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Quantum Imaging and Polarimetry with Structured Photonic Systems

Jinliang Ren

Published Jan 1, 2026• 0 citations
Publisher

Abstract

Quantum-enhanced optical sensing leverages correlations and entanglement in multiphoton states to surpass the limitations of classical measurement. However, the widespread deployment of quantum imaging and polarimetry has been hindered by bulky nonlinear crystals, alignment-sensitive free-space optics, and limited control over the spatial and polarization structure of quantum light. This thesis investigates how engineered nanophotonic metasurfaces, together with two-photon probing schemes, can overcome these constraints and enable compact, versatile, and high-performance quantum sensing platforms. The first component of the thesis introduces a metasurface-enabled quantum imaging system based on spatially entangled photon pairs generated from a subwavelength-thick lithium niobate (LiNbO3) nonlinear metasurface. Exploiting nonlocal guided-mode resonances with strong angular dispersion, the system realizes a hybrid imaging protocol that combines quantum ghost imaging with all-optical wavelength-controlled scanning. A theoretical framework linking momentum-space biphoton correlations to image formation is developed, including the effects of pump-beam waist and metasurface quality factor. Numerical simulations and proof-of-principle experiments demonstrate 2D imaging with strong contrast and establish that metasurface-based photon-pair sources can achieve fields of view and resolution-cell counts far beyond what is possible with bulk-crystal SPDC. Building on this platform, the thesis presents the first quantum phase imaging system that integrates metasurfaces for both photon-pair generation and phase-gradient detection. A silicon (Si) metasurface with a near-linear optical transfer function directly maps phase gradients of transparent samples into spatial quantum correlations, eliminating the need for interferometers or long propagation paths. Experiments show that phase gradients up to 25rad/mm can be retrieved with high fidelity, and the system supports switchable operation between amplitude and phase imaging within a significantly more compact scale. The final component of the thesis develops a two-photon probing quantum polarimetry (TPQP) protocol for characterizing scattering media. By combining Monte Carlo modeling of microscopic photon trajectories with Mueller-matrix decomposition and quantum state tomography, the framework links entanglement degradation to macroscopic polarization observables and resolves ambiguities in Mueller-matrix extraction through tailored probe states. Experiments using tissue-mimicking phantoms confirm that TPQP exhibits significantly higher sensitivity to depolarization than one-photon probing, validating its potential for quantum-enhanced polarimetric sensing and imaging. Overall, this thesis advances quantum optical sensing through two distinct but complementary directions. The first two parts demonstrate how engineered metasurfaces enable compact quantum imaging and phase-gradient detection by integrating photon-pair generation and spatial processing within ultrathin nanophotonic structures. Independently, the two-photon probing quantum polarimetry framework, implemented using a conventional BBO-based entangled source, shows how nonlinear two-photon correlations can enhance sensitivity to depolarization and improve Mueller-matrix reconstruction in scattering media. Although realized on different physical platforms, all components of this work exploit quantum correlations to extract amplitude, phase, and polarization information beyond classical approaches, contributing to the development of practical quantum sensing methodologies.

