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Communications in Theoretical Physics

Mechanisms and modulation of third-order nonlinear optical responses in spherical quantum dots confined by a Mie-type potential

Yue Wu, Xuechao Li

Published Jul 7, 2026• 0 citations
Publisher

Abstract

Abstract This paper systematically explores the third-order nonlinear optical properties and modulation mechanisms of a spherical quantum dot system confined by a Mie-type potential. We analytically solve the Schrödinger equation with Nikiforov–Uvarov method based on effective mass approximation to obtain the eigenenergies and wave function of the system. Subsequently, key third-order nonlinear optical parameters, including the third-harmonic generation (THG) coefficient, total optical absorption coefficients, and refractive index changes, are derived via the density matrix formalism. The results indicate that the nonlinear optical responses strongly depend on the geometric dimensions and the microscopic confinement parameters. By adjusting these parameters, effective control over the THG coefficient can be achieved. Furthermore, this study reveals the significant modulation effects of environmental factors. The synergistic influence of quantum dot size, confinement potential, and environmental interactions is systematically analyzed, providing a theoretical basis for designing high-performance nonlinear optical devices based on quantum dots.

DOI
10.1088/1572-9494/ae86d1

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We study the linear and nonlinear optical properties of a spherical GaAs quantum dot with screened modified Kratzer potential (SMKP) by solving the time-independent Schrödinger wave equation using the diagonalization method. The obtained electronic properties of the system alongside the compact density formalism are used to evaluate the linear, third-order nonlinear and total optical absorption coefficients and change in the relative refractive index of the system. We show that the confinement potential parameters and optical intensity significantly affects the behaviour of absorption coefficients and refractive index changes. It is important to note that the findings of this study will find application in optoelectronics and related areas.
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Analytical expressions for the linear and nonlinear optical susceptibilities of spherical quantum dots are obtained using the Schrödinger equation. To solve the Schrödinger equation, the Nikiforov-Uvarov method was used, assuming that electrons isolated in the medium are associated with the Gelman inverse quadratic potential. Using the density matrix formalism, analytical expressions were obtained for the coefficients of linear and nonlinear absorption and changes in the refractive index of quantum dots. Elements of the matrix of the electric dipole moment l=± 1 and m = 0 are obtained according to the selection rules. To demonstrate the results obtained, we used the real physical characteristics of quantum dots obtained from gallium arsenide (GaAs).