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arXiv:2504.05021 · Physical Review Letters

Entangling Two Rydberg Superatoms via Heralded Storage

Zi-Ye An, Bo-Wei Lu, Jun Li, Chao-Wei Yang, Li Li, Xiao‐Hui Bao, Jian-Wei Pan

Published May 27, 2025• 6 citations
arXivHTMLPDF

Abstract

Heralded storage of photons is crucial for advancing quantum networks. Previous realizations have primarily relied on single atoms strongly coupled to optical cavities. In this work, we present the experimental realization of heralded storage using a Rydberg superatom, a mesoscopic atomic ensemble operating in the strong blockade regime. In our approach, an input photon is initially stored in the superatom via electromagnetically induced transparency. Subsequently, a second photon is emitted conditioned on the success of the first photon's storage. Because of the collectively enhanced interaction, both the storage and the emission of the herald photon can be rather efficient in principle. As a demonstration of this technique, we use it to entangle two remote Rydberg superatoms. This method obviates the need for an intermediate node, which is commonly employed in traditional interference-based remote entanglement schemes. Our results showcase the potential of performing cavity-QED-like experiments with Rydberg superatoms. This work opens pathways for numerous applications in quantum networks and linear optical quantum computing.

DOI
10.1103/cmpn-jfqr

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Heralded storage of photons is crucial for advancing quantum networks. Previous realizations have primarily relied on single atoms strongly coupled to optical cavities. In this work, we present the experimental realization of heralded storage using a Rydberg superatom, a mesoscopic atomic ensemble operating in the strong blockade regime. In our approach, an input photon is initially stored in the superatom via electromagnetically induced transparency. Subsequently, a second photon is emitted conditioned on the success of the first photon's storage. Because of the collectively enhanced interaction, both the storage and the emission of the herald photon can be rather efficient in principle. As a demonstration of this technique, we use it to entangle two remote Rydberg superatoms. This method obviates the need for an intermediate node, which is commonly employed in traditional interference-based remote entanglement schemes. Our results showcase the potential of performing cavity-QED-like experiments with Rydberg superatoms. This work opens pathways for numerous applications in quantum networks and linear optical quantum computing.
Remote entanglement of matter qubits plays an important role in quantum networks and quantum repeater. Collective excitations generated via Rydberg blockade in an atomic ensemble-known as Rydberg superatoms-are promising candidates due to collectively enhanced atom-photon coupling and Rydberg-enabled nonlinearity. Here, we experimentally realize remote entanglement between two Rydberg superatoms via single-photon interference. The two setups are separated by 3 m and linked with two 20-m fibers, operated with independent control lasers. We verify that the entanglement generated is free from high-order excitation noise that is a key drawback in the traditional Duan-Lukin-Cirac-Zoller scheme. This Letter paves the way for entangling long-distance separated Rydberg superatoms at a high rate, as the success probability of a single-photon-based entangling scheme scales with the square root of the channel transmittance.
With Rydberg dipole interactions, a mesoscopic atomic ensemble becomes a superatom that behaves like a single atom but couples collectively with photons. It is potentially a strong candidate as a qubit in quantum information science, especially for quantum networks. In this paper, we report a cavity-enhanced single-photon interface for a Rydberg superatom and demonstrate deterministic qubit readout via a photon burst. We make use of a low-finesse ring cavity to enhance the atom–photon interaction and obtain in-fiber single-photon generation efficiency of 44%. Harnessing the dipole interaction between two Rydberg levels, we may create either a sequence of multiple single photons or nothing, conditioned on an initial qubit state. We achieve a measurement fidelity of 93.0% in 4.8 µs. Our work complements the experimental toolbox of harnessing Rydberg superatoms for quantum information applications.
With Rydberg dipole interactions, a mesoscopic atomic ensemble may behave like a two-level single atom, resulting in the so-called picture of superatom. It is in potential a strong candidate as a qubit in quantum information science, especially for efficient coupling with single photons via collective enhancement that is essential for building quantum internet to connect remote quantum computers. Previously, preliminary studies have been carried out in demonstrating basic concept of Rydberg superatom, a single-photon source, and entanglement with a single photon, etc. While a crucial element of single-shot qubit measurement is still missing. Here we realize the deterministic measurement of a superatom qubit via photon burst in a single shot. We make use of a low-finesse ring cavity to enhance the atom-photon interaction and obtain an in-fiber retrieval efficiency of 44%. Harnessing dipole interaction between two Rydberg levels, we may either create a sequence of multiple single photons or nothing, conditioned on the initial qubit state. We achieve a single-shot measurement fidelity of 93.2% in 4.8 us. Our work complements the experimental toolbox of harnessing Rydberg superatom for quantum information applications.
We demonstrate a new approach for creating deterministic photon-photon interactions for optical quantum engineering, based on a single-ended medium-finesse optical cavity containing a mesoscopic atomic ensemble. This ensemble is made transparent by a laser beam mapping intracavity photons into Rydberg polaritons. The transparency vanishes when the cloud, acting as a single collective two-level "superatom" with an enhanced coupling to light, is driven from the ground to a Rydberg state. We observe collectively-enhanced Rabi oscillations between these states, optically discriminate them in a single shot with a 95% effciency, and show that a change between the two internal states of the superatom induces a π phase rotation on the light reflected off of the cavity. These ingredients form a complete set of tools for implementing deterministic photonic entangling gates and for generating highly non-classical light without the need for a low-volume high-finesse cavity.
We discuss electromagnetically induced transparency in a cold ensemble of atoms optically excited to the Rydberg states. Strong dipole-dipole or van der Waals interactions between the atomic Rydberg states translate into large nonlocal nonlinearities for a propagating probe field. In the case of weak quantum fields, this can be used to attain a conditional phase shift of π between pairs of single photons realizing a deterministic photonic phase gate. For stronger fields, long-range interactions between the atoms constrain the medium to behave as a collection of superatoms, each comprising a blockade volume that can accommodate at most one Rydberg excitation. The propagation of a probe field is affected by its two-photon correlations within the blockade distance, which are strongly damped due to low saturation threshold of the superatoms. Our calculations reproduce and interpret the results of recent experiments.
We present a complete protocol for cavity-free quantum networking based on collective enhancement in Rydberg atom ensembles. The scheme combines Rydberg blockade, collectively enhanced light--matter coupling, and phase-matched directional emission to remove the need for optical cavities while retaining efficiencies comparable to cavity-assisted interfaces. The protocol proceeds in three steps: (i)~local control--ensemble entanglement generated by Rydberg blockade with gate fidelity Fgate≈99.93%F_{\mathrm{gate}}\approx 99.93\%Fgate​≈99.93%; (ii)~atom--photon conversion through Raman emission from an oblate spheroidal ensemble, yielding directional emission efficiency ηdir≈73%η_{\mathrm{dir}}\approx 73\%ηdir​≈73% and single-node efficiency ηnode≈40%η_{\mathrm{node}}\approx 40\%ηnode​≈40%; and (iii)~remote atom--atom entanglement via Hong--Ou--Mandel interference, producing Bell states with fidelity F>97.5%F>97.5\%F>97.5%. Incorporating quantum memories allows up to M≈100M\approx 100M≈100 retry attempts within a coherence time T2>100 μsT_2>100\,μ\mathrm{s}T2​>100μs, enabling entanglement generation rates of approximately 4 kHz4\,\mathrm{kHz}4kHz over a 20~km separation. Collectively enhanced Rydberg ensembles thus provide a practical, cavity-free interface for scalable distributed quantum computing and secure quantum communication.