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Journal of Physics D Applied Physics

Fabrication of micro-superconducting quantum interference devices based on nano laser direct writing

Wenqian Liu, Shuo Xiang, Yicong Huang, Wenzhi Zhang, Shangqing Li, Enhua Chen, Chaoyun Zhang, Xiaoliang Wang, Haohui Zhang, Songling Xiao, Tuo Zhang, Hao Zhang, Yu Liu, Jianxin Lin

Published Aug 13, 2025• 2 citations
Publisher

Abstract

Abstract We propose the fabrication of micro-superconducting quantum interference devices via nano laser direct writing (NLDW). A 20 nm thick Nb film with a critical transition temperature of 9.2 K was deposited on a silicon substrate by sputtering, and nanopatterning was performed with NLDW. After optimizing parameters such as the laser pulse width and power, we investigated the electrical performance of SQUIDs by varying the laser power between 245 mW and 270 mW in 5 mW steps. Experimentally, the voltage–flux (V–Φ) characteristics of micro SQUIDs exhibited typical periodic modulation, confirming the Josephson effect and magnetic flux quantization effect based on the NLDW process. The noise spectral density measurements of SQUID fabricated with laser power of 265 mW achieved a white noise level of 3 μ Φ 0 /Hz 1 / 2 , demonstrating comparable flux noise sensitivity compared to electron beam and ion beam fabrication processes. Furthermore, the devices retained stable superconducting and electrical performance after 101 days, illustrating excellent long-term stability. To some extent, the NLDW shows the potential to perform micro-nanopatterning of superconducting devices efficiently and cost-effectively, as well as an avenue for conducting nanoscale thermal engineering on superconducting devices for basic science research.

