Owing to the unique physical characteristics of Rydberg atoms, which play an important role in quantum information and quantum computation, the theoretical and applied research of Rydberg atoms have become the hot spots of scientific research in recent years. With the large polarizability of Rydberg atoms, even a small electric field could cause a considerable electric dipole moment, resulting in a strong dipole-dipole interaction between Rydberg atoms. The multiple excitations of the Rydberg states are strongly inhibited because of the strong dipole interaction between atoms within a mesoscopic interaction (blockade) region. We call this phenomenon the dipole blockade effect. The dipole blockade effect makes it possible to build single-photon quantum devices, implement quantum gates, generate quantum entanglement, and simulate many-body quantum problems, etc. A Rydberg atomic ensemble in the same blockade region can be regarded as a superatom. In the same way, if these atoms trapped in two optical dipole traps, each sub-ensemble can be considered as a sub-superatom which is closely related to the superatom. According to the fact that two Rydberg sub-superatoms can be strongly correlated due to sharing no more than one excited Rydberg atom, we study correlated collective excitation and quantum entanglement between two Rydberg sub-superatoms in a steady state. With the superatom model, the problem of exponentially increasing system size with the number of atoms can be circumvented to a certain extent in studying many-body physics. By solving the two-body Lindblad’s master equation accurately, we obtain the analytical expressions for the collective excitation probabilities of the two sub-superatoms, and the concurrence measuring the bipartite entanglement between them. Our results show that they are all sensitive to the number of atoms in each Rydberg superatom: the bigger (including more atoms) the Rydberg superatom, the higher the collective Rydberg excitation probability is. And that the maximally entangled state can only be obtained with two equal-sized Rydberg superatoms. When this condition is fulfilled, the mesoscopic entanglement can be generated by adding the number of atoms in each Rydberg superatom. This may provide an attractive platform for studying the quantum-classical correspondence and have potential promising applications in quantum information processing.
Owing to the unique physical characteristics of Rydberg atoms, which play an important role in quantum information and quantum computation, the theoretical and applied research of Rydberg atoms have become the hot spots of scientific research in recent years. With the large polarizability of Rydberg atoms, even a small electric field could cause a considerable electric dipole moment, resulting in a strong dipole-dipole interaction between Rydberg atoms. The multiple excitations of the Rydberg states are strongly inhibited because of the strong dipole interaction between atoms within a mesoscopic interaction (blockade) region. We call this phenomenon the dipole blockade effect. The dipole blockade effect makes it possible to build single-photon quantum devices, implement quantum gates, generate quantum entanglement, and simulate many-body quantum problems, etc. A Rydberg atomic ensemble in the same blockade region can be regarded as a superatom. In the same way, if these atoms trapped in two optical dipole traps, each sub-ensemble can be considered as a sub-superatom which is closely related to the superatom. According to the fact that two Rydberg sub-superatoms can be strongly correlated due to sharing no more than one excited Rydberg atom, we study correlated collective excitation and quantum entanglement between two Rydberg sub-superatoms in a steady state. With the superatom model, the problem of exponentially increasing system size with the number of atoms can be circumvented to a certain extent in studying many-body physics. By solving the two-body Lindblad’s master equation accurately, we obtain the analytical expressions for the collective excitation probabilities of the two sub-superatoms, and the concurrence measuring the bipartite entanglement between them. Our results show that they are all sensitive to the number of atoms in each Rydberg superatom: the bigger (including more atoms) the Rydberg superatom, the higher the collective Rydberg excitation probability is. And that the maximally entangled state can only be obtained with two equal-sized Rydberg superatoms. When this condition is fulfilled, the mesoscopic entanglement can be generated by adding the number of atoms in each Rydberg superatom. This may provide an attractive platform for studying the quantum-classical correspondence and have potential promising applications in quantum information processing.
