical simulations, I investigate some of the practicalities that arise when using tomographic reconstruction techniques, including how to estimate errors, which measurements to make and what is actually the optimal reconstruction. In particular, I show that tomographies perform better when based on the results from over-complete sets of measurements. Finally, I discuss the important issue of how to compare two processes, particularly when trying to assess the quality of a measured process by comparing it to some expected ideal. Judging possible candidate measures against a set of experimentally and theoretically motivated
The nascent field of quantum information offers the promise of dramatic speed increases for certain types of computation and logical protocols which are classically impossible. The phenomenon of nonlocality is fundamental to this study, and polarization-entangled photons o er a clean, bright, and stable system for its experimental investigation. This thesis investigates, both experimentally and theoretically, the creation, manipulation, and measurement of polarization-entangled photon pairs. Our entangled photon pairs are created through spontaneous parametric down-conversion within a pair of adjacent, orthogonally oriented nonlinear crystals. The quality and brightness of this source is then dramatically improved through the use of birefringent crystals which compensate for an angle-dependent phase shift. The use of these compensation crystals has allowed measured count rates of two million pairs per second with 97.7% fidelity (with a maximally entangled state) or alternately, ten thousand pairs per second with 99.5% fidelity. By manipulating these entangled states, it is possible to study both how they change and how they can be used. We discuss the theory of state manipulation and the experimental implementation of extremely precise single-qubit operations. To study the operations themselves, we use quantum process tomography to characterize them and have successfully implemented the first experimental realization of ancilla-assisted process tomography. To study decoherence, we implemented the first experimental decoherence-free subspace. By using techniques developed during these investigations, we are able to transform our source of entangled photons into a source of any two-photon polarization state, mixed or pure. Developing new techniques for state creation and manipulation is possible because of simultaneous development in state measurement. In addition to detailing both a theoretical analysis and experimental instructions for state tomography, we experimentally and theoretically compared state tomography with tests of local realism (Bell inequalities) and entanglement witnesses (an entanglement detection technique). In the process, we have measured the largest violations of local realism to date, both statistical (over 2400-sigma) and absolute (S = 2:826 ± 0:005 -- within 0:2% of a maximal violation).
The experiments described in this thesis form an investigation into the path towards establishing the requirements of quantum computing in a linear optical system. Our qubits are polarisation encoded photons for which the basic operations of quantum computing, single qubit rotations, are a well understood problem. The difficulty lies in the interaction of photons. To achieve these we use measurement induced non-linearities. The first experiment in this thesis describes the thorough characterisation of a controlled-sign gate based on such non-linearities. The photons are provided as pairs generated through parametric down-conversion, and as such share correlations unlikely to carry over into large scale implementations of the future. En route to such larger circuits, a characterisation of the actions of the controlled-sign gate is conducted, when the input qubits have been generated independently from each other, revealing a large drop in process fidelity. To explore the cause of this degradation of the gate performance a thorough and highly accurate model of the gate is derived including the realistic description of faulty circuitry, photon loss and multi-photon emission by the source. By simulating the effects of the various noise sources individually, the heretofore largely ignored multi-photon emission is identified as the prime cause of the degraded gate performance, causing a drop in fidelity nearly three times as large as any other error source. I further draw the first comparison between the performance of an experimental gate to the error probabilities per gate derived as thresholds for fault-tolerant quantum computing. In the absence of a single vigourous threshold value, I compare the gate performance to the models that yielded the highest threshold to date as an upper bound and to the threshold of the Gremlin-model, which allows for the most general errors. Unsurprisingly this comparison reveals that the implemented gate is clearly insufficient, however just remedying the multi-photon emission error will allow this architecture to move to within striking distance of the boundary for fault-tolerant quantum computing. The utilised methodology can be applied to any gate in any architecture and can, combined with a suitable model of the noise sources, become an important guide for developments required to achieve fault tolerant quantum computing. The final experiment on the path towards linear optical quantum computing is the demonstration of a pair of basic versions of Shor's algorithm which display the essential entanglement for the algorithm. The results again highlight the need for extensive measurements to reveal the fundamental quality of the implemented algorithm, which is not accessible with limited indicative measurements. In the second part of the thesis, I describe two experiments on other forms of entanglement by extending the actions of a Fock-State filter, a filter that is capable of attenuating single photon states stronger than multi-photon states, to produce entangled states. Furthermore this device can be used in conjunction with standard wave-plates to extend the range of operations possible on the bi-photonic qutrit space, showing that this setup suffices to produce any desired qutrit state, thereby giving access to new measurement capabilities and in the process creating and proving the first entanglement between a qubit and a qutrit.
Quantum information has been witnessing great science value and latent application since 1980's. The research work presented here consist of mainly two important parts: manipulations of multiphoton entanglement and atomic ensembles based quantum memory. In first part, the experimental technique multi-photon entanglement is further developed to study fundamental issues in quantum mechanics, remarkable applications to quantum communication and quantum computation. Specifically, we have demonstrated a bit-flip error-free transfer of quantum information, violation of Bell's inequality beyond Tsirelson's bound, teleportation of a two-qubit composite system, as well as the one-way computing by two-photon-four-qubit cluster state. To overcome un-scalability problem due to probabilistic feature in linear optical quantum information processing, we investigated in the second part the physics of atomic ensembles based quantum memory. We show that theoretically, entanglement between distant locations can be deterministically generated. The experimental work has thoroughly developed the necessary techniques and we have achieved deterministic single photon source, and interference of the photons from independent atomic ensembles, teleportation between photonic and atomic qubits, a novel way to create a robust entanglement between an atomic and a photonic qubit, and memory based entanglement swapping. We believe, the developed techniques here would dramatically facilitate progresses in many fields including global quantum communication, linear optical quantum computation and the foundations of quantum mechanics etc.
Light, which is composed of discrete quanta, or photons, is one of the most fundamental concepts in physics. Being an elementary entity, the behaviour of photons is governed by the rules of quantum mechanics. The ability to create, manipulate and measure quantum states of light is not only useful in foundational tests of quantum theory, but also in a wide range of quantum technologies – which aim to utilize non-classical properties of quantum systems to perform tasks not possible with classical resources. Only recently has it been possible to control the properties of number states of light, which have a fixed photon-number. Two-photon states are central to testing fundamental physical theories (such as locality and reality) and the implementation of quantum information technologies. The versatility of photon-pair states is en- abled by the potential entanglement properties it can posses. Thus controlling the correlations between photons is crucial to both pure and applied physics. To produce a single photon, a photon-pair state can be used. Detection of one photon indicates its twin’s existence. Many applications, such as optical quantum computation, require pure indistinguishable single photons. Heralding single pho- tons from a photon-pair will, in general, produce single photons in a mixed quantum state due to correlations within the pair. A common approach to creating photon-pairs is through the nonlinear sponta- neous four-wave mixing interaction in optical fibres. This thesis presents a theoreti- cal and experimental implementation of a scheme to tailor the spectral correlations within the pairs. Emphasis is placed on engineering the two-photon state such that they are completely uncorrelated. Spatial entanglement is naturally avoided due to the discrete nature of the optical fibre modes. Spectral correlations are eliminated by careful choice of dispersion characteristics and conditions. The purity of the photons generated by this scheme is demonstrated by means of two-photon inter- ference from independent sources. We measure a purity of (85.9 ± 1.6)% with no spectral filtering, exhibiting the usefulness of this source for quantum technologies and applications.