DOI
10.25911/9gcd-y958

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Quantum-enhanced optical sensing leverages correlations and entanglement in multiphoton states to surpass the limitations of classical measurement. However, the widespread deployment of quantum imaging and polarimetry has been hindered by bulky nonlinear crystals, alignment-sensitive free-space optics, and limited control over the spatial and polarization structure of quantum light. This thesis investigates how engineered nanophotonic metasurfaces, together with two-photon probing schemes, can overcome these constraints and enable compact, versatile, and high-performance quantum sensing platforms. The first component of the thesis introduces a metasurface-enabled quantum imaging system based on spatially entangled photon pairs generated from a subwavelength-thick lithium niobate (LiNbO3) nonlinear metasurface. Exploiting nonlocal guided-mode resonances with strong angular dispersion, the system realizes a hybrid imaging protocol that combines quantum ghost imaging with all-optical wavelength-controlled scanning. A theoretical framework linking momentum-space biphoton correlations to image formation is developed, including the effects of pump-beam waist and metasurface quality factor. Numerical simulations and proof-of-principle experiments demonstrate 2D imaging with strong contrast and establish that metasurface-based photon-pair sources can achieve fields of view and resolution-cell counts far beyond what is possible with bulk-crystal SPDC. Building on this platform, the thesis presents the first quantum phase imaging system that integrates metasurfaces for both photon-pair generation and phase-gradient detection. A silicon (Si) metasurface with a near-linear optical transfer function directly maps phase gradients of transparent samples into spatial quantum correlations, eliminating the need for interferometers or long propagation paths. Experiments show that phase gradients up to 25rad/mm can be retrieved with high fidelity, and the system supports switchable operation between amplitude and phase imaging within a significantly more compact scale. The final component of the thesis develops a two-photon probing quantum polarimetry (TPQP) protocol for characterizing scattering media. By combining Monte Carlo modeling of microscopic photon trajectories with Mueller-matrix decomposition and quantum state tomography, the framework links entanglement degradation to macroscopic polarization observables and resolves ambiguities in Mueller-matrix extraction through tailored probe states. Experiments using tissue-mimicking phantoms confirm that TPQP exhibits significantly higher sensitivity to depolarization than one-photon probing, validating its potential for quantum-enhanced polarimetric sensing and imaging. Overall, this thesis advances quantum optical sensing through two distinct but complementary directions. The first two parts demonstrate how engineered metasurfaces enable compact quantum imaging and phase-gradient detection by integrating photon-pair generation and spatial processing within ultrathin nanophotonic structures. Independently, the two-photon probing quantum polarimetry framework, implemented using a conventional BBO-based entangled source, shows how nonlinear two-photon correlations can enhance sensitivity to depolarization and improve Mueller-matrix reconstruction in scattering media. Although realized on different physical platforms, all components of this work exploit quantum correlations to extract amplitude, phase, and polarization information beyond classical approaches, contributing to the development of practical quantum sensing methodologies.
Abstract Nonlinear metasurfaces with subwavelength thickness were recently established as versatile platforms for the enhanced and tailorable generation of entangled photon pairs. The small dimensions and inherent stability of integrated metasurface sources are attractive for free-space applications in quantum communications, sensing, and imaging, yet this remarkable potential remained unexplored. Here, we formulate and experimentally demonstrate the unique benefits and practical potential of nonlinear metasurfaces for quantum imaging at infrared wavelengths, facilitating an efficient protocol combining ghost and all-optical scanning imaging. The metasurface incorporates a subwavelength-scale silica metagrating on a lithium niobate thin film. Its distinguishing feature is the capability to all-optically scan the photon emission angle in the direction across the grating simply by tuning the pump beam wavelength. Simultaneously, the photon emission is broad and anti-correlated along the grating direction, allowing for ghost imaging. Thereby, we reconstruct the images of 2D objects using just a 1D detector array in the idler path and a bucket detector in the signal path, by recording the dependencies of photon coincidences on the pump wavelength. Furthermore, we theoretically demonstrate the quantum imaging of objects with an ultra-large field of view and improved imaging resolution. Remarkably, the corresponding number of resolution cells can exceed the performance of quantum ghost imaging with conventional bulky crystals by over four orders of magnitude. The demonstrated concept can be extended to multi-wavelength operation and other applications such as quantum object tracking, paving the way for advancements in quantum technologies using ultra-compact nanostructured metasurfaces.
Quantum phase imaging enables the analysis of transparent samples with thickness and refractive index variations in scenarios requiring precise measurements under low-light conditions. Here, we present a compact quantum phase-gradient imaging system integrating a lithium niobate (LiNbO3) metasurface for generating spatially entangled photon pairs and a silicon (Si) metasurface for phase gradient extraction. By leveraging nonlocal resonances, the LiNbO3 metasurface enables efficient spontaneous parametric down-conversion (SPDC) with all-optically angularly tunable emission, while the Si metasurface provides a nearly linear optical transfer function (OTF) that differentiates the photon wavefunction and extracts phase gradients.Experimental proof-of-concept results demonstrate the imaging of up to 25~rad/mm phase gradients, achieving 89% similarity with the reference values. The pixel resolution of the system can be potentially enhanced by orders of magnitude by increasing the metasurface dimensions and resonance quality factor.Our work showcases the application of metasurfaces in both generating and detecting quantum states and establishes a new paradigm for portable quantum phase-gradient imaging, with potential applications in quantum sensing, microscopy, and LiDAR technology.
Quantum imaging leverages entanglement and photon correlations to surpass classical limits in resolution and noise performance. However, its practical deployment is constrained by bulky optical setups and limited system adaptability. Metasurfaces—ultrathin, subwavelength-structured devices—offer a compact and reconfigurable solution for wavefront control in quantum light fields. This review presents recent advances in geometric-, propagation-, and hybrid-phase metasurface designs, showcasing their contributions to enhanced spatial resolution, improved visibility, and system miniaturization across applications such as ghost imaging, quantum holography, and single-photon microscopy. It also examines key challenges—including photon loss, fabrication-induced phase noise, and the lack of dynamic tunability—while outlining future directions for developing integrated, noise-resilient, and task-specific quantum imaging platforms.
We demonstrate experimentally that a strongly enhanced generation of spatially entangled photon pairs can be achieved from metasurfaces supporting nonlocal double resonances at the signal and idler wavelengths, and reveal that multiplexed metagratings featuring different orientations allow the engineering of bi-photon polar-ization states and optically controllable generation of arbitrary polarization qutrits. Furthermore, leveraging the exceptional capabilities of the metasurface, we present a combined quantum ghost and scanning imaging protocol allowing 2D imaging with a 1D detector array.
Nonlinear optical metasurfaces, which relax the phase-matching constraints of bulk nonlinear crystals and allow for precise engineering, are opening new possibilities in the field of quantum photonics. Recent advancements have experimentally demonstrated high-resolution 2D imaging using a 1D detector array by combining quantum ghost imaging and all-optical scanning with spatially entangled photon pairs generated from a nonlinear metasurface. These findings establish metasurfaces as a promising platform for quantum imaging, communications, and sensing applications.
Quantum imaging using entangled photon pairs from spontaneous parametric down-conversion (SPDC) provides fundamental advantages over classical phase imaging in the study of transparent object, such as the operation at ultra-low photon flux and high signal-to-noise ratio [1], [2]. Metasurfaces supporting angle-dependent resonances have recently been employed to achieve phase imaging by extracting phase gradients of incident light [3]. These nanoscale metasurfaces indicate significant potential to replace bulky differential interference contrast microscopes, offering an opportunity for integration into ultra-compact biomedical devices. Together with recent development on metasurface-based quantum light source, this opens up the potential for developing a compact quantum phase imaging device, where metasurfaces serve both generation and detection functions.