Remote entanglement of matter qubits plays an important role in quantum networks and quantum repeater. Collective excitations generated via Rydberg blockade in an atomic ensemble-known as Rydberg superatoms-are promising candidates due to collectively enhanced atom-photon coupling and Rydberg-enabled nonlinearity. Here, we experimentally realize remote entanglement between two Rydberg superatoms via single-photon interference. The two setups are separated by 3 m and linked with two 20-m fibers, operated with independent control lasers. We verify that the entanglement generated is free from high-order excitation noise that is a key drawback in the traditional Duan-Lukin-Cirac-Zoller scheme. This Letter paves the way for entangling long-distance separated Rydberg superatoms at a high rate, as the success probability of a single-photon-based entangling scheme scales with the square root of the channel transmittance.
Remote entanglement of matter qubits plays an important role in quantum networks and quantum repeater. Collective excitations generated via Rydberg blockade in an atomic ensemble-known as Rydberg superatoms-are promising candidates due to collectively enhanced atom-photon coupling and Rydberg-enabled nonlinearity. Here, we experimentally realize remote entanglement between two Rydberg superatoms via single-photon interference. The two setups are separated by 3 m and linked with two 20-m fibers, operated with independent control lasers. We verify that the entanglement generated is free from high-order excitation noise that is a key drawback in the traditional Duan-Lukin-Cirac-Zoller scheme. This Letter paves the way for entangling long-distance separated Rydberg superatoms at a high rate, as the success probability of a single-photon-based entangling scheme scales with the square root of the channel transmittance.
Entanglement between a single photon and a matter qubit is an indispensable resource for quantum repeater and quantum networks. With atomic ensembles, the entanglement creation probability is typically very low to inhibit high-order events. In this paper, we propose and experimentally realize a scheme that creates atom-photon entanglement with an intrinsic efficiency of 50%. We make use of Rydberg blockade to generate two collective excitations, lying in separate internal states. By introducing the momentum degree of freedom for the excitations, and interfering them via Raman coupling, we entangle the two excitations. Via retrieving one excitation, we create the entanglement between the polarization of a single photon and the momentum of the remaining atomic excitation, with a measured fidelity of 0.901(8). The retrieved optical field is verified to be genuine single photons. The realized entanglement may be employed to create entanglement between two distant nodes in a fully heralded way and with a much higher efficiency.
In the famous quantum communication scheme developed by Duan et al. [L.M. Duan, M.D. Lukin, J.I. Cirac, and P. Zoller, Nature (London) 414 (2001) 413 ], the probability of successful generating a symmetric collective atomic state with a single-photon emitted have to be far smaller than 1 to obtain an acceptable entangled state. Based on strong dipole-dipole interaction between two Rydberg atoms, two simultaneous excitations in an atomic ensemble are greatly suppressed, which makes it possible to excite a mesoscopic cold atomic ensemble into a near-ideal singly-excited symmetric collective state accompanied by a signal-photon with near unity success probability.
Heralded storage of photons is crucial for advancing quantum networks. Previous realizations have primarily relied on single atoms strongly coupled to optical cavities. In this work, we present the experimental realization of heralded storage using a Rydberg superatom, a mesoscopic atomic ensemble operating in the strong blockade regime. In our approach, an input photon is initially stored in the superatom via electromagnetically induced transparency. Subsequently, a second photon is emitted conditioned on the success of the first photon's storage. Because of the collectively enhanced interaction, both the storage and the emission of the herald photon can be rather efficient in principle. As a demonstration of this technique, we use it to entangle two remote Rydberg superatoms. This method obviates the need for an intermediate node, which is commonly employed in traditional interference-based remote entanglement schemes. Our results showcase the potential of performing cavity-QED-like experiments with Rydberg superatoms. This work opens pathways for numerous applications in quantum networks and linear optical quantum computing.
With Rydberg dipole interactions, a mesoscopic atomic ensemble may behave like a two-level single atom, resulting in the so-called picture of superatom. It is in potential a strong candidate as a qubit in quantum information science, especially for efficient coupling with single photons via collective enhancement that is essential for building quantum internet to connect remote quantum computers. Previously, preliminary studies have been carried out in demonstrating basic concept of Rydberg superatom, a single-photon source, and entanglement with a single photon, etc. While a crucial element of single-shot qubit measurement is still missing. Here we realize the deterministic measurement of a superatom qubit via photon burst in a single shot. We make use of a low-finesse ring cavity to enhance the atom-photon interaction and obtain an in-fiber retrieval efficiency of 44%. Harnessing dipole interaction between two Rydberg levels, we may either create a sequence of multiple single photons or nothing, conditioned on the initial qubit state. We achieve a single-shot measurement fidelity of 93.2% in 4.8 us. Our work complements the experimental toolbox of harnessing Rydberg superatom for quantum information applications.
Owing to the unique physical characteristics of Rydberg atoms, which play an important role in quantum information and quantum computation, the theoretical and applied research of Rydberg atoms have become the hot spots of scientific research in recent years. With the large polarizability of Rydberg atoms, even a small electric field could cause a considerable electric dipole moment, resulting in a strong dipole-dipole interaction between Rydberg atoms. The multiple excitations of the Rydberg states are strongly inhibited because of the strong dipole interaction between atoms within a mesoscopic interaction (blockade) region. We call this phenomenon the dipole blockade effect. The dipole blockade effect makes it possible to build single-photon quantum devices, implement quantum gates, generate quantum entanglement, and simulate many-body quantum problems, etc. A Rydberg atomic ensemble in the same blockade region can be regarded as a superatom. In the same way, if these atoms trapped in two optical dipole traps, each sub-ensemble can be considered as a sub-superatom which is closely related to the superatom. According to the fact that two Rydberg sub-superatoms can be strongly correlated due to sharing no more than one excited Rydberg atom, we study correlated collective excitation and quantum entanglement between two Rydberg sub-superatoms in a steady state. With the superatom model, the problem of exponentially increasing system size with the number of atoms can be circumvented to a certain extent in studying many-body physics. By solving the two-body Lindblad’s master equation accurately, we obtain the analytical expressions for the collective excitation probabilities of the two sub-superatoms, and the concurrence measuring the bipartite entanglement between them. Our results show that they are all sensitive to the number of atoms in each Rydberg superatom: the bigger (including more atoms) the Rydberg superatom, the higher the collective Rydberg excitation probability is. And that the maximally entangled state can only be obtained with two equal-sized Rydberg superatoms. When this condition is fulfilled, the mesoscopic entanglement can be generated by adding the number of atoms in each Rydberg superatom. This may provide an attractive platform for studying the quantum-classical correspondence and have potential promising applications in quantum information processing.
Abstract Quantum optics based on highly excited atoms, also known as Rydberg atoms, has cemented itself as a powerful platform for the manipulation of light at the few-photon level. The Rydberg blockade, resulting from the strong interaction between individual Rydberg atoms, can turn a large ensemble of atoms into a system which collectively resembles a single two-level emitter, a so-called Rydberg superatom. The coupling of this artificial emitter to a driving photonic mode is collectively enhanced by Rydberg interactions, enabling strong coherent coupling at the few-photon level in free-space. The exquisite level of control achievable through this has already demonstrated its utility in applications of quantum computing and information processing. Here, we review the derivation of the collective coupling between a Rydberg superatom and a single light mode and discuss the similarity of this free-space setup to waveguide quantum electrodynamics systems of quantum emitters coupled to photonic waveguides. We also briefly review applications of Rydberg superatoms to quantum optics such as single-photon generation and single-photon subtraction.