Achieving control over physical systems down to individual quanta is central for advancing our understanding of nature and enabling emerging quantum technologies. Trapped-ion systems provide a powerful platform offering exceptional control over internal and external degrees of freedom and allowing the study of both fundamental and applied aspects of quantum dynamics. This thesis introduces an experimental toolbox, centered on problem-tailored modifications of Ramsey interferometry, for observing and manipulating dynamic processes with high temporal and spatial resolution, showcased in a trapped-ion quantum simulator. Using this versatile approach, we bridge quantum metrology and quantum thermodynamics – from tracking the motional wave packet evolution of a single ion in phase space to observing time-(in)dependent energy-level renormalizations in ultra-strongly coupled open systems. A central innovation of this thesis is the development of a stroboscopic measurement technique that establishes and maintains coherence among four oscillators: a global microwave reference, an ultraviolet polarization-gradient traveling-wave light field, and the spin and motional states of a single trapped ion. This architecture, spanning a phase-stable frequency range of more than nine orders of magnitude, enables superresolved, back-action-free tracking of motional wave packets in phase-space. In this way, we achieve noise floors of 1.8(2) nm for position and 8(2) zN μs for momentum on sub-100-nanosecond timescales. This precision enables quantum-enhanced diagnostics, non-classical state preparation, and fine-grained phase-space control, with broad implications for entanglement generation, quantum interferometry, and quantum sensing. In a complementary study, we exploit the trapped-ion system as a testbed for probing fundamental quantum interactions: We experimentally simulate a strongly coupled open quantum system, where dressed electronic states represent the system and a single motional mode serves as its environment. We observe time-dependent energy shifts up to 15% of the bare transition frequency, induced solely by ultra-strong system-environment coupling. These shifts, anticipated to be a general feature of all quantum platforms across all coupling regimes, are accurately described by the minimal-dissipation ansatz and interpreted as generalized, time-resolved Lamb shifts. Together, the results of this thesis extend the frontier of trapped-ion quantum simulation: The integration of Ramsey interferometry, stroboscopic techniques, and strong-coupling simulations offers a high-resolution window into diverse aspects of quantum dynamics. This work enables advanced studies – including squeezed states, analogues of relativistic effects such as Hawking radiation and the physics of the early universe, and autonomous quantum engines.
Achieving control over physical systems down to individual quanta is central for advancing our understanding of nature and enabling emerging quantum technologies. Trapped-ion systems provide a powerful platform offering exceptional control over internal and external degrees of freedom and allowing the study of both fundamental and applied aspects of quantum dynamics. This thesis introduces an experimental toolbox, centered on problem-tailored modifications of Ramsey interferometry, for observing and manipulating dynamic processes with high temporal and spatial resolution, showcased in a trapped-ion quantum simulator. Using this versatile approach, we bridge quantum metrology and quantum thermodynamics – from tracking the motional wave packet evolution of a single ion in phase space to observing time-(in)dependent energy-level renormalizations in ultra-strongly coupled open systems. A central innovation of this thesis is the development of a stroboscopic measurement technique that establishes and maintains coherence among four oscillators: a global microwave reference, an ultraviolet polarization-gradient traveling-wave light field, and the spin and motional states of a single trapped ion. This architecture, spanning a phase-stable frequency range of more than nine orders of magnitude, enables superresolved, back-action-free tracking of motional wave packets in phase-space. In this way, we achieve noise floors of 1.8(2) nm for position and 8(2) zN μs for momentum on sub-100-nanosecond timescales. This precision enables quantum-enhanced diagnostics, non-classical state preparation, and fine-grained phase-space control, with broad implications for entanglement generation, quantum interferometry, and quantum sensing. In a complementary study, we exploit the trapped-ion system as a testbed for probing fundamental quantum interactions: We experimentally simulate a strongly coupled open quantum system, where dressed electronic states represent the system and a single motional mode serves as its environment. We observe time-dependent energy shifts up to 15% of the bare transition frequency, induced solely by ultra-strong system-environment coupling. These shifts, anticipated to be a general feature of all quantum platforms across all coupling regimes, are accurately described by the minimal-dissipation ansatz and interpreted as generalized, time-resolved Lamb shifts. Together, the results of this thesis extend the frontier of trapped-ion quantum simulation: The integration of Ramsey interferometry, stroboscopic techniques, and strong-coupling simulations offers a high-resolution window into diverse aspects of quantum dynamics. This work enables advanced studies – including squeezed states, analogues of relativistic effects such as Hawking radiation and the physics of the early universe, and autonomous quantum engines.
