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Metamaterials, Metadevices, and Metasystems

All-dielectric metasurfaces for measuring multi-photon quantum-polarization states (Conference Presentation)

Kai Wang, James Titchener, Sergey Kruk, Lei Xu, Hung-Pin Chung, Matthew Parry, Ivan I. Kravchenko, Yen-Hung Chen, Alexander S. Solntsev, Yuri S. Kivshar, Dragomir N. Neshev, Andrey A. Sukhorukov

Published Sep 17, 2018• 0 citations
Publisher

Abstract

With recent advances in nanophotonics, metasurfaces based on nano-resonators have facilitated novel types of optical devices. In particular, the interplay between different degrees of freedom, involving polarization and spatial modes, boosted classical polarization measurements and imaging applications. However, the use of metasurfaces for measuring the quantum states of light remains largely unexplored. Conventionally, the task of quantum state tomography is realized with several bulk optical elements, which need to be reconfigured multiple times. Such setups can suffer from decoherence, and there is a fundamental and practical interest in developing integrated solutions for measurement of multi-photon quantum states. We present a new concept and the first experimental realization of all-dielectric metasurfaces with no tuneable elements for imaging-based reconstruction of the full quantum state of entangled photons. Most prominently, we implement multi-photon interferometric measurements on a sub-wavelength thin optical element, which delivers ultimate miniaturization and extremely high robustness. Specifically, we realize a highly transparent all-dielectric metasurface, which spatially splits different components of quantum-polarization states. Then, a simple one-shot measurement of correlations with polarization-insensitive on-off click detectors enables complete reconstruction of multi-photon density matrices with high precision. In our experiment, we prepare sets of polarization states and reconstruct their density matrices with a high fidelity of over 99% for single photon states and above 95% for two-photon states. Our work provides a fundamental advance in the imaging of quantum states, where multi-photon quantum interference takes place at sub-wavelength scale.

