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arXiv:2402.12610 · Physical Review Letters

Nature of Topological Phase Transition of Kitaev Quantum Spin Liquids

Huanzhi Hu, Frank Krüger

Published Oct 2, 2024• 5 citations
arXivHTMLPDF

Abstract

We investigate the nature of the topological quantum phase transition between the gapless and gapped Kitaev quantum spin liquid phases away from the exactly solvable point. The transition is driven by anisotropy of the Kitaev couplings. At the critical point, the two Dirac points of the gapless Majorana modes merge, resulting in the formation of a semi-Dirac point with quadratic and linear band touching directions. We derive an effective Gross-Neveu-Yukawa-type field theory that describes the topological phase transition in the presence of additional magnetic interactions. We obtain the infrared scaling form of the propagator of the dynamical Ising order parameter field and perform a renormalization-group analysis. The universality of the transition is found to be different from that of symmetry-breaking phase transitions of semi-Dirac electrons. However, as in the electronic case, the Majorana fermions acquire an anomalous dimension, indicative of the breakdown of the fractionalized quasiparticle description.

DOI
10.1103/physrevlett.133.146603

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We investigate the nature of the topological quantum phase transition between the gapless and gapped Kitaev quantum spin liquid phases away from the exactly solvable point. The transition is driven by anisotropy of the Kitaev couplings. At the critical point, the two Dirac points of the gapless Majorana modes merge, resulting in the formation of a semi-Dirac point with quadratic and linear band touching directions. We derive an effective Gross-Neveu-Yukawa-type field theory that describes the topological phase transition in the presence of additional magnetic interactions. We obtain the infrared scaling form of the propagator of the dynamical Ising order parameter field and perform a renormalization-group analysis. The universality of the transition is found to be different from that of symmetry-breaking phase transitions of semi-Dirac electrons. However, as in the electronic case, the Majorana fermions acquire an anomalous dimension, indicative of the breakdown of the fractionalized quasiparticle description.
We investigate the nature of the topological phase transition of the antiferromagnetic Kitaev model on a honeycomb lattice in the presence of a magnetic field along the [111] direction. The field opens a topological gap in the Majorana fermion spectrum and leads to a sequence of topological phase transitions before the field-polarized state is reached. At mean-field level, the gap first closes at the three M points in the Brillouin zone, where the Majorana fermions form Dirac cones, resulting in a change of Chern number by three. An odd number of Dirac fermions in infrared is unusual and requires Berry curvature compensation in ultraviolet, which occurs via topological, ringlike hybridization gaps with higher-energy bands. We perform a renormalization-group analysis of the topological phase transition at the three M points within the Yukawa theory, allowing for intravalley and intervalley fluctuations of the spin-liquid bond operators. We find that the latter lead to a breaking of Lorentz invariance and hence a different universality compared with the standard Ising Gross-Neveu-Yukawa class.
We determine the phase diagrams of anisotropic Kitaev-Heisenberg models on the honeycomb lattice using parton mean-field theories based on different Majorana fermion representations of the S=1/2 spin operators. First, we use a two-dimensional Jordan-Wigner transformation (JWT) involving a semi-infinite snake string operator. To ensure that the fermionized Hamiltonian remains local, we consider the limit of extreme Ising exchange anisotropy in the Heisenberg sector. Second, we use the conventional Kitaev representation in terms of four Majorana fermions subject to local constraints, which we enforce through Lagrange multipliers. For both representations, we self-consistently decouple the interaction terms in the bond and magnetization channels and determine the phase diagrams as a function of the anisotropy of the Kitaev couplings and the relative strength of the Ising exchange. While both mean-field theories produce identical phase boundaries for the topological phase transition between the gapless and gapped Kitaev quantum spin liquids, the JWT fails to correctly describe the magnetic instability and finite-temperature behavior. Our results show that the magnetic phase transition is first order at low temperatures but becomes continuous above a certain temperature. At this energy scale, we also observe a finite-temperature crossover on the quantum-spin-liquid side, from a fractionalized paramagnet at low temperatures, in which gapped flux excitations are frozen out, to a conventional paramagnet at high temperatures. Published by the American Physical Society 2024
