A trapped-ion harmonic oscillator represents a rich and well-controlled platform for tests of quantum physics, with applications to quantum simulations, quantum sensing, and quantum information processing. Owing to its net charge, the ion's motion is affected by changes in the electric potential. Consequently, electric field and potential curvature noise will limit the coherence of the ion's harmonic oscillation. While in some respects, this serves as a limitation in the performance of the trapped ion system (for example, in the fidelity of two-qubit gates or quantum simulations with motional quanta), it also opens an opportunity to use the ion as a precise field sensor and to use engineered quantum states of motion to enhance the sensitivity to these fields beyond the standard quantum limit (SQL). This thesis describes the implementation of such applications on a single beryllium ion confined in a Paul trap. In the thesis, I present the theory of an ideal harmonic oscillator and the implementation of this system using the motion of a single trapped ion, including producing special quantum states of motion; these states include the energy eigenstates of the harmonic oscillator, called number states, up to n=100, superpositions of number states of the form (1/√2)(|0> + |n>), with n up to 18, and coherently displaced number states with an average occupation up to approximately 300. I describe how we use these quantum states of motion for precise sensing of fluctuations of the harmonic oscillator frequency. The sensitivity of the (1/√2)(|0> + |n>) state ideally follows the 1/n Heisenberg scaling for frequency sensitivity. Additionally, I describe investigations of the spectrum of motional frequency noise using a series of coherent displacements of the motion of the ion, with features similar to Ramsey and dynamical decoupling sequences for two-level systems. While these displaced states don't improve sensitivity over the SQL, they can be simply and rapidly implemented with trapped ions. I discuss extensions to all of these experiments, including to multiple ions in a new trap designed to confine 3 or 4 ions in individually tunable potential wells.
A trapped-ion harmonic oscillator represents a rich and well-controlled platform for tests of quantum physics, with applications to quantum simulations, quantum sensing, and quantum information processing. Owing to its net charge, the ion's motion is affected by changes in the electric potential. Consequently, electric field and potential curvature noise will limit the coherence of the ion's harmonic oscillation. While in some respects, this serves as a limitation in the performance of the trapped ion system (for example, in the fidelity of two-qubit gates or quantum simulations with motional quanta), it also opens an opportunity to use the ion as a precise field sensor and to use engineered quantum states of motion to enhance the sensitivity to these fields beyond the standard quantum limit (SQL). This thesis describes the implementation of such applications on a single beryllium ion confined in a Paul trap. In the thesis, I present the theory of an ideal harmonic oscillator and the implementation of this system using the motion of a single trapped ion, including producing special quantum states of motion; these states include the energy eigenstates of the harmonic oscillator, called number states, up to n=100, superpositions of number states of the form (1/√2)(|0> + |n>), with n up to 18, and coherently displaced number states with an average occupation up to approximately 300. I describe how we use these quantum states of motion for precise sensing of fluctuations of the harmonic oscillator frequency. The sensitivity of the (1/√2)(|0> + |n>) state ideally follows the 1/n Heisenberg scaling for frequency sensitivity. Additionally, I describe investigations of the spectrum of motional frequency noise using a series of coherent displacements of the motion of the ion, with features similar to Ramsey and dynamical decoupling sequences for two-level systems. While these displaced states don't improve sensitivity over the SQL, they can be simply and rapidly implemented with trapped ions. I discuss extensions to all of these experiments, including to multiple ions in a new trap designed to confine 3 or 4 ions in individually tunable potential wells.
Quantum noise is a fundamental limitation for quantum sensors and results in the so-called shot-noise limit. Nowadays, several systems such as optical clocks or gravitational wave detectors approach measurement sensitivities where this limitation poses a major contribution to the total statistical uncertainty. It is known that this limit can be overcome by preparing the probe in a non-classical state. We will give an overview over the different non-classical states that have been implemented in the motion of single trapped ions and discuss their individual advantages and limitations in metrology. Possible applications for the presented experiments are the measurement of small oscillating electric fields and trapping frequencies. The Focus will be on our experimental work on Fock states, where quantum-enhanced sensing in both scenarios is possible with the same quantum state.
Coherently displaced number states of a harmonically bound ion can be coupled to two internal states of the ion by a laser-induced motional sideband interaction. The internal states can subsequently be read out in a projective measurement via state-dependent fluorescence, with near-unit fidelity. This leads to a rich set of line shapes when recording the internal-state excitation probability after a sideband excitation, as a function of the frequency detuning of the displacement drive with respect to the ion's motional frequency. We precisely characterize the coherent displacement based on the resulting line shapes, which exhibit sharp features that are useful for oscillator frequency determination from the single quantum regime up to very large coherent states with average occupation numbers of several hundred. We also introduce a technique based on multiple coherent displacements and free precession for characterizing noise on the trapping potential in the frequency range of 500 Hz–400 kHz. Signals from the ion are directly used to find and eliminate sources of technical noise in this typically unaccessed part of the spectrum.
