Measurements on states of light underpins the entire fields of classical and quantum optics. Without measurement we are unable to gain any information about the light we are studying or about the processes it has undergone. The property of the density matrix of light prior to measurement that we want to measure also relies heavily on the measurement technique we employ. We can use a single-photon detector to measure the particle nature of light--the photon--the discrete quanta of the electromagnetic field. We can conversely measure the wave nature of the light field by making phase-sensitive measurements. In this thesis, we shall explore some advanced implementations and applications of these measurement schemes. First, we shall focus on a specific type of single-photon detector: the Superconducting-Nanowire Single-Photon Detector. We will first consider the integration of these detectors on optical waveguides, and discuss their optical characterisation. Then we will consider a practical application of these detectors by investigating a method to perform broadband spectroscopy with a single detector. We shall then progress to phase-sensitive measurements, and consider the intermediate regime between measuring the wave-like and particle-like nature of light. First we will perform a fundamental investigation of the transition between both measurement regimes. We will see how varying the phase reference itself allows us to tune between both regimes. Following this we will discuss an application of this intermediate regime, by considering an experimental setup to perform state tomography with a weak phase reference. The final consideration of this thesis will be a theoretical benchmarking scheme for a practical application of quantum optics. The manipulation of certain quantum states of light followed by a photon-number measurement can have practical applications in a variety of fields, and therefore validating the results is of extreme importance. On this final topic, we will discuss an experimentally friendly technique to benchmark the output of such measurements by considering smaller subsystems, and the practical requirements of this technique.
Measurements on states of light underpins the entire fields of classical and quantum optics. Without measurement we are unable to gain any information about the light we are studying or about the processes it has undergone. The property of the density matrix of light prior to measurement that we want to measure also relies heavily on the measurement technique we employ. We can use a single-photon detector to measure the particle nature of light--the photon--the discrete quanta of the electromagnetic field. We can conversely measure the wave nature of the light field by making phase-sensitive measurements. In this thesis, we shall explore some advanced implementations and applications of these measurement schemes. First, we shall focus on a specific type of single-photon detector: the Superconducting-Nanowire Single-Photon Detector. We will first consider the integration of these detectors on optical waveguides, and discuss their optical characterisation. Then we will consider a practical application of these detectors by investigating a method to perform broadband spectroscopy with a single detector. We shall then progress to phase-sensitive measurements, and consider the intermediate regime between measuring the wave-like and particle-like nature of light. First we will perform a fundamental investigation of the transition between both measurement regimes. We will see how varying the phase reference itself allows us to tune between both regimes. Following this we will discuss an application of this intermediate regime, by considering an experimental setup to perform state tomography with a weak phase reference. The final consideration of this thesis will be a theoretical benchmarking scheme for a practical application of quantum optics. The manipulation of certain quantum states of light followed by a photon-number measurement can have practical applications in a variety of fields, and therefore validating the results is of extreme importance. On this final topic, we will discuss an experimentally friendly technique to benchmark the output of such measurements by considering smaller subsystems, and the practical requirements of this technique.
The implementation of optical quantum technologies requires precise and complete characterisation tools for multi-mode nonclassical states of light. In this thesis, we propose and we implement experimentally three applications of optical quantum measurements, which combine aspects of light that are described by both discrete and continuous variables. In the rst part of this thesis, we present a new scheme for interferometric phase estimation, which uses double homodyne measurements as an alternative to photon counting. We show that, without requiring a phase reference, this scheme can achieve the optimum phase estimation precision for all path-symmetric probe states with a de ned number of photons. Furthermore, the estimation procedure is robust against state preparation imperfections, and naturally yields the same precision for all values of the estimated phase. We implement the proposed scheme experimentally, using a polarisation interferometer probed by a single-photon signal, and temporally multiplexing a single homodyne detector. We repeat the experiment with classical probe states. For both cases, we demonstrate the accuracy and precision of the proposed method, our implementation deviating by 5% from the fundamental precision bound. We demonstrate that, in our scheme, single-photon probe states can provide better precision than weak coherent ones. These results indicate that hybrid quantum resources, which combine tools from the discrete and continuous-variable paradigms, can play a signi cant role in practical sensing scenarios. In the second part of this thesis, we present an application in the eld of information thermodynamics, reporting an experimental realisation, in a photonic setup, of Maxwell's demon. We show that a measurement at the few-photons level, followed by a feed-forward operation, allows the extraction of work from intense thermal light into an electric circuit. The interpretation of the experiment leads us to the derivation of an equality relating work extraction to information acquired by measurement. We prove a bound using this relation, and show that it is in agreement with the experimental results. Our work puts forward photonic systems as a platform for experiments in the eld of information thermodynamics. In the third part of this thesis, we present a new method for the characterisation of broadband parametric down-conversion, based on stimulated frequency generation. In particular, we analyse the information contained in the frequency generation produced in the same mode as a seeding beam, for a type-II down-conversion process. We derive a model for this signal and argue that its detection can provide a useful characterisation tool in the high-gain regime, allowing for a self-referenced estimation of squeezing gain. We propose a method for measuring this signal and present an experimental realisation, based on a wave-guided source, at telecommunication wavelengths. Our experimental results demonstrate that the proposed measurement is an e ective experimental handle for discerning the intricate structure of broadband parametric down-conversion.
