Trapped ion systems are at the forefront of the development of various forms of quantum technology. Continuing to improve and establish new devices and techniques for the control of trapped ions is a vital element of ongoing research. In this thesis, a range of experiments which aim to expand the quantum toolkit of trapped ion systems are presented. These results primarily focus on the control and detection of bound motional states of a single trapped 88Sr+ ion for the purposes of quantum simulation and computation. We demonstrate how the interference between motional modes can reveal an interesting new interpretation of the mechanism behind light-matter interaction and introduce two separate techniques for the detection of motional states, based on the Autler-Townes effect and the use of composite pulses respectively. Additionally, we introduce a novel method to perform micromotion compensation and build upon previous works studying the effects of trapping electric fields on a single trapped Rydberg ion, observing the second-order quadrupolar response of the ion with a highly precise sensitivity.
Trapped ion systems are at the forefront of the development of various forms of quantum technology. Continuing to improve and establish new devices and techniques for the control of trapped ions is a vital element of ongoing research. In this thesis, a range of experiments which aim to expand the quantum toolkit of trapped ion systems are presented. These results primarily focus on the control and detection of bound motional states of a single trapped 88Sr+ ion for the purposes of quantum simulation and computation. We demonstrate how the interference between motional modes can reveal an interesting new interpretation of the mechanism behind light-matter interaction and introduce two separate techniques for the detection of motional states, based on the Autler-Townes effect and the use of composite pulses respectively. Additionally, we introduce a novel method to perform micromotion compensation and build upon previous works studying the effects of trapping electric fields on a single trapped Rydberg ion, observing the second-order quadrupolar response of the ion with a highly precise sensitivity.
Trapped ions are one of the leading platforms for quantum technologies due to their excellent control over their internal electronic and external motional degrees of freedom. Many techniques and interesting effects rely on the coupling of the ions to their motion, which makes precise control of them paramount. In this work, two novel techniques for motional state detection are presented. They allow the probing of certain motional states with a single measurement, without affecting the motion of the measured ion. These techniques are employed to generate and detect a highly entangled state between two motional modes in a novel manner. Furthermore, we harness the rich and intricate dynamics arising from the coupling of the ion's motion to its electronic degrees of freedom to study the emergence of interference. Theoretical predictions, describing interference both in the quantum and the classical regimes, are verified, offering a new and more intuitive description of interference, not just for trapped ions, but for a variety of systems that can be described in a similar way. On the other hand, Rydberg excitation with trapped ions enables new interaction mechanisms and makes them extremely sensitive to their surroundings. This thesis presents advances towards Rydberg experiments with longer ion strings and concludes with a first demonstration of coherent population transfer between Rydberg states in trapped ions. The methods developed significantly increase the toolbox for trapped Rydberg ions, enabling more sophisticated experiments, especially when multiple different Rydberg states are involved, and allow more flexibility when using longer ion strings.
Interference underpins some of the most practical and impactful properties of both the classical and quantum worlds. In this work we experimentally investigate a new formalism to describe interference effects, based on collective states which have enhanced or suppressed coupling to a two-level system. We employ a single trapped ion, whose electronic state is coupled to two of the ion's motional modes in order to simulate a multi-mode light-matter interaction. We observe the emergence of phononic bright and dark states for both a single phonon and a superposition of coherent states and demonstrate that a view of interference which is based solely on their decomposition in the collective basis is able to intuitively describe their coupling to a single atom. This work also marks the first time that multi-mode bright and dark states have been formed with the bounded motion of a single trapped ion and we highlight the potential of the methods discussed here for use in quantum information processing.
Since the dawn of quantum information science, laser-cooled trapped atomic ions have been one of the most compelling systems for the physical realization of a quantum computer. By applying qubit state dependent forces to the ions, their collective motional modes can be used as a bus to realize entangling quantum gates. Ultrafast state-dependent kicks [1] can provide a universal set of quantum logic operations, in conjunction with ultrafast single qubit rotations [2], which uses only ultrafast laser pulses. This may present a clearer route to scaling a trapped ion processor [3]. In addition to the role that spin-dependent kicks (SDKs) play in quantum computation, their utility in fundamental quantum mechanics research is also apparent. In this thesis, we present a set of experiments which demonstrate some of the principle properties of SDKs including ion motion independence (we demonstrate single ion thermometry from the ground state to near room temperature and the largest Schrodinger cat state ever created in an oscillator), high speed operations (compared with conventional atom-laser interactions), and multi-qubit entanglement operations with speed that is not fundamentally limited by the trap oscillation frequency. We also present a method to provide higher stability in the radial mode ion oscillation frequencies of a linear radiofrequency (rf) Paul trap--a crucial factor when performing operations on the rf-sensitive modes. Finally, we present the highest atomic position sensitivity measurement of an isolated atom to date of ~0.5 nm Hz^(-1/2) with a minimum uncertainty of 1.7 nm using a 0.6 numerical aperature (NA) lens system, along with a method to correct aberrations and a direct position measurement of ion micromotion (the inherent oscillations of an ion trapped in an oscillating rf field). This development could be used to directly image atom motion in the quantum regime, along with sensing forces at the yoctonewton [10^(-24) N)] scale for gravity sensing, and 3D imaging of atoms from static to higher frequency motion. These ultrafast atomic qubit manipulation tools demonstrate inherent advantages over conventional techniques, offering a fundamentally distinct regime of control and speed not previously achievable.
