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arXiv:1608.00254 · Physical review. B./Physical review. B

Topological spin liquids in the ruby lattice with anisotropic Kitaev interactions

Saeed S. Jahromi, Mehdi Kargarian, Seyed Farhad Masoudi, A. Langari

Published Sep 26, 2016• 14 citations
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Abstract

The ruby lattice is a four-valent lattice interpolating between honeycomb and triangular lattices. In this work we investigate the topological spin-liquid phases of a spin Hamiltonian with Kitaev interactions on the ruby lattice using exact diagonalization and perturbative methods. The latter interactions combined with the structure of the lattice yield a model with ${\mathbb{Z}}_{2}\ifmmode\times\else\texttimes\fi{}{\mathbb{Z}}_{2}$ gauge symmetry. We mapped out the phase diagram of the model and found gapped and gapless spin-liquid phases. While the low-energy sector of the gapped phase corresponds to the well-known topological color code model on a honeycomb lattice, the low-energy sector of the gapless phases is described by an effective spin model with three-body interactions on a triangular lattice. A gap is opened in the spectrum in small magnetic fields, where we showed that the ground state has a finite topological entanglement entropy. We argue that the gapped phases could be possibly described by exotic excitations, and their corresponding spectrum is richer than the Ising phase of the Kitaev model.