Trapped ions are a powerful and flexible platform used for scientific applications ranging from studies of fundamental physics and precision spectroscopy to quantum simulation and quantum information processing. These applications are enabled by the excellent control that can be exerted over the long-lived atomic states of trapped ions using electromagnetic fields. In crystals containing multiple ions, the shared motion is used as a mediator to couple the atomic states of distant ions. This thesis focuses on improving the control over ion motion, and in particular for crystals that contain multiple ion species. The first set of experiments discussed in this thesis is the application of a ground-state cooling method known as electromagnetically-induced-transparency (EIT) cooling to 25Mg+. This ion has a complex hyperfine structure which enables the implementation of a long-lived qubit. By demonstrating EIT cooling on 25Mg+, it is shown that such qubit ions are also compatible with this resource-efficient sub-Doppler cooling method. The normal modes of trapped-ion motion are well-described by quantum harmonic oscillators, and the second set of experiments described in this thesis covers the direct, rapid, and parametric coupling between two harmonic oscillators in the motion modes of multi-ion crystals. This coupling can be used to indirectly cool ion modes that are otherwise difficult or inefficient to cool. It can also be used to perform mid-circuit non-destructive readout of trapped-ion motion, which is useful for the study of states encoded in the ion motion, such as those used for bosonic error correction.
Abstract Coupled harmonic oscillators are ubiquitous in physics and play a prominent role in quantum science. They are a cornerstone of quantum mechanics and quantum field theory, where second quantization relies on harmonic oscillator operators to create and annihilate particles. Descriptions of quantum tunneling, beamsplitters, coupled potential wells, ``hopping terms'', decoherence, and many other phenomena rely on coupled harmonic oscillators. However, the ability to couple separate quantum harmonic oscillators directly, with coupling rates that substantially exceed decoherence rates, has remained elusive. Here, we realize high-fidelity coherent exchange of single motional quanta between harmonic oscillators -- in this case, spectrally separated harmonic modes of motion of a trapped ion crystal -- where the timing, strength, and phase of the coupling are controlled through an oscillating electric potential with suitable spatial variation. The coupling rate can be made much larger than the decoherence rates, enabling demonstrations of high-fidelity quantum state transfer, entanglement of motional modes, and Hong-Ou-Mandel-type interference. We also project a harmonic oscillator into its ground state by measurement and preserve that state during repetitions of the projective measurement, an important prerequisite for non-destructive syndrome measurement in continuous-variable quantum error correction. Controllable coupling between harmonic oscillators has potential applications in quantum information processing with continuous variables, quantum simulation, and precision measurements. It can also enable cooling and quantum logic spectroscopy involving motional modes of trapped ions that are not directly accessible.
Achieving control over physical systems down to individual quanta is central for advancing our understanding of nature and enabling emerging quantum technologies. Trapped-ion systems provide a powerful platform offering exceptional control over internal and external degrees of freedom and allowing the study of both fundamental and applied aspects of quantum dynamics. This thesis introduces an experimental toolbox, centered on problem-tailored modifications of Ramsey interferometry, for observing and manipulating dynamic processes with high temporal and spatial resolution, showcased in a trapped-ion quantum simulator. Using this versatile approach, we bridge quantum metrology and quantum thermodynamics – from tracking the motional wave packet evolution of a single ion in phase space to observing time-(in)dependent energy-level renormalizations in ultra-strongly coupled open systems. A central innovation of this thesis is the development of a stroboscopic measurement technique that establishes and maintains coherence among four oscillators: a global microwave reference, an ultraviolet polarization-gradient traveling-wave light field, and the spin and motional states of a single trapped ion. This architecture, spanning a phase-stable frequency range of more than nine orders of magnitude, enables superresolved, back-action-free tracking of motional wave packets in phase-space. In this way, we achieve noise floors of 1.8(2) nm for position and 8(2) zN μs for momentum on sub-100-nanosecond timescales. This precision enables quantum-enhanced diagnostics, non-classical state preparation, and fine-grained phase-space control, with broad implications for entanglement generation, quantum interferometry, and quantum sensing. In a complementary study, we exploit the trapped-ion system as a testbed for probing fundamental quantum interactions: We experimentally simulate a strongly coupled open quantum system, where dressed electronic states represent the system and a single motional mode serves as its environment. We observe time-dependent energy shifts up to 15% of the bare transition frequency, induced solely by ultra-strong system-environment coupling. These shifts, anticipated to be a general feature of all quantum platforms across all coupling regimes, are accurately described by the minimal-dissipation ansatz and interpreted as generalized, time-resolved Lamb shifts. Together, the results of this thesis extend the frontier of trapped-ion quantum simulation: The integration of Ramsey interferometry, stroboscopic techniques, and strong-coupling simulations offers a high-resolution window into diverse aspects of quantum dynamics. This work enables advanced studies – including squeezed states, analogues of relativistic effects such as Hawking radiation and the physics of the early universe, and autonomous quantum engines.
We investigate high frequency motional states of trapped atomic ions. Trapped ions in rf traps are confined by an approximate harmonic potential and exhibit quantum motional states that mediate essential techniques in quantum computing, simulation, networking, and precision measurement. However, motional state decoherence mechanisms, heating and dephasing, are broadly limiting: reduced two-qubit gate fidelities; lower fidelity and lifetime of highly nonclassical bosonic states; long laser cooling times; and large recoil heating rates. These also challenge the scalability of increasingly sophisticated protocols. We propose high motional frequency ion trapping as an operating regime that addresses these challenges and reshapes the design landscape for quantum information experiments and quantum control techniques. We report an experimentally motivated investigation of realizing this high-frequency regime and discuss the consequences for laser cooling, motional state coherence, fidelity and lifetime of nonclassical bosonic states, and scalability of experimental runtimes. We report clear design trajectories for ion traps to reach high motional frequency, a new limiting mechanism for laser cooling at these high frequencies, and more than an order-of-magnitude speedup in experimental duty cycles with larger speed ups possible for quantum error correction protocols. Taken together, high motional frequency ion trapping has broad implications for the future of quantum information experiments.