A trapped-ion harmonic oscillator represents a rich and well-controlled platform for tests of quantum physics, with applications to quantum simulations, quantum sensing, and quantum information processing. Owing to its net charge, the ion's motion is affected by changes in the electric potential. Consequently, electric field and potential curvature noise will limit the coherence of the ion's harmonic oscillation. While in some respects, this serves as a limitation in the performance of the trapped ion system (for example, in the fidelity of two-qubit gates or quantum simulations with motional quanta), it also opens an opportunity to use the ion as a precise field sensor and to use engineered quantum states of motion to enhance the sensitivity to these fields beyond the standard quantum limit (SQL). This thesis describes the implementation of such applications on a single beryllium ion confined in a Paul trap. In the thesis, I present the theory of an ideal harmonic oscillator and the implementation of this system using the motion of a single trapped ion, including producing special quantum states of motion; these states include the energy eigenstates of the harmonic oscillator, called number states, up to n=100, superpositions of number states of the form (1/√2)(|0> + |n>), with n up to 18, and coherently displaced number states with an average occupation up to approximately 300. I describe how we use these quantum states of motion for precise sensing of fluctuations of the harmonic oscillator frequency. The sensitivity of the (1/√2)(|0> + |n>) state ideally follows the 1/n Heisenberg scaling for frequency sensitivity. Additionally, I describe investigations of the spectrum of motional frequency noise using a series of coherent displacements of the motion of the ion, with features similar to Ramsey and dynamical decoupling sequences for two-level systems. While these displaced states don't improve sensitivity over the SQL, they can be simply and rapidly implemented with trapped ions. I discuss extensions to all of these experiments, including to multiple ions in a new trap designed to confine 3 or 4 ions in individually tunable potential wells.
Achieving control over physical systems down to individual quanta is central for advancing our understanding of nature and enabling emerging quantum technologies. Trapped-ion systems provide a powerful platform offering exceptional control over internal and external degrees of freedom and allowing the study of both fundamental and applied aspects of quantum dynamics. This thesis introduces an experimental toolbox, centered on problem-tailored modifications of Ramsey interferometry, for observing and manipulating dynamic processes with high temporal and spatial resolution, showcased in a trapped-ion quantum simulator. Using this versatile approach, we bridge quantum metrology and quantum thermodynamics – from tracking the motional wave packet evolution of a single ion in phase space to observing time-(in)dependent energy-level renormalizations in ultra-strongly coupled open systems. A central innovation of this thesis is the development of a stroboscopic measurement technique that establishes and maintains coherence among four oscillators: a global microwave reference, an ultraviolet polarization-gradient traveling-wave light field, and the spin and motional states of a single trapped ion. This architecture, spanning a phase-stable frequency range of more than nine orders of magnitude, enables superresolved, back-action-free tracking of motional wave packets in phase-space. In this way, we achieve noise floors of 1.8(2) nm for position and 8(2) zN μs for momentum on sub-100-nanosecond timescales. This precision enables quantum-enhanced diagnostics, non-classical state preparation, and fine-grained phase-space control, with broad implications for entanglement generation, quantum interferometry, and quantum sensing. In a complementary study, we exploit the trapped-ion system as a testbed for probing fundamental quantum interactions: We experimentally simulate a strongly coupled open quantum system, where dressed electronic states represent the system and a single motional mode serves as its environment. We observe time-dependent energy shifts up to 15% of the bare transition frequency, induced solely by ultra-strong system-environment coupling. These shifts, anticipated to be a general feature of all quantum platforms across all coupling regimes, are accurately described by the minimal-dissipation ansatz and interpreted as generalized, time-resolved Lamb shifts. Together, the results of this thesis extend the frontier of trapped-ion quantum simulation: The integration of Ramsey interferometry, stroboscopic techniques, and strong-coupling simulations offers a high-resolution window into diverse aspects of quantum dynamics. This work enables advanced studies – including squeezed states, analogues of relativistic effects such as Hawking radiation and the physics of the early universe, and autonomous quantum engines.
Trapped ions are a powerful and flexible platform used for scientific applications ranging from studies of fundamental physics and precision spectroscopy to quantum simulation and quantum information processing. These applications are enabled by the excellent control that can be exerted over the long-lived atomic states of trapped ions using electromagnetic fields. In crystals containing multiple ions, the shared motion is used as a mediator to couple the atomic states of distant ions. This thesis focuses on improving the control over ion motion, and in particular for crystals that contain multiple ion species. The first set of experiments discussed in this thesis is the application of a ground-state cooling method known as electromagnetically-induced-transparency (EIT) cooling to 25Mg+. This ion has a complex hyperfine structure which enables the implementation of a long-lived qubit. By demonstrating EIT cooling on 25Mg+, it is shown that such qubit ions are also compatible with this resource-efficient sub-Doppler cooling method. The normal modes of trapped-ion motion are well-described by quantum harmonic oscillators, and the second set of experiments described in this thesis covers the direct, rapid, and parametric coupling between two harmonic oscillators in the motion modes of multi-ion crystals. This coupling can be used to indirectly cool ion modes that are otherwise difficult or inefficient to cool. It can also be used to perform mid-circuit non-destructive readout of trapped-ion motion, which is useful for the study of states encoded in the ion motion, such as those used for bosonic error correction.