This thesis is concerned with the generation of non-classical quantum states of light, the photon-level manipulation of quantum states and the accurate tomography of both quantum states and quantum processes. In optics, quantum information can be encoded and processed in both discrete and continuous variables. Hybrid approaches combining for example homodyne detection with conditional state preparation and manipulation are gaining increasing prominence. The development and characterization of a time-domain balanced homodyne detector (BHD) is presented. The detector has a bandwidth of 80 MHz, a signal-to-noise ratio of 14.5 dB and an efficiency of 86% making it well-suited to pulse-to-pulse measurement of quantum optical states. The BHD is employed to perform quantum state tomography (QST) of non-classical multi-photon Fock states generated by spontaneous parametric down-conversion. A detailed investigation of the mode-matching between the local oscillator used for homodyne detection and the generated Fock states is presented. The one-, two- and three-photon Fock states are reconstructed with a combined preparation and detection efficiency exceeding 50%. Fock states have a number of applications in quantum state engineering, where non-classical ancilla states and conditional measurements enable photon-level manipulation of quantum states. Fock state filtration (FSF) is investigated - an example of a post-selected beam splitter which is a basic building block for many quantum state engineering protocols. A model is developed incorporating the effect of experimental imperfections. An experimental implementation of a Fock state filter is fully characterized by means of coherent-state quantum process tomography (QPT). The reconstructed process is found to be consistent with the model. The filter preferentially removes the single-photon component from an arbitrary input quantum state. Calibration of optical detectors in the quantum regime is discussed. Quantum detector tomography (QDT) is reviewed and contrasted with a new technique for performing QST with a calibrated detector known as the fitting of data patterns (FDP). The first experimental characterization of a BHD is performed by probing the detector with phase-averaged coherent states. The FDP method is shown to be applicable to the estimation of quantum processes, where a detector response is not assumed - thus demonstrating the versatility of the FDP approach as a new method in the quantum tomography toolbox.
This thesis is concerned with the generation of non-classical quantum states of light, the photon-level manipulation of quantum states and the accurate tomography of both quantum states and quantum processes. In optics, quantum information can be encoded and processed in both discrete and continuous variables. Hybrid approaches combining for example homodyne detection with conditional state preparation and manipulation are gaining increasing prominence. The development and characterization of a time-domain balanced homodyne detector (BHD) is presented. The detector has a bandwidth of 80 MHz, a signal-to-noise ratio of 14.5 dB and an efficiency of 86% making it well-suited to pulse-to-pulse measurement of quantum optical states. The BHD is employed to perform quantum state tomography (QST) of non-classical multi-photon Fock states generated by spontaneous parametric down-conversion. A detailed investigation of the mode-matching between the local oscillator used for homodyne detection and the generated Fock states is presented. The one-, two- and three-photon Fock states are reconstructed with a combined preparation and detection efficiency exceeding 50%. Fock states have a number of applications in quantum state engineering, where non-classical ancilla states and conditional measurements enable photon-level manipulation of quantum states. Fock state filtration (FSF) is investigated - an example of a post-selected beam splitter which is a basic building block for many quantum state engineering protocols. A model is developed incorporating the effect of experimental imperfections. An experimental implementation of a Fock state filter is fully characterized by means of coherent-state quantum process tomography (QPT). The reconstructed process is found to be consistent with the model. The filter preferentially removes the single-photon component from an arbitrary input quantum state. Calibration of optical detectors in the quantum regime is discussed. Quantum detector tomography (QDT) is reviewed and contrasted with a new technique for performing QST with a calibrated detector known as the fitting of data patterns (FDP). The first experimental characterization of a BHD is performed by probing the detector with phase-averaged coherent states. The FDP method is shown to be applicable to the estimation of quantum processes, where a detector response is not assumed - thus demonstrating the versatility of the FDP approach as a new method in the quantum tomography toolbox.
This thesis reports the realization and applications of a versatile wideband balanced homodyne detector operating in the time domain and intended for Quantum Optical Tomography. The detector can work with high repetition rate lasers used for the production and measurement of the electric field quadratures of quantum states of light. Full characterization of the detector by shot-noise measurements and by verifying its capability to reconstruct the density matrix and Wigner function of various states of interest is given. By overcoming photodiodes response mismatch, high frequency electronics issues and by choosing an appropriate optical set-up, a high level of common mode suppression (52.4dB) and a low electronic noise gave a shot-to-electronic noise ratio of I3dB for a Local Oscillator with 6.2 x 108 photons-per-pulse on a ~ 100MHz bandwidth. Results for the characterization of a single-photon Fock state are presented. An average efficiency of 56% was obtained for the generation/detection of the state.
Quantum optics is central to emerging quantum technologies such as quantum metrology and quantum information. The continuous variable (CV) approach to encoding information in a physical system, for example the electromagnetic field quadratures has significant advantages over discrete variables (DV) encoding. CV offers higher density encoding in a single optical state and on-demand state preparation for example. However, techniques for CV preparation, manipulation and measurement are not as well developed as the corresponding DV approach. In this thesis we present methods to characterize quantum detectors that operate in the CV regime, and discuss their application to CV state preparation. A quantum detector is described by its positive operator valued measure (POVM) set, with one operator for each measurement outcome. We present an experimental scheme for detector tomography, that is reconstruction of the POVM set of an unknown detector by means of measurement outcomes for a set of tomographically complete input states. We use this scheme to experimentally determine the POVM set of an avalanche photodiode (APD) and a time-multiplexed-detector (TMD) and compare the results to models of the detectors. We introduce a weak-homodyne photon-number-resolving detector (PNRD) , which uses a weak local oscillator beam to set a phase reference for the detection process. We develop a theoretical description of the sensitivity regimes for this detector using the Wigner phase space picture. We also present experimental detector tomography for a weak-homodyne detector based on two APDs. In many cases it is sufficient to calibrate the efficiencies of previously characterized PNRDs. We experimentally demonstrate a scheme using correlated photons produced by spontaneous parametric downconversion (SPDC) to determine the efficiencies of PNRDs, based on the photon number statistics of the source. The same SPDC source is also used to demonstrate preparation of photonic states in the photon number basis and for a first proof-of-principle experiment with a weak-homodyne PNRD based on a TMD.