Over the last few decades, quantised excitations of the electromagnetic field have proven to be an ideal system with which to investigate and harness quantum optical phenomena. The techniques developed have enabled fundamental tests of quantum mechanics as well as practical applications in quantum metrology and quantum information processing. Advancing to larger-scale entangled quantum systems will open up new regimes of quantum many-body physics, allowing us to probe the limits of quantum mechanics and enabling truly quantum-enhanced technologies. However, moving towards this goal will require further experimental and theoretical innovations. The work described in this thesis focuses on several different aspects of optical quantum information, but are ultimately all linked by this long-term aim. The first part of this thesis describes a novel method for strain-based active control of quantum optical circuits and a new method for the characterisation of high efficiency detectors. Building on this, I discuss in detail two different fields of quantum optics that stand to benefit from these techniques. I initially consider quantum-enhanced metrology, including work aimed towards demonstrating a truly better-than-classical phase measurement, and a theoretical exploration of multiple-phase estimation. Finally, I focus on linear-optical quantum information processing, exploring in detail the use of time-frequency encodings for quantum computing.
Quantum optics has successfully been used to test fundamental principles in quantum physics and to demonstrate the potential of quantum-enhanced technologies. Linear quantum optics, in which large quantum states of light are produced by optical interference of smaller quantum states, has proved to be particularly fruitful. Further progress will rely both on developing improved experimental tools to manipulate and measure quantum light, and on expanding and refining the range of applications of these technologies. This thesis presents our contributions towards both of these endeavours. We first focus on some of the components necessary for linear quantum optics, starting with the requirement for reconfigurable interference between several optical modes. We propose a novel design for interferometers that satisfy this requirement, which is based on a new mathematical decomposition of unitary matrices used to describe optical interference. We show that our design is more efficient than previously known designs. We also experimentally demonstrate a modular approach to building these devices, which is based on the assembly of multiple UV-written integrated photonic chips. These chips are characterised, and three of them are assembled into a structure shown to enable a wide range of optical transformations. We then study methods of photon detection, showing how photon detectors can be calibrated and discussing the operation of superconducting photon number resolving transition edge sensors. Next, we study two applications of linear optics. We examine the applicability of a proposal for simulating molecular spectroscopy using quantum optics in the presence of experimental imperfections. Our findings are illustrated with a proof of principle experiment in which we simulate part of the vibronic spectrum of the tropolone molecule. Finally, we study a class of optical devices, known as optical Ising machines, that has been shown to find solutions to difficult combinatorial problems. Describing the optical pulses in these devices in phase space as Gaussian quasi-probability distributions that evolve stochastically, we analyse the computational mechanism of these machines and show in theory that they can be simplified without affecting their performance.
