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arXiv:2604.18295

Quantum theory for phonon lasing and non-classical state generation in mixed-species and single trapped ions

David Baur, Tanja Behrle, Ivan Rojkov, Jan Jeske, Susanne Yelin, Jonathan Home, Florentin Reiter

quant-phSubmitted Apr 20, 2026• Announced Apr 21, 2026• 0 citations
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Abstract

In this article we present a comprehensive theoretical investigation of phonon lasing with mixed-species trapped ions, as demonstrated in [T. Behrle, Phys. Rev. Lett. 131 (2023)], employing both a semi-classical mean-field description and a full quantum theory. We derive an analytic expression for the second-order coherence function, confirming the experimental observation of the system's lasing behaviour above threshold. Building on the successful implementation of the two-ion lasing scheme, we propose a novel approach for achieving phonon lasing with a single trapped ion, offering significant experimental advantages and making the implementation of multiple phonon lasers within a single setup feasible. Furthermore, we explore lasing in a squeezed basis and in different regimes of the Lamb-Dicke approximation, highlighting the potential to produce non-classical states with promising applications in precision sensing. Our analysis of a sensing protocol based on squeezed states, using experimentally feasible parameters, shows a sensitivity enhancement of up to two orders of magnitude.

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15 pages, 13 figures

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In this article we present a comprehensive theoretical investigation of phonon lasing with mixed-species trapped ions, as demonstrated in [T. Behrle, Phys. Rev. Lett. 131 (2023)], employing both a semi-classical mean-field description and a full quantum theory. We derive an analytic expression for the second-order coherence function, confirming the experimental observation of the system's lasing behaviour above threshold. Building on the successful implementation of the two-ion lasing scheme, we propose a novel approach for achieving phonon lasing with a single trapped ion, offering significant experimental advantages and making the implementation of multiple phonon lasers within a single setup feasible. Furthermore, we explore lasing in a squeezed basis and in different regimes of the Lamb-Dicke approximation, highlighting the potential to produce non-classical states with promising applications in precision sensing. Our analysis of a sensing protocol based on squeezed states, using experimentally feasible parameters, shows a sensitivity enhancement of up to two orders of magnitude.
The quantum phonon laser state is a vibrational state generated by phonon coherent amplification based on quantum mechanics. Its core is coherent excitation and manipulation of phonon quantum states by controlling phonon dynamics. This technology breaks classical limits of traditional phonon lasers, offering new methods for quantum information. Previous research on quantum phonon lasers focused on quantum van der Pol oscillators. As typical nonlinear quantum systems, they show significant value in trapped-ion systems. These breakthroughs extend nonlinear dynamics into the quantum domain and provide platforms for exploring quantum nonlinear phenomena. Although realized in two-ion systems, practical applications remain challenging. This paper explores how a single trapped ion generates quantum phonon laser states using a three-level model. By solving the quantum master equation numerically, steady-state characteristics are analyzed, focusing on quantum statistics including the Wigner function and second-order correlation function. An experimental scheme is proposed based on a single trapped 40Ca+ ion, using bichromatic blue-sideband and red-sideband lasers to generate quantum phonon laser states. By introducing the characteristic function of motional states, precise quantum state tomography is achieved. Additionally, a two-level model discusses the phonon laser threshold effect. However, the three-level model shows significantly different thresholds and more accurately describes the quantum phonon laser's physical mechanisms.
We present a theoretical model for realizing squeezed lasing in a trapped-ion system without relying on engineered baths or tailored dissipative reservoirs. Our approach leverages the intrinsic ion-phonon interactions, where two trapped ions, each interacting with a shared vibrational mode, are driven on both red- and blue-sideband transitions. This enables the creation of a squeezed state of motion through the dynamic coupling between the ions' internal states and the phonon mode. Unlike traditional methods that require bath engineering, our model demonstrates that squeezed lasing can be achieved through a direct manipulation of ion-phonon interactions, with no external reservoirs required. We explore the steady-state behavior of the system, analyzing the onset of lasing, gain-loss balance, and the role of the squeezing parameter in shaping the phonon field's statistical properties. Furthermore, we show how external coherent drives can stabilize phase coherence and achieve controlled quadrature squeezing, offering a simple yet effective method for achieving squeezed lasing in quantum mechanical systems. Our findings provide new insights into the realization of squeezed states in phonon-based systems, with potential applications in quantum metrology and information processing.