Conditional quantum optical processes enable a wide range of technologies from generation of highly non-classical states to implementation of quantum logic operations. The process fidelity that can be achieved in a realistic implementation depends on a number of system parameters. Here we experimentally examine Fock state filtration, a canonical example of a broad class of conditional quantum operations acting on a single optical field mode. This operation is based upon interference of the mode to be manipulated with an auxiliary single-photon state at a beam splitter, resulting in the entanglement of the two output modes. A conditional projective measurement onto a single photon state at one output mode heralds the success of the process. This operation, which implements a measurement-induced nonlinearity, is capable of suppressing particular photon-number probability amplitudes of an arbitrary quantum state. We employ coherent-state process tomography to determine the precise operation realized in our experiment, which is mathematically represented by a process tensor. To identify the key sources of experimental imperfection, we develop a realistic model of the process and identify three main contributions that significantly hamper its efficacy. The experimentally reconstructed process tensor is compared with the model, yielding a fidelity better than 0.95. This enables us to identify three key challenges to overcome in realizing a filter with optimal performance—namely the single-photon nature of the auxiliary state, high mode overlap of the optical fields involved, and the need for photon-number-resolving detection when heralding. The results show that the filter does indeed exhibit a non-linear response as a function of input photon number and preserves the phase relation between Fock layers of the output state, providing promise for future applications.
The implementation of optical quantum technologies requires precise and complete characterisation tools for multi-mode nonclassical states of light. In this thesis, we propose and we implement experimentally three applications of optical quantum measurements, which combine aspects of light that are described by both discrete and continuous variables. In the rst part of this thesis, we present a new scheme for interferometric phase estimation, which uses double homodyne measurements as an alternative to photon counting. We show that, without requiring a phase reference, this scheme can achieve the optimum phase estimation precision for all path-symmetric probe states with a de ned number of photons. Furthermore, the estimation procedure is robust against state preparation imperfections, and naturally yields the same precision for all values of the estimated phase. We implement the proposed scheme experimentally, using a polarisation interferometer probed by a single-photon signal, and temporally multiplexing a single homodyne detector. We repeat the experiment with classical probe states. For both cases, we demonstrate the accuracy and precision of the proposed method, our implementation deviating by 5% from the fundamental precision bound. We demonstrate that, in our scheme, single-photon probe states can provide better precision than weak coherent ones. These results indicate that hybrid quantum resources, which combine tools from the discrete and continuous-variable paradigms, can play a signi cant role in practical sensing scenarios. In the second part of this thesis, we present an application in the eld of information thermodynamics, reporting an experimental realisation, in a photonic setup, of Maxwell's demon. We show that a measurement at the few-photons level, followed by a feed-forward operation, allows the extraction of work from intense thermal light into an electric circuit. The interpretation of the experiment leads us to the derivation of an equality relating work extraction to information acquired by measurement. We prove a bound using this relation, and show that it is in agreement with the experimental results. Our work puts forward photonic systems as a platform for experiments in the eld of information thermodynamics. In the third part of this thesis, we present a new method for the characterisation of broadband parametric down-conversion, based on stimulated frequency generation. In particular, we analyse the information contained in the frequency generation produced in the same mode as a seeding beam, for a type-II down-conversion process. We derive a model for this signal and argue that its detection can provide a useful characterisation tool in the high-gain regime, allowing for a self-referenced estimation of squeezing gain. We propose a method for measuring this signal and present an experimental realisation, based on a wave-guided source, at telecommunication wavelengths. Our experimental results demonstrate that the proposed measurement is an e ective experimental handle for discerning the intricate structure of broadband parametric down-conversion.
We report about the realization and the applications of an efficient pulsed optical homodyne apparatus operating in the time domain at the high repetition rates characteristic of commonly used mode-locked lasers for the analysis of quantum light states. We give a full characterization of our system by shot-noise measurements and by verifying its capability to work in a gated configuration at lower acquisition rates. We demonstrate the potential of this high-frequency time-domain detector by applying it to the reconstruction of the density matrix elements and of the Wigner functions of various field states by means of quantum tomography. Results are shown for the complete characterization of simple coherent states with low average photon number, of single-photon Fock states and of the so-called single-photon added coherent states, which result from the elementary excitation of a classical wave-like field. Wigner functions with negative values are observed for the non-classical states and an overall efficiency of about 60% is obtained for the generation/detection system.
A single-photon Fock state has been generated by means of conditional preparation from a two-photon state emitted in the process of spontaneous parametric down-conversion. A recently developed high-frequency homodyne tomography technique has been used to completely characterize the Fock state by means of a pulse-to-pulse analysis of the detectors' difference photocurrent. The density matrix elements of the generated state have been retrieved with a final detection efficiency of about 57%. A comparison has been performed between the phase-averaged tomographic reconstructions of the Wigner function as obtained from the measured density-matrix elements and from a direct Abel transform of the homodyne data. The ability of our system to work at the full repetition rate of the pulsed laser (82MHz) substantially simplifies the detection scheme, allowing for more ``exotic'' quantum states to be generated and analyzed.