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Dissecting Kitaev Spin Liquid into Collective Patterns of Spin Coupling Bonds in Real Space

Qiyun Fu, Zexin Fang, Tieyan Si

Published Oct 9, 2025• 0 citations
Publisher

Abstract

How to characterize the topological order of quantum spin liquids remains a long-standing theoretical challenge. In this work, we employ the pattern decomposition method to analyze the fine structure of the Kitaev spin liquid on a finite honeycomb lattice. The Kitaev Hamiltonian decomposes into six sub-Hamiltonians whose weight factors form periodic patterns under unit cell translations. Correspondingly, the eigenstates of the Kitaev spin liquid are partitioned into six degenerate subspaces, unveiling the ordered structure of the spin liquid state. The critical point of the topological phase transition from a gapped to a gapless phase is identified through the sub-Hamiltonians. This Hamiltonian dissection approach reveals the fine structure of the Kitaev spin liquid and offers a promising platform for the quantum simulation of spin liquids.

DOI
10.20944/preprints202510.0657.v1

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How to characterize the topological order of quantum spin liquids remains a long-standing theoretical challenge. In this work, we employ the pattern decomposition method to analyze the fine structure of the Kitaev spin liquid on a finite honeycomb lattice. The Kitaev Hamiltonian decomposes into six sub-Hamiltonians whose weight factors form periodic patterns under unit cell translations. Correspondingly, the eigenstates of the Kitaev spin liquid are partitioned into six degenerate subspaces, unveiling the ordered structure of the spin liquid state. The critical point of the topological phase transition from a gapped to a gapless phase is identified through the sub-Hamiltonians. This Hamiltonian dissection approach reveals the fine structure of the Kitaev spin liquid and offers a promising platform for the quantum simulation of spin liquids.
The ruby lattice is a four-valent lattice interpolating between honeycomb and triangular lattices. In this work we investigate the topological spin-liquid phases of a spin Hamiltonian with Kitaev interactions on the ruby lattice using exact diagonalization and perturbative methods. The latter interactions combined with the structure of the lattice yield a model with ${\mathbb{Z}}_{2}\ifmmode\times\else\texttimes\fi{}{\mathbb{Z}}_{2}$ gauge symmetry. We mapped out the phase diagram of the model and found gapped and gapless spin-liquid phases. While the low-energy sector of the gapped phase corresponds to the well-known topological color code model on a honeycomb lattice, the low-energy sector of the gapless phases is described by an effective spin model with three-body interactions on a triangular lattice. A gap is opened in the spectrum in small magnetic fields, where we showed that the ground state has a finite topological entanglement entropy. We argue that the gapped phases could be possibly described by exotic excitations, and their corresponding spectrum is richer than the Ising phase of the Kitaev model.
We study the quantum-spin-liquid phase in a variant of the Kitaev model where the bonds of the honeycomb lattice are distributed in a Kekul\'e pattern. The system supports gapped and gapless Z2{Z}_{2}Z2​ quantum spin liquids with interesting differences from the original Kitaev model, the most notable being a gapped Z2{Z}_{2}Z2​ spin liquid on a kagome lattice. Perturbing the exactly solvable model with antiferromagnetic Heisenberg perturbations, we find a magnetically ordered phase stabilized by a quantum ``order by disorder'' mechanism, as well as an exotic continuous quantum phase transition between the topological spin liquid and this magnetically ordered phase. Using a combination of field theory and Monte Carlo simulations, we find that the transition likely belongs to the $3D\text{\ensuremath{-}}XY\ifmmode\times\else\texttimes\fi{}{Z}_{2}$ universality class.
These lecture notes focus on the Kitaev honeycomb model, a two-dimensional quantumsystem with three distinct Ising-type interactions, depending on the direction of eachbond. This model has proven particularly important for describing quantum spin liquids,as well as for applications in topological quantum computing, due to its exotictopological properties. It constitutes the first exactly solvable theoretical model thatfully captures the behavior of a quantum spin liquid. We begin by presenting the geometryof the model, the Hamiltonian that describes the system, and Alexei Kitaev's effort toobtain an exact analytical solution, based on the decomposition of the Hilbert spaceinto flux sectors. We then present Ettore Majorana's observation that the Dirac equationalso admits real solutions, leading to the theoretical prediction