In quantum technologies, it is essential to understand and exploit the interplay of light and matter. We introduce an approach creating and maintaining the coherence of four oscillators: a global microwave reference field, a polarization-gradient traveling-wave pattern of light, and the spin and motional states of a single trapped ion. Our method employs a UV light pattern capable of achieving a gigahertz-modulation bandwidth, here demonstrated in the megahertz regime, allowing for stroboscopic tracking of dynamic changes in phase space. We achieve noise floors of 1.8(2)nm for position and $8(2)\phantom{\rule{4.pt}{0ex}}\text{zN}\phantom{\rule{0.16em}{0ex}}\phantom{\rule{0.16em}{0ex}}\textmu{}\mathrm{s}$ for momentum observables, superresolving variations on timescales $\ensuremath{\lesssim}100$ ns. The implications of our findings contribute to enhancing quantum control and metrological applications.
The fundamental laws of quantum mechanics are far from our everyday life experiences. However, they have been extremely successful in explaining observations in microscopic physical systems and are, already, harnessed for several applications. Moreover, in combination with relativistic considerations, basic phenomena from quantum mechanics are accredited a central role in the (macroscopic) evolution of our universe. In this thesis, we employ a trapped ion quantum simulator to experimentally investigate two fundamental quantum mechanical effects that have been extensively studied for many decades. In the first investigation, we implement non-adiabatic changes of the ions’ trapping potential in order to amplify quantum vacuum fluctuations. Following theoretical works by others, this mechanism can be interpreted as an analog to the creation of particles during cosmic inflation in the early universe. Such cosmological particles are considered as the seeds for the formation of the large-scale structures in our universe that we observe nowadays. In our analog quantum simulation, the creation of particles is evidenced by the detection of a squeezed state in the motion of the ions. A remarkable feature of this mechanism is the accompanying creation of quantum entanglement. In case of the cosmological particles, this entanglement spreads over large, cosmic distances. In the second investigation, we benchmark a theoretical concept in the framework of open quantum systems in a most basic system and under near-ideal conditions. In nature, any quantum system inevitably interacts with its environment and, thereby, needs ultimately to be considered an open system that can build up correlations and, even, entanglement with its environment. We implement a spin-1/2 system in the electronic degree of freedom of a single trapped ion, which we couple to a bosonic environment, formed by a motional degree of freedom of the ion. Further, we implement a tunable interaction between system and environment that, in turn, can lead to entanglement. By performing measurements on the open system only, we observe quantum non-Markovian behavior, which we quantify using a rigorously defined measure. Thereby, we reveal that the quantification of such quantum memory effects is fundamentally limited by fundamental quantum mechanical measurement uncertainties. The investigations presented in this thesis significantly expand the capabilities of our trapped ion platform to perform analog quantum simulations of fundamental quantum mechanical problems under near-ideal conditions, and enable future studies of increased complexity and under more realistic conditions.
A trapped-ion harmonic oscillator represents a rich and well-controlled platform for tests of quantum physics, with applications to quantum simulations, quantum sensing, and quantum information processing. Owing to its net charge, the ion's motion is affected by changes in the electric potential. Consequently, electric field and potential curvature noise will limit the coherence of the ion's harmonic oscillation. While in some respects, this serves as a limitation in the performance of the trapped ion system (for example, in the fidelity of two-qubit gates or quantum simulations with motional quanta), it also opens an opportunity to use the ion as a precise field sensor and to use engineered quantum states of motion to enhance the sensitivity to these fields beyond the standard quantum limit (SQL). This thesis describes the implementation of such applications on a single beryllium ion confined in a Paul trap. In the thesis, I present the theory of an ideal harmonic oscillator and the implementation of this system using the motion of a single trapped ion, including producing special quantum states of motion; these states include the energy eigenstates of the harmonic oscillator, called number states, up to n=100, superpositions of number states of the form (1/√2)(|0> + |n>), with n up to 18, and coherently displaced number states with an average occupation up to approximately 300. I describe how we use these quantum states of motion for precise sensing of fluctuations of the harmonic oscillator frequency. The sensitivity of the (1/√2)(|0> + |n>) state ideally follows the 1/n Heisenberg scaling for frequency sensitivity. Additionally, I describe investigations of the spectrum of motional frequency noise using a series of coherent displacements of the motion of the ion, with features similar to Ramsey and dynamical decoupling sequences for two-level systems. While these displaced states don't improve sensitivity over the SQL, they can be simply and rapidly implemented with trapped ions. I discuss extensions to all of these experiments, including to multiple ions in a new trap designed to confine 3 or 4 ions in individually tunable potential wells.