Based on the dipole blockade effect and with the aid of the superatom (SA) model, we propose a scheme to investigate the correlated evolution of two Rydberg sub-superatoms (SSAs), formed by two spatially separated atomic Rydberg sub-ensembles but in the same blockade region. Starting from the pure separable states, we investigate the in-phase or anti-phase correlated dynamics and explore how two Rydberg SSAs entangle with each other mediated by a single Rydberg excitation. Starting from the entangled states, we discuss the robustness of the system against decoherence induced by the dephasing rate. Our results show that both the correlated evolution of two Rydberg SSAs and their collective-state entanglement are usually sensitive to the number of each Rydberg SSA. This allows us to coherently manipulate the Rydberg ensemble over long distances from the single-quantum level to the mesoscopic level by changing the number of atoms. Furthermore, the method for dividing an SA into two SSAs and obtaining their spin operators without any approximation can be readily generalized to the case of many SSAs. It may have potential promising applications in quantum information processing and provide an attractive platform to study the quantum-classical correspondence, many-body physics and so on.
Owing to the long lifetime of Rydberg atom, easy to operate and easy to control the interaction between Rydberg atoms, Rydberg atom has attracted considerable attention in quantum information and quantum optics fields. Specially, the anti-blockade effect, as a physical resource, can be used to implement various tasks in quantum information processing. Based on the rigid dipole blockade, an ensemble of two-level Rydberg atoms trapped in three magneto-optical traps can be regarded as a superatom. Based on the superatom model, the in-phase and anti-phase dynamics of the three-body Rydberg superatoms are studied by adjusting the numbers of atoms, and the W state and two kinds of maximal entangled states are generated simultaneously. Our work has great potential applications in coherent manipulation and quantum information processing.The numerical simulations are performed based on the superatom model and thereby the formidable obstacle that the Hilbert space dimension grows exponentially with the particle number increasing can be completely removed. As a result, the quantum control and quantum entanglement can be achieved from the single-quanta level to the mesoscopic level.
Since the establishment of quantum mechanics, quantum entanglement has become one of the most important realms in quantum physics. On the one hand, it reflects some of the most fascinating features, such as quantum coherence, probability and non-locality and so on. On the other hand, it proves to be an indispensable resource of quantum information processing and quantum computation, which is considered to greatly promote the development of human science and technology. In the past decades, inspired by advances in quantum information theory and quantum physics, people have been searching for suitable systems with great enthusiasm to prepare the robust and manipulable quantum entanglement. Recently, Rydberg atoms have been considered to be a good candidate for many quantum information and quantum computation tasks. Compared with general neutral atoms, Rydberg atoms with large principal quantum number have several advantages in the quantum information and computation service. Firstly, they have finite lifetimes much larger than general neutral atoms, which indicates that the long-time entanglement between Rydberg atoms can be achieved. Secondly, due to the high-excitation level, Rydberg-excitation atoms have long-ranged dipole-dipole interaction much stronger than ground state atoms. This strong atomic interaction leads to the so-called blockade effect: when one atom is excited to Rydberg level, the excitation of the neighboring atoms will be strictly suppressed due to the energy shift induced by the strong atomic interaction. On the contrast, if the energy shift is compensated for by the detuning between the energy levels and the driven laser field, these atoms can be excited with higher probability simultaneously. These effects imply that Rydberg atoms provide an excellent platform for investigating the quantum information and quantum computation process, and many important achievements based on them have been achieved. Encouraged by these researches on entanglement and Rydberg atoms, in this paper, we study the steady-state and transient dynamical properties of two-body entanglement and the Rydberg-excitation properties in a dilute gas of Rydberg atoms, which can be represented by a tetrahedrally arranged interacting four-atom model. By solving numerically the master equation of four atoms involving Rydberg level, we investigate the higher-order Rydberg excitations and bipartite entanglement, which is estimated by concurrence. Our results show that the bipartite entanglement can only achieve its maximal value in the strongest dipole blockade regime rather than anti-blockade one (the high-order Rydberg excitations). Furthermore, the physical essence of quantum entanglement is analyzed theoretically in relevant regimes. Our work can naturally extend to more complicated atomic space structures, and might be treated as a good platform for fulfilling many quantum information tasks by employing the quantum entanglement.