This thesis is concerned with the generation of non-classical quantum states of light, the photon-level manipulation of quantum states and the accurate tomography of both quantum states and quantum processes. In optics, quantum information can be encoded and processed in both discrete and continuous variables. Hybrid approaches combining for example homodyne detection with conditional state preparation and manipulation are gaining increasing prominence. The development and characterization of a time-domain balanced homodyne detector (BHD) is presented. The detector has a bandwidth of 80 MHz, a signal-to-noise ratio of 14.5 dB and an efficiency of 86% making it well-suited to pulse-to-pulse measurement of quantum optical states. The BHD is employed to perform quantum state tomography (QST) of non-classical multi-photon Fock states generated by spontaneous parametric down-conversion. A detailed investigation of the mode-matching between the local oscillator used for homodyne detection and the generated Fock states is presented. The one-, two- and three-photon Fock states are reconstructed with a combined preparation and detection efficiency exceeding 50%. Fock states have a number of applications in quantum state engineering, where non-classical ancilla states and conditional measurements enable photon-level manipulation of quantum states. Fock state filtration (FSF) is investigated - an example of a post-selected beam splitter which is a basic building block for many quantum state engineering protocols. A model is developed incorporating the effect of experimental imperfections. An experimental implementation of a Fock state filter is fully characterized by means of coherent-state quantum process tomography (QPT). The reconstructed process is found to be consistent with the model. The filter preferentially removes the single-photon component from an arbitrary input quantum state. Calibration of optical detectors in the quantum regime is discussed. Quantum detector tomography (QDT) is reviewed and contrasted with a new technique for performing QST with a calibrated detector known as the fitting of data patterns (FDP). The first experimental characterization of a BHD is performed by probing the detector with phase-averaged coherent states. The FDP method is shown to be applicable to the estimation of quantum processes, where a detector response is not assumed - thus demonstrating the versatility of the FDP approach as a new method in the quantum tomography toolbox.
In 2009, physicists at the National Institute of Standards and Technology in Colorado, Boulder developed what could arguable be called the first rudimentary quantum computer [1]. The past decade has seen unprecedented improvements in quantum information science culminating in the demonstration of quantum supremacy --- that quantum computers can solve problems that are impractical to be solved on the best supercomputers [2]. This remarkable progress necessitates the development of techniques to characterize the quantum devices that are being developed. In my thesis, I will focus on such devices that manipulate and detect light. In Chapter 1, I will introduce the reader to the historical underpinnings of the study of light. After surveying the history of light since time immemorial, I will delve into the developments in the study of light in the 19th and the early 20th century. I will then present a brief introduction to quantum mechanics. I end this chapter by demonstrating how light is quantized. In Chapter 2, I will introduce the various tools necessary to delve into this dissertation. After defining quadrature operators and Wigner functions, I will introduce various states of light used in this thesis. I will then discuss how the evolution, as well as detection of quantum optical states, are modelled. I will then present the formalism of Gaussian quantum information that simplifies the manipulation of certain states of light. Finally, I will briefly talk about quantum metrology and show its advantage in phase estimation. In Chapter 3, I will introduce a method to characterize linear and quadratically nonlinear optical systems. After motivating the need for this work, I will introduce the modifications necessary to the standard Mach-Zehnder interferometer in order to characterize optical systems with it. I will then show how to characterize linear optical systems with coherent probes. I will also show that this scheme is shot-noise limited. I will then show that by using single photons in addition, we can characterize quadratically nonlinear optical systems. Finally, I will show that no advantage is gained in sensitivity by using squeezed light along with coherent light as probes. In Chapter 4, I will introduce a method to characterize photodetectors. This is done by developing an experimental method to find the Wigner functions of the POVM set corresponding to a photodetector. After motivating the necessity of this work as well as describing the proposed experimental setup, I will show how this scheme can
A longstanding goal in quantum optics has been to realize a photon-number-resolving detector that efficiently counts the number of photons in an optical field. This goal has been largely met with the development of transition edge sensors which can count up to roughly 20 photons with efficiencies over 95%. This thesis presents three experiments that employ these detectors to characterize and prepare quantum states of light. Firstly, we develop a weak-field homodyne detector. By replacing the photodiodes conventionally used in homodyne detection with transition edge sensors, we experimentally implement a versatile measurement device that can tune between photon counting and quadrature measurements. We study the transition between these complementary measurement regimes and determine the minimum local oscillator strength needed to perform quadrature measurements. Secondly, we use the weak-field homodyne detector as a quantum state engineering tool. We propose a scheme to prepare a wide range of definite parity states, including two- and four-component Schrödinger cat states of arbitrary size with nearly perfect fidelity. Thirdly, we perform optical interferometry using quantum states of light with the aim of surpassing the maximal precision achievable with classical light, i.e. the shot-noise limit. We propose and experimentally implement a scheme that uses high-gain squeezed vacuum sources and transition edge sensors to prepare loss-tolerant entangled states containing up to 8 photons. While our achieved precision does not unconditionally (i.e. without post-selecting on certain measurement trials) surpass the shot-noise limit, our results do demonstrate the robustness of these entangled states to loss despite their size.