Phononic bright and dark states: Investigating multi-mode light-matter interactions with a single trapped ion
Harry Parke, Robin Thomm, Alan C. Santos, A. Cidrim, Gerard T. Higgins, Marion Mallweger, Natalia Kuk, Shalina Salim, Romain Bachelard, Celso J. Villas-Bôas, Markus Hennrich
Interference underpins some of the most practical and impactful properties of both the classical and quantum worlds. In this work we experimentally investigate a new formalism to describe interference effects, based on collective states which have enhanced or suppressed coupling to a two-level system. We employ a single trapped ion, whose electronic state is coupled to two of the ion's motional modes in order to simulate a multi-mode light-matter interaction. We observe the emergence of phononic bright and dark states for both a single phonon and a superposition of coherent states and demonstrate that a view of interference which is based solely on their decomposition in the collective basis is able to intuitively describe their coupling to a single atom. This work also marks the first time that multi-mode bright and dark states have been formed with the bounded motion of a single trapped ion and we highlight the potential of the methods discussed here for use in quantum information processing.
Interference underpins some of the most practical and impactful properties of both the classical and quantum worlds. In this work we experimentally investigate a new formalism to describe interference effects, based on collective states which have enhanced or suppressed coupling to a two-level system. We employ a single trapped ion, whose electronic state is coupled to two of the ion's motional modes in order to simulate a multi-mode light-matter interaction. We observe the emergence of phononic bright and dark states for both a single phonon and a superposition of coherent states and demonstrate that a view of interference which is based solely on their decomposition in the collective basis is able to intuitively describe their coupling to a single atom. This work also marks the first time that multi-mode bright and dark states have been formed with the bounded motion of a single trapped ion and we highlight the potential of the methods discussed here for use in quantum information processing.
Trapped ion systems are at the forefront of the development of various forms of quantum technology. Continuing to improve and establish new devices and techniques for the control of trapped ions is a vital element of ongoing research. In this thesis, a range of experiments which aim to expand the quantum toolkit of trapped ion systems are presented. These results primarily focus on the control and detection of bound motional states of a single trapped 88Sr+ ion for the purposes of quantum simulation and computation. We demonstrate how the interference between motional modes can reveal an interesting new interpretation of the mechanism behind light-matter interaction and introduce two separate techniques for the detection of motional states, based on the Autler-Townes effect and the use of composite pulses respectively. Additionally, we introduce a novel method to perform micromotion compensation and build upon previous works studying the effects of trapping electric fields on a single trapped Rydberg ion, observing the second-order quadrupolar response of the ion with a highly precise sensitivity.
Classical theory asserts that several electromagnetic waves cannot interact with matter if they interfere destructively to zero, whereas quantum mechanics predicts a nontrivial light-matter dynamics even when the average electric field vanishes. Here, we show that in quantum optics, classical interference emerges from collective bright and dark states of light, i.e., particular cases of two-mode binomial states, which are entangled superpositions of multimode photon-number states. This makes it possible to explain wave interference using the particle description of light and the superposition principle for linear systems only. It also sheds new light on an old debate concerning the origin of complementarity.
Trapped ions are one of the leading platforms for quantum technologies due to their excellent control over their internal electronic and external motional degrees of freedom. Many techniques and interesting effects rely on the coupling of the ions to their motion, which makes precise control of them paramount. In this work, two novel techniques for motional state detection are presented. They allow the probing of certain motional states with a single measurement, without affecting the motion of the measured ion. These techniques are employed to generate and detect a highly entangled state between two motional modes in a novel manner. Furthermore, we harness the rich and intricate dynamics arising from the coupling of the ion's motion to its electronic degrees of freedom to study the emergence of interference. Theoretical predictions, describing interference both in the quantum and the classical regimes, are verified, offering a new and more intuitive description of interference, not just for trapped ions, but for a variety of systems that can be described in a similar way. On the other hand, Rydberg excitation with trapped ions enables new interaction mechanisms and makes them extremely sensitive to their surroundings. This thesis presents advances towards Rydberg experiments with longer ion strings and concludes with a first demonstration of coherent population transfer between Rydberg states in trapped ions. The methods developed significantly increase the toolbox for trapped Rydberg ions, enabling more sophisticated experiments, especially when multiple different Rydberg states are involved, and allow more flexibility when using longer ion strings.