Multi-photon lasing has been realized in systems with strong nonlinear interactions between emitters and cavity modes, where single-photon processes are suppressed. Coherence between the internal states of a quantum emitter, or among multiple emitters, plays a key role. Such continuous nonclassical sources of light can find applications in quantum computation, quantum sensing, quantum metrology, and quantum communication. This thesis explores the multi-photon lasing phenomena in various quantum dot-photonic crystal cavity quantum electrodynamic (QED) setups. Exciton-phonon interactions are inevitable in such systems and are incorporated using the polaron-transformed master equation. The Born-Markov approximation is employed to obtain the reduced density matrix rate equation. Using quantum laser theory, we derived the Scully-Lamb laser rate equations and evaluated the single- and multi-photon excess emission rates defined as the difference between emission and absorption rates into the cavity mode without mean-field approximations. We investigated cooperative two-photon lasing, correlated emission lasing, hyperradiant lasing, non-degenerate two-mode two-photon lasing, and continuous variable entanglement in open quantum systems with single or multiple semiconductor quantum dots (two-level, three-level, and four-level) driven coherently/incoherently and coupled to single/ bimodal cavities.
Quantum computing promises solutions to some of the world's most important problems that classical computers have failed to address. The trapped-ion-based quantum computing platform has a lot of advantages for doing so: ions are perfectly identical and near-perfectly isolated, feature long coherent times, and allow high-fidelity individual laser-controlled operations. One of the greatest remaining obstacles in trapped-ion-based quantum computing is the issue of scalability. The approach that we take to address this issue is a modular architecture: separate ion traps, each with a manageable number of ions, are interconnected via photonic links. To avoid photon-generated crosstalk between qubits and utilize advantages of different kinds of ions for each role, we use two distinct species - ¹⁷¹Yb⁺ as memory qubits and ¹³⁸Ba⁺ as communication qubits. The qubits based on ¹⁷¹Yb⁺ are defined within the hyperfine "clock" states characterized by a very long coherence time while ¹³⁸Ba⁺ ions feature visible-range wavelength emission lines. Current optical and fiber technologies are more efficient in this range than at shorter wavelengths. We present a theoretical description and experimental demonstration of the key elements of a quantum network based on the mixed-species paradigm. The first one is entanglement between an atomic qubit and the polarization degree of freedom of a pure single photon. We observe a value of the second-order correlation function g⁽²⁾(0) = (8.1 ± 2.3)⨉10⁻⁵ without background subtraction, which is consistent with the lowest reported value in any system. Next, we show mixed-species entangling gates with two ions using the Mølmer-Sørensen and Cirac-Zoller protocols. Finally, we theoretically generalize mixed-species entangling gates to long ion chains and characterize the roles of normal modes there. In addition, we explore sympathetic cooling efficiency in such mixed-species crystals. Besides these developments, we demonstrate new techniques for manipulating states within the D₃⸝₂-manifold of zero-nuclear-spin ions - a part of a protected qubit scheme promising seconds-long coherence times proposed by Aharon et al. in 2013. As a next step, we provide a detailed description of the protocols for three- and four-node networks with mixed species, along with a novel design for the third trap with in-vacuum optics to optimize light collection.
The phonon laser realized in a trapped ion, i.e., a self-sustained mechanical oscillator, has demonstrated the unique characteristics in practically detecting externally applied electric signals without the prerequisite of sideband cooling. Entering the quantum regime via sideband cooling is expected to further improve its sensing performance. Here we report the first experimental realization of a quantum-regime single-ion phonon laser (nˉ<10\bar{n}<10nˉ<10) using a trapped 40Ca+^{40}\mathrm{Ca}^+40Ca+ ion and demonstrate electrometry based on its phase-space symmetry-breaking response to weak resonant electric fields. By tuning the phonon-laser parameters, we reveal that the sensing performance is fundamentally governed by the finite-time relaxation dynamics of the underlying open quantum system. We find that a slow Liouvillian relaxation, correlated with the finite experimental interaction window, effectively enhances the dynamic susceptibility while maintaining the structural robustness of the limit cycle. This regime, when applied to the detection of electric fields, produces a shot-noise-limited peak sensitivity of 14.15±0.77 μV/m/Hz14.15 \pm 0.77~μ\mathrm{V/m}/\sqrt{\mathrm{Hz}}14.15±0.77 μV/m/Hz​ and a minimum detectable field variation of δEmin≈1.83 μV/mδE_{\mathrm{min}} \approx 1.83~μ\mathrm{V/m}δEmin​≈1.83 μV/m. Our results establish quantum phonon lasers as a practical platform for advanced sensing and highlight the central role of Liouvillian dynamics in non-equilibrium electrometry.