Trapped ions are a powerful and flexible platform used for scientific applications ranging from studies of fundamental physics and precision spectroscopy to quantum simulation and quantum information processing. These applications are enabled by the excellent control that can be exerted over the long-lived atomic states of trapped ions using electromagnetic fields. In crystals containing multiple ions, the shared motion is used as a mediator to couple the atomic states of distant ions. This thesis focuses on improving the control over ion motion, and in particular for crystals that contain multiple ion species. The first set of experiments discussed in this thesis is the application of a ground-state cooling method known as electromagnetically-induced-transparency (EIT) cooling to 25Mg+. This ion has a complex hyperfine structure which enables the implementation of a long-lived qubit. By demonstrating EIT cooling on 25Mg+, it is shown that such qubit ions are also compatible with this resource-efficient sub-Doppler cooling method. The normal modes of trapped-ion motion are well-described by quantum harmonic oscillators, and the second set of experiments described in this thesis covers the direct, rapid, and parametric coupling between two harmonic oscillators in the motion modes of multi-ion crystals. This coupling can be used to indirectly cool ion modes that are otherwise difficult or inefficient to cool. It can also be used to perform mid-circuit non-destructive readout of trapped-ion motion, which is useful for the study of states encoded in the ion motion, such as those used for bosonic error correction.
Trapped ions are a powerful and flexible platform used for scientific applications ranging from studies of fundamental physics and precision spectroscopy to quantum simulation and quantum information processing. These applications are enabled by the excellent control that can be exerted over the long-lived atomic states of trapped ions using electromagnetic fields. In crystals containing multiple ions, the shared motion is used as a mediator to couple the atomic states of distant ions. This thesis focuses on improving the control over ion motion, and in particular for crystals that contain multiple ion species. The first set of experiments discussed in this thesis is the application of a ground-state cooling method known as electromagnetically-induced-transparency (EIT) cooling to 25Mg+. This ion has a complex hyperfine structure which enables the implementation of a long-lived qubit. By demonstrating EIT cooling on 25Mg+, it is shown that such qubit ions are also compatible with this resource-efficient sub-Doppler cooling method. The normal modes of trapped-ion motion are well-described by quantum harmonic oscillators, and the second set of experiments described in this thesis covers the direct, rapid, and parametric coupling between two harmonic oscillators in the motion modes of multi-ion crystals. This coupling can be used to indirectly cool ion modes that are otherwise difficult or inefficient to cool. It can also be used to perform mid-circuit non-destructive readout of trapped-ion motion, which is useful for the study of states encoded in the ion motion, such as those used for bosonic error correction.
Cooling the motion of trapped ions to near the quantum ground state is crucial for many applications in quantum information processing and quantum metrology. However, certain motional modes of trapped-ion crystals can be difficult to cool due to weak or zero interaction between the modes and the cooling radiation, typically laser beams. We overcome this challenge by coupling a mode with weak cooling radiation interaction to one with strong cooling radiation interaction using parametric modulation of the trapping potential, thereby enabling indirect cooling of the former. In this way, we demonstrate near-ground-state cooling of motional modes with weak or zero cooling radiation interaction in multi-ion crystals of the same and mixed ion species, specifically 9Be+-9Be+, 9Be+-25Mg+, and 9Be+-25Mg+-9Be+ crystals. This approach can be generally applied to any Coulomb crystal where certain motional modes cannot be directly cooled efficiently, including crystals containing molecular ions, highly-charged ions, charged fundamental particles, or charged macroscopic objects.
Cooling the motion of trapped ions to near the quantum ground state is crucial for many applications in quantum information processing and quantum metrology. However, certain motional modes of trapped-ion crystals can be difficult to cool due to weak or zero interaction between the modes and the cooling radiation, typically laser beams. We overcome this challenge by coupling a mode that interacts weakly with cooling radiation to one that interacts strongly with cooling radiation using parametric modulation of the trapping potential, thereby enabling indirect cooling of the weakly interacting mode. In this way, we demonstrate near-ground-state cooling of motional modes with weak or zero cooling radiation interaction in multi-ion crystals of the same and mixed ion species, specifically Be + 9 − Be + 9 , Be + 9 − Mg + 25 , and Be + 9 − Mg + 25 − Be + 9 crystals. This approach can be generally applied to any Coulomb crystal where certain motional modes cannot be directly cooled efficiently, including crystals containing molecular ions, highly charged ions, charged fundamental particles, or charged macroscopic objects. Published by the American Physical Society 2024
Abstract Coupled harmonic oscillators are ubiquitous in physics and play a prominent role in quantum science. They are a cornerstone of quantum mechanics and quantum field theory, where second quantization relies on harmonic oscillator operators to create and annihilate particles. Descriptions of quantum tunneling, beamsplitters, coupled potential wells, ``hopping terms'', decoherence, and many other phenomena rely on coupled harmonic oscillators. However, the ability to couple separate quantum harmonic oscillators directly, with coupling rates that substantially exceed decoherence rates, has remained elusive. Here, we realize high-fidelity coherent exchange of single motional quanta between harmonic oscillators -- in this case, spectrally separated harmonic modes of motion of a trapped ion crystal -- where the timing, strength, and phase of the coupling are controlled through an oscillating electric potential with suitable spatial variation. The coupling rate can be made much larger than the decoherence rates, enabling demonstrations of high-fidelity quantum state transfer, entanglement of motional modes, and Hong-Ou-Mandel-type interference. We also project a harmonic oscillator into its ground state by measurement and preserve that state during repetitions of the projective measurement, an important prerequisite for non-destructive syndrome measurement in continuous-variable quantum error correction. Controllable coupling between harmonic oscillators has potential applications in quantum information processing with continuous variables, quantum simulation, and precision measurements. It can also enable cooling and quantum logic spectroscopy involving motional modes of trapped ions that are not directly accessible.