DOI
10.1103/physrevb.94.125145

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The ruby lattice is a four-valent lattice interpolating between honeycomb and triangular lattices. In this work we investigate the topological spin-liquid phases of a spin Hamiltonian with Kitaev interactions on the ruby lattice using exact diagonalization and perturbative methods. The latter interactions combined with the structure of the lattice yield a model with Z2\ifmmode×\else\texttimes\fiZ2{\mathbb{Z}}_{2}\ifmmode\times\else\texttimes\fi{}{\mathbb{Z}}_{2}Z2​\ifmmode×\else\texttimes\fiZ2​ gauge symmetry. We mapped out the phase diagram of the model and found gapped and gapless spin-liquid phases. While the low-energy sector of the gapped phase corresponds to the well-known topological color code model on a honeycomb lattice, the low-energy sector of the gapless phases is described by an effective spin model with three-body interactions on a triangular lattice. A gap is opened in the spectrum in small magnetic fields, where we showed that the ground state has a finite topological entanglement entropy. We argue that the gapped phases could be possibly described by exotic excitations, and their corresponding spectrum is richer than the Ising phase of the Kitaev model.
The ruby lattice has been the subject of much interest recently due its realization in Rydberg atom arrays, where its rich variety of frustrated interactions gives rise to topologically ordered quantum spin liquids. Similarly, numerical studies of ruby-lattice spin models, with both isotropic and anisotropic interactions, have provided evidence of gapped and gapless spin-liquid ground states with different low-energy gauge structures. Motivated by these findings, we perform a projective symmetry group (PSG) classification of U(1) and Z2\mathbb{Z}_{2}Z2​ fermionic spinon mean-field theories$\unicode{x2014}$respecting space-group and time-reversal symmetries$\unicode{x2014}$for S=1/2S=1/2S=1/2 spins. We obtain a total of 50 U(1) and 64 Z2\mathbb{Z}_{2}Z2​ PSGs, and upon restricting their realization via mean-field Ansa¨tze\textit{Ansätze}Ansa¨tze with up to second-nearest-neighbor singlet amplitudes (relevant to the models studied here), only 8 U(1) and 18 Z2\mathbb{Z}_{2}Z2​ distinct states are obtained. We present the singlet fields for all Ansa¨tze\textit{Ansätze}Ansa¨tze up to third-nearest-neighboring bonds and discuss their spinon dispersions as well as their dynamical spin structure factors. Building on this information, we also obtain the phase diagram of the Heisenberg model in the presence of first (J1J_{1}J1​), second (J1′J_{1}'J1′​), and third (J2J_{2}J2​) neighbor antiferromagnetic couplings within a self-consistent mean-field approximation.
We theoretically studied an exactly solvable gamma matrix generalization of the Kitaev spin model on the ruby lattice, which is a honeycomb lattice with 'expanded' vertices and links. We find that this model displays an exceptionally rich phase diagram that includes (i) gapless phases with stable spin Fermi surfaces, (ii) gapless phases with low-energy Dirac cones and quadratic band touching points and (iii) gapped phases with finite Chern numbers possessing the values ±4,±3,±2 and ±1. The model is then generalized to include Ising-like interactions that break the exact solvability of the model in a controlled manner. When these terms are dominant, they lead to a trivial Ising ordered phase which is shown to be adiabatically connected to a large coupling limit of the exactly solvable phase. In the limit where these interactions are weak, we treat them within mean-field theory and present the resulting phase diagrams. We discuss the nature of the transitions between various phases. Our results show the richness of possible ground states in closely related magnetic systems.
The formation of quantum spin liquids in frustrated magnets represents an exciting possibility due to the rather exotic features they harbor, including fractionalized excitations and emergent gauge fields. \nUnfortunately, they are notoriously difficult to study as there are often no good analytical methods available and quantum Monte Carlo simulations are hindered by the negative sign problem. \nThe Kitaev honeycomb model is a notable exception of a frustrated quantum model which is exactly solvable and which hosts a number of distinct quantum spin liquid ground states. \nAs such, it allows for a rare opportunity to study the physics of spin liquids with full analytical control. \n \nIn this thesis, we study the fractionalization of spin-1/2 moments into Majorana fermions and an emergent Z2 gauge field in a generalization of the Kitaev honeycomb model to a number of three-dimensional lattices. \nWhile the excitations of the gauge field are always gapped, the fermionic quasiparticles may exhibit a gapless dispersion, forming fully two-dimensional Fermi surfaces, symmetry protected nodal lines, or topological Weyl nodes. \nWe show that one can deduce rather general constraints on the possible gapless excitations by making use of an object called the projective symmetry group. \nIn doing so we provide a scheme for classifying the various gapless Kitaev spin liquids. \nA thorough analysis is carried out for a number of these spin liquids, primarily investigating the stability of the gapless modes and the novel features resulting from their sometimes non-trivial topology, as well as their effects on certain equal-time correlation functions.
We study the spin-1/21/21/2 Kitaev-Heisenberg model on the square-hexagon-dodecagon lattice with a symmetry-preserving tri-coloring of the Kitaev exchanges. We focus on two cases: (i) the pure Kitaev model with anisotropic exchanges and (ii) the Kitaev-Heisenberg model with isotropic Kitaev exchange. In the absence of Heisenberg interactions, we use the standard mapping of the Kitaev model onto a quadratic Majorana-fermion problem in a Z2\mathbb{Z}_2Z2​ gauge field. We find a gapped energy spectrum throughout the positive-coupling phase diagram, except at a single point where the twofold-degenerate energy bands form a Dirac cone. This unique gapped region corresponds to a toric code phase. However, depending on the couplings, vortex excitations on square, hexagonal, and dodecagonal plaquettes realize three distinct relative assignments to the eee and mmm anyons. We determine these relative assignments from the physical fermion parity of the vortex sectors and locate their boundaries by tracking zero crossings of vortex-bound Majorana levels. For the isotropic Kitaev-Heisenberg model, we combine graph-based projected entangled-pair-state calculations, exact diagonalizations, and linear spin-wave theory to study the entire phase diagram. Apart from the toric code topological phases that are robust around the Kitaev limits, we obtain four collinear magnetically ordered phases that can be characterized by their local and relative orderings of hexagonal plaquettes. We also identify a special point at which the ground state is a product state.
We study quantum disordered ground states of the two-dimensional Heisenberg-Kitaev model on the triangular lattice using a Schwinger boson approach. Our aim is to identify and characterize potential gapped quantum spin liquid phases that are stabilized by anisotropic Kitaev interactions. For antiferromagnetic Heisenberg and Kitaev couplings and sufficiently small spin SSS, we find three different symmetric Z2{Z}_{2}Z2​ spin liquid phases, separated by two continuous quantum phase transitions. Interestingly, the gap of elementary excitations remains finite throughout the transitions. The first spin liquid phase corresponds to the well-known zero-flux state in the Heisenberg limit, which is stable with respect to small Kitaev couplings and develops ${120}^{\ensuremath{\circ}}$ order in the semiclassical limit at large SSS. In the opposite Kitaev limit, we find a different spin liquid ground state, which is a quantum disordered version of a magnetically ordered state with antiferromagnetic chains, in accordance with results in the classical limit. Finally, at intermediate couplings, we find a spin liquid state with unusual spin correlations. Upon spinon condensation, this state develops Bragg peaks at incommensurate momenta in close analogy to the magnetically ordered Z2 vortex crystal phase, which has been analyzed in recent theoretical works.
We study the quantum-spin-liquid phase in a variant of the Kitaev model where the bonds of the honeycomb lattice are distributed in a Kekul\'e pattern. The system supports gapped and gapless Z2{Z}_{2}Z2​ quantum spin liquids with interesting differences from the original Kitaev model, the most notable being a gapped Z2{Z}_{2}Z2​ spin liquid on a kagome lattice. Perturbing the exactly solvable model with antiferromagnetic Heisenberg perturbations, we find a magnetically ordered phase stabilized by a quantum ``order by disorder'' mechanism, as well as an exotic continuous quantum phase transition between the topological spin liquid and this magnetically ordered phase. Using a combination of field theory and Monte Carlo simulations, we find that the transition likely belongs to the $3D\text{\ensuremath{-}}XY\ifmmode\times\else\texttimes\fi{}{Z}_{2}$ universality class.