The outstanding degree of control over trapped ions in Paul traps gives rise to the development of novel quantum manipulation techniques. Optical transitions can be used for precise manipulation of internal and external states. This way, non-classical states can be created which are a key component of quantum algorithms based on quantum logic operations. This powerful optical toolbox enabled the trapped ion system to assume leadership in the field of quantum computation. This thesis addresses two major challenges in the field of micro ion trap quantum optics. The temperature dependence of the heating rate from the ion trap surface is analysed in a novel cryogenic micro ion trap. Furthermore segmented traps allow state manipulations by time dependent electrical potentials, generated by the control voltages. These electrical fields provide a fast and reliable control handle to the ions external degrees of freedom. Quantum computation in Paul trap arrays is based on a combination of ion crystal transport, splitting and merging operations, while laser driven quantum state manipulations are mainly carried out on small ion crystals. Within this thesis a basic building block was realised by performing transport operations with a single ground-state cooled ion. As a highlight of experimental achievements, shuttling in the non-adiabatic regime, on the timescale of the motional period was demonstrated with low residual energy transfer. For his endeavour a specialised low noise arbitrary function generator was designed and manufactured during this thesis. Arbitrary voltage ramps at a sampling rate of up to 2.5 MS/s on up to 12 channels allow the study of a novel excitation method by directly manipulating the ion using electrical forces. Accurate numerical simulations in combination with the fast high resolution voltage supply allow deterministic quantum manipulations via momentum kicks. I report the first experimental demonstration of displaced number states with trapped ions.
Trapped ions are one of the leading platforms for quantum technologies due to their excellent control over their internal electronic and external motional degrees of freedom. Many techniques and interesting effects rely on the coupling of the ions to their motion, which makes precise control of them paramount. In this work, two novel techniques for motional state detection are presented. They allow the probing of certain motional states with a single measurement, without affecting the motion of the measured ion. These techniques are employed to generate and detect a highly entangled state between two motional modes in a novel manner. Furthermore, we harness the rich and intricate dynamics arising from the coupling of the ion's motion to its electronic degrees of freedom to study the emergence of interference. Theoretical predictions, describing interference both in the quantum and the classical regimes, are verified, offering a new and more intuitive description of interference, not just for trapped ions, but for a variety of systems that can be described in a similar way. On the other hand, Rydberg excitation with trapped ions enables new interaction mechanisms and makes them extremely sensitive to their surroundings. This thesis presents advances towards Rydberg experiments with longer ion strings and concludes with a first demonstration of coherent population transfer between Rydberg states in trapped ions. The methods developed significantly increase the toolbox for trapped Rydberg ions, enabling more sophisticated experiments, especially when multiple different Rydberg states are involved, and allow more flexibility when using longer ion strings.
This thesis describes new results on the entanglement of atomic spins in Ramsey interferometry, optical atomic clocks and trapped ions. It is divided into three parts: First, we investigate improvements to conventional Ramsey interferometry with entanglement and adding only rotations of the collective spin to adjust the signal and measurement directions. The geometric degrees of freedom, connected to the rotations, are analytically optimized for a large class of generalized Ramsey protocols to allow efficient optimization of all parameters. Besides a unification of existing approaches, the main result is that there is only one new protocol, where a previously unused double inversion is applied. Studies of the local sensitivity show that this protocol reaches the fundamental quantum Fisher information limit and is yet robust against errors during preparation and measurement. In the second section we investigate the conditions under which optical atomic clocks exhibit increased long-term stability when applying weakly entangled, spin squeezed states. We discuss the common case of an atomic clock with a single ensemble, typical Brownian frequency noise and finite dead time. Theoretical modelling of the servo loop allows quantitative predictions of the optimal stability for given values of dead time and laser noise, in very good agreement with numerical simulations of the closed feedback loop. The main result is that, even with the current most stable lasers, the clock stability can only be improved for ensembles below a critical atom number of about one thousand in optical Sr lattice clocks. Even with a future improvement of the laser performance by one order of magnitude, the critical atom number still remains below 100,000. In contrast, clocks based on smaller, non-scalable ensembles, such as ion clocks, can already benefit from squeezed states with current clock lasers. Thus the last section considers the robust generation of entanglement in ion traps. An error budget including relevant experimental error sources is calculated for state-of-the-art quantum gates, driven by oscillating microwave gradients in surface traps. Amplitude modulation of the driving fields is shown to efficiently counteract the current limitations from motional mode instability. The predicted increase of the gate quality was demonstrated by the group of C. Ospelkaus at PTB Braunschweig, who measured gates with errors as low as ~ 10^(-3). In a similar approach, interactions between spin and motion can also be generated by combining oscillating rf-fields with a static magnetic field gradient. Penning traps designed for precision spectroscopy already feature large magnetic field gradients at the edge of a magnetic bottle configuration. We present parameters and conditions under which laser-free coupling of spin and quantized motion for (anti-)protons is possible at these points, in a step towards quantum logic spectroscopy for (anti-)protons.