ABSTRACT The multi‐photon bunching effect, arising from intrinsic bosonic exchange symmetry in path interference, underpins numerous quantum information techniques. However, conventional bunching in real space faces challenges in tailoring complex structured light fields. Here, we leverage dielectric metasurfaces with polarization entanglement to generate conjugated structured photons and achieve active control over nonlocal spin bunching between two photons. In the prepared spin–orbit hybrid entangled state, projective spin measurement on the idler photon nonlocally heralds the creation of a conjugated structured photon in the signal arm, residing on a higher‐order Poincaré sphere. By adjusting the relative phase to alter entanglement properties, continuous control can be achieved from spin bunching to anti‐bunching. Exploiting this phase sensitivity enables reconstruction of the conjugated photon's complex amplitude. This work establishes spin bunching as a paradigm for quantum correlation control and demonstrates metasurfaces as a compact, multifunctional platform for structured photonic quantum state engineering and metrology.
ABSTRACT The multi‐photon bunching effect, arising from intrinsic bosonic exchange symmetry in path interference, underpins numerous quantum information techniques. However, conventional bunching in real space faces challenges in tailoring complex structured light fields. Here, we leverage dielectric metasurfaces with polarization entanglement to generate conjugated structured photons and achieve active control over nonlocal spin bunching between two photons. In the prepared spin–orbit hybrid entangled state, projective spin measurement on the idler photon nonlocally heralds the creation of a conjugated structured photon in the signal arm, residing on a higher‐order Poincaré sphere. By adjusting the relative phase to alter entanglement properties, continuous control can be achieved from spin bunching to anti‐bunching. Exploiting this phase sensitivity enables reconstruction of the conjugated photon's complex amplitude. This work establishes spin bunching as a paradigm for quantum correlation control and demonstrates metasurfaces as a compact, multifunctional platform for structured photonic quantum state engineering and metrology.
Quantum entanglement, a fundamental concept in quantum mechanics, lies at the heart of many current and future quantum technologies. A pivotal task is the generation and control of diverse quantum entangled states in a more compact and flexible manner. Here, we introduce an approach to achieve diverse path entanglement by exploiting the interaction between noncommutative metasurfaces and entangled photons. Different from other path entanglements, our quantum path entanglement is evolution path entanglement of photons on Poincaré sphere. Due to quantum entanglement between idler photons and structured signal photons, evolution path of idler photons on the fundamental Poincaré sphere can be nonlocally mirrored by structured signal photons on any higher-order Poincaré sphere, resulting in quantum path entanglement. Benefiting from noncommutative metasurfaces, diverse quantum path entanglement can be switched across different higher-order Poincaré spheres using distinct combination sequences of metasurfaces. Our method allows for the tuning of diverse quantum path entanglement across a broad spectrum of quantum states, offering a significant advancement in the manipulation of quantum entanglement.
Abstract Metasurfaces utilize engineered nanostructures to achieve control on all possible dimensions of light, encouraging versatile applications, including beam steering, multifunctional lensing, and multiplexed holograms. Towards the quantum optical regime for metasurfaces, although significant efforts have been put into generating and analyzing specific quantum states, control schemes to further manipulate these quantum states or information are still limited. Here, based on a metasurface, we propose and experimentally demonstrate a continuous heralding scheme to remotely control a vortex beam with high robustness to noise using polarization-entangled photon pairs. Our metasurface entangles polarization and orbital angular momentum (OAM) and the polarization selection on heralding photon erases the which-OAM information on signal photon. It induces an interference of two different OAM states remotely, manifesting a continuous orbital rotation. Our results show that metasurfaces have potential applications in quantum communication and information processing in entangling information with increasing complexity in the content.
