Quantum metasurface for multiphoton interference and state reconstruction
Kai Wang, James Titchener, Sergey Kruk, Lei Xu, Hung-Pin Chung, Matthew Parry, Ivan I. Kravchenko, Yen-Hung Chen, Alexander S. Solntsev, Yuri S. Kivshar, Dragomir N. Neshev, Andrey A. Sukhorukov
Metasurfaces based on resonant nanophotonic structures have enabled innovative types of flat-optics devices that often outperform the capabilities of bulk components, yet these advances remain largely unexplored for quantum applications. We show that nonclassical multiphoton interferences can be achieved at the subwavelength scale in all-dielectric metasurfaces. We simultaneously image multiple projections of quantum states with a single metasurface, enabling a robust reconstruction of amplitude, phase, coherence, and entanglement of multiphoton polarization-encoded states. One- and two-photon states are reconstructed through nonlocal photon correlation measurements with polarization-insensitive click detectors positioned after the metasurface, and the scalability to higher photon numbers is established theoretically. Our work illustrates the feasibility of ultrathin quantum metadevices for the manipulation and measurement of multiphoton quantum states, with applications in free-space quantum imaging and communications.
Metasurfaces based on resonant nanophotonic structures have enabled innovative types of flat-optics devices that often outperform the capabilities of bulk components, yet these advances remain largely unexplored for quantum applications. We show that nonclassical multiphoton interferences can be achieved at the subwavelength scale in all-dielectric metasurfaces. We simultaneously image multiple projections of quantum states with a single metasurface, enabling a robust reconstruction of amplitude, phase, coherence, and entanglement of multiphoton polarization-encoded states. One- and two-photon states are reconstructed through nonlocal photon correlation measurements with polarization-insensitive click detectors positioned after the metasurface, and the scalability to higher photon numbers is established theoretically. Our work illustrates the feasibility of ultrathin quantum metadevices for the manipulation and measurement of multiphoton quantum states, with applications in free-space quantum imaging and communications.
With recent advances in nanophotonics, metasurfaces based on nano-resonators have facilitated novel types of optical devices. In particular, the interplay between different degrees of freedom, involving polarization and spatial modes, boosted classical polarization measurements and imaging applications. However, the use of metasurfaces for measuring the quantum states of light remains largely unexplored. Conventionally, the task of quantum state tomography is realized with several bulk optical elements, which need to be reconfigured multiple times. Such setups can suffer from decoherence, and there is a fundamental and practical interest in developing integrated solutions for measurement of multi-photon quantum states. We present a new concept and the first experimental realization of all-dielectric metasurfaces with no tuneable elements for imaging-based reconstruction of the full quantum state of entangled photons. Most prominently, we implement multi-photon interferometric measurements on a sub-wavelength thin optical element, which delivers ultimate miniaturization and extremely high robustness. Specifically, we realize a highly transparent all-dielectric metasurface, which spatially splits different components of quantum-polarization states. Then, a simple one-shot measurement of correlations with polarization-insensitive on-off click detectors enables complete reconstruction of multi-photon density matrices with high precision. In our experiment, we prepare sets of polarization states and reconstruct their density matrices with a high fidelity of over 99% for single photon states and above 95% for two-photon states. Our work provides a fundamental advance in the imaging of quantum states, where multi-photon quantum interference takes place at sub-wavelength scale.
Summary form only given. Measurements of quantum states of photons are conventionally performed with series of optical elements in bulk setups [1] or optical chips incorporating multiple tunable beam splitters. Here, we suggest and develop experimentally, for the first time to our knowledge, a new concept of quantum-polarization measurements with a single all-dielectric resonant metasurface [2]. The operating principle is presented in Fig. 1(a): A metasurface spatially splits different components of photon polarization states, which then enables full reconstruction of the photon state based on the photon correlations with simple polarization-insensitive single-photon detectors or EMCCD cameras. The subwavelength thin structure provides an ultimate miniaturization, and can facilitate quantum tomography by spatially-resolved imaging without a need for reconfiguration. Such parallel-detection approach promises not only better robustness and scalability, but also the possibility to study the dynamics of quantum states in real-time.
Metasurface enables the generation and manipulation of multiphoton entanglement with flat optics, providing a more efficient platform for large-scale photonic quantum information processing. Here, we show that a single metasurface optical device would allow more efficient characterizations of multiphoton entangled states, such as shadow tomography, which generally requires fast and complicated control of optical setups to perform information-complete measurements, a demanding task using conventional optics. The compact and stable device here allows implementations of general positive operator valued measures with a reduced sample complexity and significantly alleviates the experimental complexity to implement shadow tomography. Integrating self-learning and calibration algorithms, we observe notable advantages in the reconstruction of multiphoton entanglement, including using fewer measurements, having higher accuracy, and being robust against experimental imperfections. Our work unveils the feasibility of metasurface as a favorable integrated optical device for efficient characterization of multiphoton entanglement, and sheds light on scalable photonic quantum technologies with ultra-thin optical devices.