Motional modes of trapped-ion crystals in Penning traps can now be cooled to near their ground states via electromagnetically induced transparency (EIT) cooling. Numerical simulations are valuable tools for interpreting EIT cooling results and optimizing experimental protocols, but existing molecular dynamics codes are limited to the simulation of Doppler cooling. In this work, we fill this gap by implementing a semiclassical model of EIT cooling in a novel MD code. By simultaneously evolving the ions' internal quantum states and classical motion, we are able to calculate the instantaneous EIT laser forces acting on the ions. We first validate our code by comparing the single-ion cooling rate to fully quantum simulation results. Next, we analyze cooling of the drumhead modes in planar ion crystals, quantifying the effects of planar ion motion and a finite laser beam width. Finally, we demonstrate efficient EIT cooling of the axial modes in 3D ellipsoidal crystals containing up to 500 ions. Such crystals are a promising platform for future quantum sensing experiments with enhanced sensitivity. We find that the mode spectra of 3D crystals can be engineered to enable sympathetic cooling of the low-frequency E×B modes. This numerical framework provides a powerful tool for modeling sub-Doppler cooling techniques and for optimizing future quantum sensing and quantum information experiments.
Trapped ions offer a controlled and versatile platform for the simulation of spin and spin-boson quantum systems. The Coulomb interaction between ions trapped in a harmonic potential can be used to mediate interactions between effective spins in the ion chain. Generally, coherent operations on ions are performed on ground-state qubits encoded in magnetically insensitive hyperfine sublevels. In this thesis, we extend this toolbox with the aim of simultaneously manipulating both ground-state and optical qubits, with the latter encoded in metastable optically excited states. The optical qubit provides another set of coherent and dissipative operations that can be performed on the ions, opening new avenues for quantum computing and simulation. In our experiment, we use 171Yb+ and 172Yb+ ions to encode ground-state and optical qubits. We discuss the laser setup needed to address the narrow quadrupole transition from 2S1/2 →2 D3/2 of 3.02 Hz linewidth, and we describe spectroscopy techniques to study this transition in both the isotopes. We describe how the low linewidth allows resolved sideband cooling on the shared motional modes in an ion chain, enabling sympathetic cooling with one ion, 172Yb+ , while simultaneously performing coherent operations on the 171Yb+ ion. Finally, we discuss the prospects of using this tool for light-shift entangling gates, showing the flexibility of this trapped-ion system for simulating coherent as well as dissipative quantum systems.
A trapped-ion harmonic oscillator represents a rich and well-controlled platform for tests of quantum physics, with applications to quantum simulations, quantum sensing, and quantum information processing. Owing to its net charge, the ion's motion is affected by changes in the electric potential. Consequently, electric field and potential curvature noise will limit the coherence of the ion's harmonic oscillation. While in some respects, this serves as a limitation in the performance of the trapped ion system (for example, in the fidelity of two-qubit gates or quantum simulations with motional quanta), it also opens an opportunity to use the ion as a precise field sensor and to use engineered quantum states of motion to enhance the sensitivity to these fields beyond the standard quantum limit (SQL). This thesis describes the implementation of such applications on a single beryllium ion confined in a Paul trap. In the thesis, I present the theory of an ideal harmonic oscillator and the implementation of this system using the motion of a single trapped ion, including producing special quantum states of motion; these states include the energy eigenstates of the harmonic oscillator, called number states, up to n=100, superpositions of number states of the form (1/√2)(|0> + |n>), with n up to 18, and coherently displaced number states with an average occupation up to approximately 300. I describe how we use these quantum states of motion for precise sensing of fluctuations of the harmonic oscillator frequency. The sensitivity of the (1/√2)(|0> + |n>) state ideally follows the 1/n Heisenberg scaling for frequency sensitivity. Additionally, I describe investigations of the spectrum of motional frequency noise using a series of coherent displacements of the motion of the ion, with features similar to Ramsey and dynamical decoupling sequences for two-level systems. While these displaced states don't improve sensitivity over the SQL, they can be simply and rapidly implemented with trapped ions. I discuss extensions to all of these experiments, including to multiple ions in a new trap designed to confine 3 or 4 ions in individually tunable potential wells.