of Majorana fermions-- particles that are identical to their antiparticles. We examine how the spatialseparation of Majorana operators leads to the rise of unbound Majorana fermions, andshowcase the exotic topological properties that manifest in physical systems such assuperconducting wires. Next, we represent the Hamiltonian in the basis of Majoranafermions, by expressing spin operators using four Majorana operators. The transitionfrom the extended space L~\tilde{\mathcal{L}}L~ to the physical subspace L\mathcal{L}Lis achieved through a gauge transformation of the Z2\mathbb{Z}_2Z2​ group. We thenreformulate the Hamiltonian in the basis of complex bond and matter fermions, transitionto momentum space, and assume that the system lies in the zero-flux sector. Through theBogoliubov--de Gennes transformation, we arrive at the final diagonalized Hamiltonianin the quasiparticle basis. Finally, we represent the possible phases -- the gaplessphase (phase BBB) and the gapped phases (phase AαiA_{\alpha_i}Aαi​​) -- compute thecorresponding energy spectrum, and present the complete phase diagram. By employing thecorrelation function, we show that all phases are characterized by strong quantumentanglement and spin fractionalization, classifying the system as a quantum spin liquid.
Kitaev's model of spins interacting on a honeycomb lattice describes a quantum spin liquid, where an emergent static Z2{\mathbb{Z}}_{2}Z2​ gauge field is coupled to Majorana fermions. In the presence of an external magnetic field and for a range of interaction strengths, the system behaves as a gapped, non-Abelian quantum spin liquid. In this phase, the vortex excitations of the emergent Z2{\mathbb{Z}}_{2}Z2​ gauge field have Majorana zero modes bound to them. Motivated by recent experimental progress in measuring and characterizing real materials that could exhibit spin-liquid behavior, we analytically calculate the dynamical spin structure factor in the non-Abelian phase of the Kitaev's honeycomb model. In particular, we treat the case of quenched disorder in the vortex configurations. Our calculations reveal a peak in the low-energy dynamical structure factor that is a signature of the spin-liquid behavior. We map the effective Hamiltonian to that of a chiral ppp-wave superconductor by using the Jordan-Wigner transformation. Subsequently, we analytically calculate the wave functions of the Majorana zero modes, the energy splitting for finite separation of the vortices and, finally, the dynamical structure factor in presence of quenched disorder.
We perform large-scale density matrix renormalization group simulations of the SU(4) Heisenberg model on the honeycomb lattice to address the long-standing question of its ground state in an unbiased and quantitatively controlled manner. We find reliable numerical evidence that the ground state is a gapped spin-orbital liquid, presumably with a Z_{4} topological order, characterized by a finite topological entanglement entropy close to ln(4), the absence of both SU(4) and lattice symmetry breaking, and a variationally optimized ground-state energy well below the previously proposed π-flux variational state. By exploiting full SU(4) symmetry and keeping up to 12 800 SU(4) multiplets, corresponding to more than 1×10^{6} U(1) states, we achieve unprecedented accuracy for two-dimensional SU(4) quantum magnets. Finite-size scaling of energies and entanglement entropies supports a robust gapped phase in the two-dimensional limit, while a gapless critical state on narrow cylinders is identified as a proximate remnant of a Dirac spin-orbital liquid. Our results find the SU(4) honeycomb Heisenberg model a realization of a gapped topological spin-orbital liquid and provide convincing numerical evidence for topological order in a highly symmetric two-dimensional quantum magnet.
We investigate the nature of the topological quantum phase transition between the gapless and gapped Kitaev quantum spin liquid phases away from the exactly solvable point. The transition is driven by anisotropy of the Kitaev couplings. At the critical point, the two Dirac points of the gapless Majorana modes merge, resulting in the formation of a semi-Dirac point with quadratic and linear band touching directions. We derive an effective Gross-Neveu-Yukawa-type field theory that describes the topological phase transition in the presence of additional magnetic interactions. We obtain the infrared scaling form of the propagator of the dynamical Ising order parameter field and perform a renormalization-group analysis. The universality of the transition is found to be different from that of symmetry-breaking phase transitions of semi-Dirac electrons. However, as in the electronic case, the Majorana fermions acquire an anomalous dimension, indicative of the breakdown of the fractionalized quasiparticle description.