Quantum-enhanced optical sensing leverages correlations and entanglement in multiphoton states to surpass the limitations of classical measurement. However, the widespread deployment of quantum imaging and polarimetry has been hindered by bulky nonlinear crystals, alignment-sensitive free-space optics, and limited control over the spatial and polarization structure of quantum light. This thesis investigates how engineered nanophotonic metasurfaces, together with two-photon probing schemes, can overcome these constraints and enable compact, versatile, and high-performance quantum sensing platforms. The first component of the thesis introduces a metasurface-enabled quantum imaging system based on spatially entangled photon pairs generated from a subwavelength-thick lithium niobate (LiNbO3) nonlinear metasurface. Exploiting nonlocal guided-mode resonances with strong angular dispersion, the system realizes a hybrid imaging protocol that combines quantum ghost imaging with all-optical wavelength-controlled scanning. A theoretical framework linking momentum-space biphoton correlations to image formation is developed, including the effects of pump-beam waist and metasurface quality factor. Numerical simulations and proof-of-principle experiments demonstrate 2D imaging with strong contrast and establish that metasurface-based photon-pair sources can achieve fields of view and resolution-cell counts far beyond what is possible with bulk-crystal SPDC. Building on this platform, the thesis presents the first quantum phase imaging system that integrates metasurfaces for both photon-pair generation and phase-gradient detection. A silicon (Si) metasurface with a near-linear optical transfer function directly maps phase gradients of transparent samples into spatial quantum correlations, eliminating the need for interferometers or long propagation paths. Experiments show that phase gradients up to 25rad/mm can be retrieved with high fidelity, and the system supports switchable operation between amplitude and phase imaging within a significantly more compact scale. The final component of the thesis develops a two-photon probing quantum polarimetry (TPQP) protocol for characterizing scattering media. By combining Monte Carlo modeling of microscopic photon trajectories with Mueller-matrix decomposition and quantum state tomography, the framework links entanglement degradation to macroscopic polarization observables and resolves ambiguities in Mueller-matrix extraction through tailored probe states. Experiments using tissue-mimicking phantoms confirm that TPQP exhibits significantly higher sensitivity to depolarization than one-photon probing, validating its potential for quantum-enhanced polarimetric sensing and imaging. Overall, this thesis advances quantum optical sensing through two distinct but complementary directions. The first two parts demonstrate how engineered metasurfaces enable compact quantum imaging and phase-gradient detection by integrating photon-pair generation and spatial processing within ultrathin nanophotonic structures. Independently, the two-photon probing quantum polarimetry framework, implemented using a conventional BBO-based entangled source, shows how nonlinear two-photon correlations can enhance sensitivity to depolarization and improve Mueller-matrix reconstruction in scattering media. Although realized on different physical platforms, all components of this work exploit quantum correlations to extract amplitude, phase, and polarization information beyond classical approaches, contributing to the development of practical quantum sensing methodologies.
Abstract Nonlinear metasurfaces with subwavelength thickness were recently established as versatile platforms for the enhanced and tailorable generation of entangled photon pairs. The small dimensions and inherent stability of integrated metasurface sources are attractive for free-space applications in quantum communications, sensing, and imaging, yet this remarkable potential remained unexplored. Here, we formulate and experimentally demonstrate the unique benefits and practical potential of nonlinear metasurfaces for quantum imaging at infrared wavelengths, facilitating an efficient protocol combining ghost and all-optical scanning imaging. The metasurface incorporates a subwavelength-scale silica metagrating on a lithium niobate thin film. Its distinguishing feature is the capability to all-optically scan the photon emission angle in the direction across the grating simply by tuning the pump beam wavelength. Simultaneously, the photon emission is broad and anti-correlated along the grating direction, allowing for ghost imaging. Thereby, we reconstruct the images of 2D objects using just a 1D detector array in the idler path and a bucket detector in the signal path, by recording the dependencies of photon coincidences on the pump wavelength. Furthermore, we theoretically demonstrate the quantum imaging of objects with an ultra-large field of view and improved imaging resolution. Remarkably, the corresponding number of resolution cells can exceed the performance of quantum ghost imaging with conventional bulky crystals by over four orders of magnitude. The demonstrated concept can be extended to multi-wavelength operation and other applications such as quantum object tracking, paving the way for advancements in quantum technologies using ultra-compact nanostructured metasurfaces.