DOI
10.1117/12.2320424

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With recent advances in nanophotonics, metasurfaces based on nano-resonators have facilitated novel types of optical devices. In particular, the interplay between different degrees of freedom, involving polarization and spatial modes, boosted classical polarization measurements and imaging applications. However, the use of metasurfaces for measuring the quantum states of light remains largely unexplored. Conventionally, the task of quantum state tomography is realized with several bulk optical elements, which need to be reconfigured multiple times. Such setups can suffer from decoherence, and there is a fundamental and practical interest in developing integrated solutions for measurement of multi-photon quantum states. We present a new concept and the first experimental realization of all-dielectric metasurfaces with no tuneable elements for imaging-based reconstruction of the full quantum state of entangled photons. Most prominently, we implement multi-photon interferometric measurements on a sub-wavelength thin optical element, which delivers ultimate miniaturization and extremely high robustness. Specifically, we realize a highly transparent all-dielectric metasurface, which spatially splits different components of quantum-polarization states. Then, a simple one-shot measurement of correlations with polarization-insensitive on-off click detectors enables complete reconstruction of multi-photon density matrices with high precision. In our experiment, we prepare sets of polarization states and reconstruct their density matrices with a high fidelity of over 99% for single photon states and above 95% for two-photon states. Our work provides a fundamental advance in the imaging of quantum states, where multi-photon quantum interference takes place at sub-wavelength scale.
Summary form only given. Measurements of quantum states of photons are conventionally performed with series of optical elements in bulk setups [1] or optical chips incorporating multiple tunable beam splitters. Here, we suggest and develop experimentally, for the first time to our knowledge, a new concept of quantum-polarization measurements with a single all-dielectric resonant metasurface [2]. The operating principle is presented in Fig. 1(a): A metasurface spatially splits different components of photon polarization states, which then enables full reconstruction of the photon state based on the photon correlations with simple polarization-insensitive single-photon detectors or EMCCD cameras. The subwavelength thin structure provides an ultimate miniaturization, and can facilitate quantum tomography by spatially-resolved imaging without a need for reconfiguration. Such parallel-detection approach promises not only better robustness and scalability, but also the possibility to study the dynamics of quantum states in real-time.
Metasurfaces based on resonant nanophotonic structures have enabled innovative types of flat-optics devices that often outperform the capabilities of bulk components, yet these advances remain largely unexplored for quantum applications. We show that nonclassical multiphoton interferences can be achieved at the subwavelength scale in all-dielectric metasurfaces. We simultaneously image multiple projections of quantum states with a single metasurface, enabling a robust reconstruction of amplitude, phase, coherence, and entanglement of multiphoton polarization-encoded states. One- and two-photon states are reconstructed through nonlocal photon correlation measurements with polarization-insensitive click detectors positioned after the metasurface, and the scalability to higher photon numbers is established theoretically. Our work illustrates the feasibility of ultrathin quantum metadevices for the manipulation and measurement of multiphoton quantum states, with applications in free-space quantum imaging and communications.
Characterizing the indistinguishability of photons is a key task in quantum photonics, underpinning the tuning and stabilization of the photon sources and thereby increasing the accuracy of quantum operations. The protocols for measuring the degree of indistinguishability conventionally require photon-coincidence measurements at several different time or phase delays, which is a fundamental bottleneck towards fast measurements and real-time monitoring of indistinguishability. Here, we develop a static dielectric metasurface grating without any reconfigurable elements that realizes a tailored multiport transformation in the free-space configuration without the need for phase locking and enables single-shot characterization of the indistinguishability between two photons in multiple degrees of freedom including time, spectrum, spatial modes, and polarization. Topology optimization is employed to design a silicon metasurface with polarization independence, high transmission, and high tolerance to measurement noise. We fabricate the metasurface and experimentally quantify the indistinguishability of photons in the time domain with fidelity over 98.4%. We anticipate that the developed framework based on ultrathin metasurfaces can be further extended for multi-photon states and additional degrees of freedom associated with spatial modalities.
Quantum-enhanced optical sensing leverages correlations and entanglement in multiphoton states to surpass the limitations of classical measurement. However, the widespread deployment of quantum imaging and polarimetry has been hindered by bulky nonlinear crystals, alignment-sensitive free-space optics, and limited control over the spatial and polarization structure of quantum light. This thesis investigates how engineered nanophotonic metasurfaces, together with two-photon probing schemes, can overcome these constraints and enable compact, versatile, and high-performance quantum sensing platforms. The first component of the thesis introduces a metasurface-enabled quantum imaging system based on spatially entangled photon pairs generated from a subwavelength-thick lithium niobate (LiNbO3) nonlinear metasurface. Exploiting nonlocal guided-mode resonances with strong angular dispersion, the system realizes a hybrid imaging protocol that combines quantum ghost imaging with all-optical wavelength-controlled scanning. A theoretical framework linking momentum-space biphoton correlations to image formation is developed, including the effects of pump-beam waist and metasurface quality factor. Numerical simulations and proof-of-principle experiments demonstrate 2D imaging with strong contrast and establish that metasurface-based photon-pair sources can achieve fields of view and resolution-cell counts far beyond what is possible with bulk-crystal SPDC. Building on this platform, the thesis presents the first quantum phase imaging system that integrates metasurfaces for both photon-pair generation and phase-gradient detection. A silicon (Si) metasurface with a near-linear optical transfer function directly maps phase gradients of transparent samples into spatial quantum correlations, eliminating the need for interferometers or long propagation paths. Experiments show that phase gradients up to 25rad/mm can be retrieved with high fidelity, and the system supports switchable operation between amplitude and phase imaging within a significantly more compact scale. The final component of the thesis develops a two-photon probing quantum polarimetry (TPQP) protocol for characterizing scattering media. By combining Monte Carlo modeling of microscopic photon trajectories with Mueller-matrix decomposition and quantum state tomography, the framework links entanglement degradation to macroscopic polarization observables and resolves ambiguities in Mueller-matrix extraction through tailored probe states. Experiments using tissue-mimicking phantoms confirm that TPQP exhibits significantly higher sensitivity to depolarization than one-photon probing, validating its potential for quantum-enhanced polarimetric sensing and imaging. Overall, this thesis advances quantum optical sensing through two distinct but complementary directions. The first two parts demonstrate how engineered metasurfaces enable compact quantum imaging and phase-gradient detection by integrating photon-pair generation and spatial processing within ultrathin nanophotonic structures. Independently, the two-photon probing quantum polarimetry framework, implemented using a conventional BBO-based entangled source, shows how nonlinear two-photon correlations can enhance sensitivity to depolarization and improve Mueller-matrix reconstruction in scattering media. Although realized on different physical platforms, all components of this work exploit quantum correlations to extract amplitude, phase, and polarization information beyond classical approaches, contributing to the development of practical quantum sensing methodologies.
Twisted photons can in principle carry a discrete unbounded amount of orbital angular momentum (OAM), which are of great significance for quantum communication and fundamental tests of quantum theory. However, the methods for characterization of the OAM quantum states present a fundamental limit for miniaturization. Metasurfaces can exploit new degrees of freedom to manipulate optical fields beyond the capabilities of bulk optics, opening a broad range of novel and superior applications in quantum photonics. Here we present a scheme to reconstruct the density matrix of the OAM quantum states of single photons with all-dielectric metasurfaces composed of birefringent meta-atoms. We have also measured the Schmidt number of the OAM entanglement by the multiplexing of multiple degrees of freedom. Our work represents a step toward the practical application of quantum metadevices for the measurement of OAM quantum states in free-space quantum imaging and communications.