The interaction between light and matter has captivated physicists for centuries, from early studies of vision and refraction in ancient Greece to the development of quantum mechanics and quantum electrodynamics in the past century. While the response of a single quantum emitter to light is well understood, the radiative properties of an ensemble of closely spaced emitters are far more intricate. Coupling to a shared electromagnetic environment induces coherent and dissipative interactions between emitters, giving rise to a collective response that cannot be captured by treating them independently. In the regime of few excitations, the system hosts delocalized subradiant states, that is, coherent superpositions that are largely decoupled from the electromagnetic field and thus decay at suppressed rates. While this weak coupling makes subradiant states attractive for quantum technologies, it also renders them difficult to manipulate. At higher excitation densities, the intrinsic nonlinearity of emitters and the exponential growth of the Hilbert space make theoretical and numerical descriptions of the system and its dynamics increasingly challenging. This thesis explores two fundamental questions: How can subradiant and dark states be selectively accessed and harnessed for practical applications in quantum technologies? And how can interacting ensembles of quantum emitters be efficiently simulated to uncover their many-body physics? The first part of the thesis develops protocols for controlling and addressing dark states in free-space and waveguide-coupled atomic arrays, demonstrating their utility in quantum storage and the deterministic generation of entangled photonic states. Incorporating atomic motion, we further show that collective subradiant states can enhance cooling in dense atomic arrays, offering new avenues for controlling motional dynamics. In the second part, we introduce cumulant expansions of the equations of motion as a powerful tool to analytically and numerically investigate collective decay in the many-body regime. We first examine the collective decay of fully excited atomic arrays in free space, characterizing the onset and scaling of the superradiant burst across different geometries. In collaboration with experiments on ultracold erbium atoms in optical lattices, we provide the first direct observations of many-body collective effects in free-space ordered arrays, including early-time superradiant bursts, late-time subradiant tails, and the emergence of atomic correlations throughout the dynamics. Finally, we theoretically and numerically explore the transient formation of multi-excitation subradiant states, and demonstrate how the existence of multiple dissipation channels suppresses steady-state superradiance in extended arrays.
In this article we present a comprehensive theoretical investigation of phonon lasing with mixed-species trapped ions, as demonstrated in [T. Behrle, Phys. Rev. Lett. 131 (2023)], employing both a semi-classical mean-field description and a full quantum theory. We derive an analytic expression for the second-order coherence function, confirming the experimental observation of the system's lasing behaviour above threshold. Building on the successful implementation of the two-ion lasing scheme, we propose a novel approach for achieving phonon lasing with a single trapped ion, offering significant experimental advantages and making the implementation of multiple phonon lasers within a single setup feasible. Furthermore, we explore lasing in a squeezed basis and in different regimes of the Lamb-Dicke approximation, highlighting the potential to produce non-classical states with promising applications in precision sensing. Our analysis of a sensing protocol based on squeezed states, using experimentally feasible parameters, shows a sensitivity enhancement of up to two orders of magnitude.
Trapped ions offer a pristine platform for quantum computation and simulation, but improving their coherence remains a crucial challenge. Here, we propose and analyze a new strategy to enhance the coherent interactions in trapped ion systems via parametric amplification of the ions' motion-by squeezing the collective motional modes (phonons), the spin-spin interactions they mediate can be significantly enhanced. We illustrate the power of this approach by showing how it can enhance collective spin states useful for quantum metrology, and how it can improve the speed and fidelity of two-qubit gates in multi-ion systems, important ingredients for scalable trapped ion quantum computation. Our results are also directly relevant to numerous other physical platforms in which spin interactions are mediated by bosons.