Quantum-enhanced optical sensing leverages correlations and entanglement in multiphoton states to surpass the limitations of classical measurement. However, the widespread deployment of quantum imaging and polarimetry has been hindered by bulky nonlinear crystals, alignment-sensitive free-space optics, and limited control over the spatial and polarization structure of quantum light. This thesis investigates how engineered nanophotonic metasurfaces, together with two-photon probing schemes, can overcome these constraints and enable compact, versatile, and high-performance quantum sensing platforms. The first component of the thesis introduces a metasurface-enabled quantum imaging system based on spatially entangled photon pairs generated from a subwavelength-thick lithium niobate (LiNbO3) nonlinear metasurface. Exploiting nonlocal guided-mode resonances with strong angular dispersion, the system realizes a hybrid imaging protocol that combines quantum ghost imaging with all-optical wavelength-controlled scanning. A theoretical framework linking momentum-space biphoton correlations to image formation is developed, including the effects of pump-beam waist and metasurface quality factor. Numerical simulations and proof-of-principle experiments demonstrate 2D imaging with strong contrast and establish that metasurface-based photon-pair sources can achieve fields of view and resolution-cell counts far beyond what is possible with bulk-crystal SPDC. Building on this platform, the thesis presents the first quantum phase imaging system that integrates metasurfaces for both photon-pair generation and phase-gradient detection. A silicon (Si) metasurface with a near-linear optical transfer function directly maps phase gradients of transparent samples into spatial quantum correlations, eliminating the need for interferometers or long propagation paths. Experiments show that phase gradients up to 25rad/mm can be retrieved with high fidelity, and the system supports switchable operation between amplitude and phase imaging within a significantly more compact scale. The final component of the thesis develops a two-photon probing quantum polarimetry (TPQP) protocol for characterizing scattering media. By combining Monte Carlo modeling of microscopic photon trajectories with Mueller-matrix decomposition and quantum state tomography, the framework links entanglement degradation to macroscopic polarization observables and resolves ambiguities in Mueller-matrix extraction through tailored probe states. Experiments using tissue-mimicking phantoms confirm that TPQP exhibits significantly higher sensitivity to depolarization than one-photon probing, validating its potential for quantum-enhanced polarimetric sensing and imaging. Overall, this thesis advances quantum optical sensing through two distinct but complementary directions. The first two parts demonstrate how engineered metasurfaces enable compact quantum imaging and phase-gradient detection by integrating photon-pair generation and spatial processing within ultrathin nanophotonic structures. Independently, the two-photon probing quantum polarimetry framework, implemented using a conventional BBO-based entangled source, shows how nonlinear two-photon correlations can enhance sensitivity to depolarization and improve Mueller-matrix reconstruction in scattering media. Although realized on different physical platforms, all components of this work exploit quantum correlations to extract amplitude, phase, and polarization information beyond classical approaches, contributing to the development of practical quantum sensing methodologies.
Light carries both spin (polarization) and orbital angular momentum. Combining these degrees of freedom produces hybrid spin-orbit states that live in a high-dimensional Hilbert space, offering greater information capacity and robustness for optical communication, quantum technologies, and metrology. However, generating arbitrary states in these spaces and characterizing them efficiently has remained difficult. Here we show a compact metasurface that generates arbitrary spin-orbit states in a four-dimensional Hilbert space, visualized on a Poincaré hypersphere, with straightforward scalability to higher dimensions. Using a tetratomic unit cell, the single-layer device precisely controls complex amplitude, phase, and polarization. We further introduce an efficient interferometric scheme that reconstructs the full density matrix of any N-dimensional spin-orbit state using only three interferograms. This approach uncovers an intrinsic spin-orbit parity order that governs the symmetry of projected intensity patterns, independent of the weighting of the eigenmodes, and enables controlled mode transformations through higher-order geometric phases. These advances establish a versatile platform for high-dimensional photonic technologies.
Optical metasurfaces open new avenues for the precise wavefront control of light for integrated quantum technology. Here, we demonstrate a hybrid integrated quantum photonic system that is capable of entangling and disentangling two-photon spin states at a dielectric metasurface. Via the interference of single-photon pairs at a nanostructured dielectric metasurface, a path-entangled two-photon NOON state with circular polarization that exhibits a quantum HOM interference visibility of 86 ± 4% is generated. Furthermore, we demonstrate nonclassicality andphase sensitivity in a metasurface-based interferometer with a fringe visibility of 86.8 ± 1.1% in the coincidence counts. This high visibility proves the metasurface-induced path entanglement inside the interferometer. Our findings provide a promising way to develop hybrid-integrated quantum technology operating in the high-dimensional mode space in various applications, such as imaging, sensing, and computing.
Metasurfaces, with their capability to control all possible dimensions of light, have become integral to quantum optical applications, including quantum state generation, operation, and tomography. We utilize a metasurface to generate polarization–hologram hybrid entanglement between a signal–idler photon pair to construct a quantum hologram. The properties of the quantum hologram can be revealed by collapsing the polarization degree of freedom of the idler photon, inducing interference between two holographic states of the signal photon as a meaningful and selective erasure of the holographic content. On the contrary, interference disappears when the idler photon is detected without observing polarization. This process can be further interpreted as a quantum holographic eraser, where the erasing action is visualized with erased contents in holograms. Our construction of a polarization–hologram hybrid entangled state with metasurfaces will be useful for quantum communication with enhanced robustness, anticounterfeiting applications through the additional quantum degrees of freedom or phase difference between two holographic states, and as an emerging platform for exploring fundamental quantum concepts for entanglement and nonlocality.