We investigate the phase diagram of a bilayer Kitaev honeycomb model with Ising interlayer interactions, deriving effective models via perturbation theory and performing Majorana mean-field theory calculations. We show that a diverse array of magnetic and topological phase transitions occur, depending on the direction of the interlayer Ising interaction and the relative sign of Kitaev interactions. When two layers have the same sign of the Kitaev interaction, a first-order transition from a Kitaev spin liquid to a magnetically ordered state takes place. The magnetic order points along the Ising axis and it is (anti)ferromagnetic for (anti)ferromagnetic Kitaev interactions. However, when two layers have opposite signs of the Kitaev interaction, we observe a notable weakening of magnetic ordering tendencies and the Kitaev spin liquid survives up to a remarkably larger interlayer exchange. Our mean-field analysis suggests the emergence of an intermediate gapped Z2{\mathbb{Z}}_{2}Z2​ spin-liquid state, which eventually becomes unstable upon vison condensation. The confined phase is described by a highly frustrated ${120}^{\ensuremath{\circ}}$ compass model. We furthermore use perturbation theory to study the model with the Ising axis pointing along the $\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{z}$ axis or lying in the xyxyxy plane. In both cases, our analysis reveals the formation of one-dimensional Ising chains, which remain decoupled in perturbation theory, resulting in a subextensive ground-state degeneracy. Our results highlight the interplay between topological order and magnetic ordering tendencies in bilayer quantum spin liquids.
A quantum spin liquid is a magnetic phase of matter that is remarkable for its ground state long-range entanglement and fractional excitations. A quantum spin liquid appears in the well-known Kitaev honeycomb spin-half model. In a magnetic field, there is a phase transition to a topological phase with an energy gap in the bulk and chiral Majorana fermions at the edge. However, recent nuclear magnetic resonance experiments suggest excitations without a gap in this phase, signalled by the cubic temperature dependence of the spin-lattice relaxation rate at low temperatures. In this work, I propose a mechanism to account for this experimental result. I use the localization of chiral Majorana modes in defects to explain the presence of gapless modes in the bulk. Treating the weak interaction between the chiral modes in the defects within a mean-field approximation, I find that these modes remain gapless when the interaction is below a critical value that depends on the magnetic field strength. I used the effective low-energy theory to calculate the spin-lattice relaxation rate and found a behavior that agrees with the experimental result.
The competition between fractionalized spin-liquid states and magnetically ordered phases is an important paradigm in frustrated magnetism. Spin-orbit coupled Mott insulators with Ising-like magnetic anisotropies, such as Kitaev materials, are a particularly rich playground to explore this competition. In this work, we use effective field theory methods to show that a direct quantum phase transition can occur in two-dimensional (2D) Ising spin systems between a topologically ordered chiral spin liquid and a phase with magnetic long-range order. Such a transition can be protected by lattice symmetries and is described by a theory of massless Majorana fields coupled to non-Abelian SO(N)\text{SO}(N)SO(N) gauge fields with a Chern-Simons term. We further show that Euclidean Majorana zero modes bound to Z2{\mathbb{Z}}_{2}Z2​ monopole-instantons in the emergent non-Abelian gauge field are key to understanding spontaneous symmetry breaking in the ordered phase.
Topological phase transitions are typically associated with the formation of gapless states. Spontaneous symmetry breaking can lead to a gap opening, thereby obliterating the topological nature of the system. Here we highlight a completely different destiny for a topological transition in the presence of interaction. Solving a Bernevig-Hughes-Zhang model with local interaction, we show that dynamical quantum fluctuations can lead to the opening of a gap without any symmetry breaking. As we vary the interaction and the bare mass of the model, the continuous gapless topological transition turns into a first-order one, associated with the presence of a massive Dirac fermion at the transition point, showing a Gross-Neveu critical behavior near the quantum critical endpoint. We identify the gap opening as a condensed matter analog of the Coleman-Weinberg mechanism of mass generation.