Quantum information is a rapidly developing field that merges the principles of quantum mechanics with information theory to explore new ways of processing and transmitting information. Qubits, which utilize superposition and entanglement, offer the potential for exponentially faster computation and secure communication methods that are fundamentally different from classical systems. This thesis contributes to the future of quantum information by studying two key platforms using neutral atoms: atomic arrays and atomic ensembles. It summarizes essential theoretical and experimental methods in the field and discusses key findings. To achieve entanglement among atomic qubits, Rydberg interactions are utilized, with two main effects discussed in this thesis. The Rydberg blockade effect is introduced where atoms trapped in an ensemble can form a two-level superatom. A state-insensitive optical lattice is used to achieve long coherence time for both the ground and Rydberg states. Long-lived Rabi oscillations and Ramsey interference are reported to demonstrate the collective enhancement of √N in a superatom. Furthermore, Rydberg dephasing is separated from Rydberg blockade and is investigated as a method to generate single photons from multiply excited states. This thesis presents both theoretical models and temporal evolution measurements of Rydberg dephasing from an initially unentangled Rydberg spinwave into an entangled single photon state. Additionally, this thesis examines the collective atomic dipole moment of a superatom, ⟨E⟩. Theoretical and experimental work are conducted to study the dipole moment when the phase-matched emission is combined with a coherent field in a homodyne detection method. This work advances our understanding of Rydberg interactions and collective dipole moments, contributing to the rapidly developing field of quantum information. The goal is to pave the way for the next era of quantum information through collaborative efforts and innovative research.
Highly excited Rydberg states, neutral atomic states with one or more electrons promoted to states of large principal quantum number n are now commonly used for producing quantum entanglement. This is facilitated through the "Rydberg Blockade" effect where the presence of a single Rydberg atom blocks excitation of further atoms in a surrounding mesoscopic volume due to strong atom-atom interactions induced by the large dipole moments associated with Rydberg atoms. In this work, we report the first observation of this phenomenon in a hot atomic beam using very high n, n ~300 - 500, strontium nF Rydberg states. Inside the blockaded volume (size around 0.1mm), the Rydberg number distribution is sub-Poissonian. However, as predicted by theoretical calculations, due to the anisotropic nature of the atom-atom interactions, the blockade is incomplete. However, the blockade effect is sufficiently strong to enable detailed study of few-body atom-atom interactions and of entanglement. Doubly-excited Rydberg states having a pair of electrons excited to high lying energy levels are typically difficult to create and are short lived because of "autoionization" resulting from electron-electron scattering. Strontium Rydberg atoms are used to study this scattering and we demonstrate an efficient mechanism to eliminate "autoionization" pointing to the production of long-lived strongly correlated two-electron-excited atomic states.
Abstract Quantum optics based on highly excited atoms, also known as Rydberg atoms, has cemented itself as a powerful platform for the manipulation of light at the few-photon level. The Rydberg blockade, resulting from the strong interaction between individual Rydberg atoms, can turn a large ensemble of atoms into a system which collectively resembles a single two-level emitter, a so-called Rydberg superatom. The coupling of this artificial emitter to a driving photonic mode is collectively enhanced by Rydberg interactions, enabling strong coherent coupling at the few-photon level in free-space. The exquisite level of control achievable through this has already demonstrated its utility in applications of quantum computing and information processing. Here, we review the derivation of the collective coupling between a Rydberg superatom and a single light mode and discuss the similarity of this free-space setup to waveguide quantum electrodynamics systems of quantum emitters coupled to photonic waveguides. We also briefly review applications of Rydberg superatoms to quantum optics such as single-photon generation and single-photon subtraction.