DOI
10.1088/1361-6463/adfae9

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Abstract We propose the fabrication of micro-superconducting quantum interference devices via nano laser direct writing (NLDW). A 20 nm thick Nb film with a critical transition temperature of 9.2 K was deposited on a silicon substrate by sputtering, and nanopatterning was performed with NLDW. After optimizing parameters such as the laser pulse width and power, we investigated the electrical performance of SQUIDs by varying the laser power between 245 mW and 270 mW in 5 mW steps. Experimentally, the voltage–flux (V–Φ) characteristics of micro SQUIDs exhibited typical periodic modulation, confirming the Josephson effect and magnetic flux quantization effect based on the NLDW process. The noise spectral density measurements of SQUID fabricated with laser power of 265 mW achieved a white noise level of 3 μ Φ 0 /Hz 1 / 2 , demonstrating comparable flux noise sensitivity compared to electron beam and ion beam fabrication processes. Furthermore, the devices retained stable superconducting and electrical performance after 101 days, illustrating excellent long-term stability. To some extent, the NLDW shows the potential to perform micro-nanopatterning of superconducting devices efficiently and cost-effectively, as well as an avenue for conducting nanoscale thermal engineering on superconducting devices for basic science research.
Thermal effects serve as universal stimuli for material transformation, capable of inducing processes, such as crystallization, evaporation, and melting in various materials. In this paper, we propose an efficient and cost-effective fabrication method based on nano-laser direct writing (NLDW) technology for the fabrication of Nb constricted junctions and superconducting quantum interference devices induced by thermal effects. By narrowing the spacing between laser paths step by step, the I–V characteristics of constricted junctions can be continuously adjusted from collective Cooper pair transport to Josephson junction behavior. Additionally, the heat-affected zones induced by laser irradiation were characterized by heat transfer simulations and electrical transport behavior. Furthermore, the flux noise spectral density of a patterned superconducting quantum interference device based on NLDW is 2.8μΦ0/Hz1/2 in the white noise range, which exhibits comparable performance to devices based on traditional ion beam or electron beam etching processes. In this case, this technique could provide a reliable and reproducible pathway for scaling up the fabrication of superconducting quantum circuits, as well as an avenue to conduct nanoscale thermal engineering in superconducting materials research for basic science.
We report on nanopatterned YBa2Cu3O7-δ (YBCO) direct current superconducting quantum interference devices (SQUIDs) based on grain boundary Josephson junctions. The nanoSQUIDs are fabricated by epitaxial growth of 120 nm-thick films of the high-transition temperature cuprate superconductor YBCO via pulsed laser deposition on MgO bicrystal substrates with 24° misorientation angle, followed by sputtering of dAu = 65 nm thick Au. Nanopatterning is performed by Ga focused ion beam (FIB) milling. The SQUID performance is comparable to devices on SrTiO3 (STO), as demonstrated by electric transport and noise measurements at 4.2 K. MgO has orders of magnitude smaller dielectric permittivity than STO; i.e., one may avoid Au as a resistively shunting layer to reduce the intrinsic thermal flux noise of the nanoSQUIDs. However, we find that the Au layer is important for avoiding degradation during FIB milling. Hence, we compare devices with different dAu produced by thinning the Au layer via Ar ion milling after FIB patterning. We find that the reduction of dAu yields an increase in junction resistance, however at the expense of a reduction of the critical current and increase in SQUID inductance. This results in an estimated thermal flux noise that is almost independent of dAu. However, for two devices on MgO with 65 nm-thick Au, we find an order of magnitude lower low-frequency excess noise as compared to nanoSQUIDs on STO or those on MgO with reduced dAu. For one of those devices we obtain with bias-reversal readout ultra-low flux noise of ∼175 nΦ0 Hz-1/2 down to ∼10 Hz.
Science and industry demand ever more sensitive measurements on ever smaller systems, as exemplified by spintronics, nanoelectromechanical system, and spin-based quantum information processing, where single electronic spin detection poses a grand challenge. Superconducting quantum interference devices (SQUIDs) have yet to be effectively applied to nanoscale measurements. Here, we show that a simple bilayer deposition route, combining photolithography with focused ion beam patterning, produces high performance nanoscale SQUIDs. We present results of noise measurements on these nanoSQUIDs which correspond to a magnetic flux sensitivity of around 0.2μΦ0∕Hz1∕2. This represents one of the lowest noise values achieved for a SQUID device operating above 1K.
A superconducting quantum interference device (SQUID) miniaturized into the nanoscale is promising in the inductive detection of a single electron spin. A nano-SQUID with a strong spin coupling coefficient, a low flux noise, and a wide working magnetic field range is highly desired in a single spin resonance measurement. Nano-SQUIDs with Dayem bridge junctions excel in a high working field range and in the direct coupling from spins to the bridge. However, the common planar structure of nano-SQUIDs is known for problems such as a shallow flux modulation depth and a troublesome hysteresis in current–voltage curves. Here, we developed a fabrication process for creating three-dimensional (3-D) niobium (Nb) nano-SQUIDs with nanobridge junctions that can be tuned independently. Characterization of the device shows up to 45.9% modulation depth with a reversible current–voltage curve. Owning to the large modulation depth, the measured flux noise is as low as 0.34 μΦ 0 /Hz 1/2 . The working field range of the SQUID is greater than 0.5 T parallel to the SQUID plane. We believe that 3-D Nb nano-SQUIDs provide a promising step toward effective single-spin inductive detection.
We report on the fabrication and characterization of micrometer-sized superconducting quantum interference devices (SQUIDs) based on nanoscale vanadium/copper/vanadium Josephson weak links. Magnetically driven quantum interference patterns have been measured for temperatures in the 0.24–2 K range. As DC SQUIDs, these devices obtain flux-to-voltage transfer function values as high as 450 μV/Φ0 leading to promising magnetic flux resolution ΦN<3 μΦ0/Hz, being here limited by the room temperature preamplification stage. Significant improvement in the flux noise performance figures is expected with the adoption of cryogenic preamplification. The presented devices are suitable for operation as small-area SQUIDs at sub-Kelvin temperature, but their design can also be upscaled to include input coils enabling their use as sensitive magnetometers via the adoption of optimized electronic readout stages based on flux feedback schemes.
Nano-Superconducting Quantum Interference Devices (nano-SQUIDs) are usually fabricated from a single layer of either Nb or Al. We describe here a simple method for fabricating suspended nano-bridges in Nb/Al thin-film bilayers. We use these suspended bridges, which act as Josephson weak links, to fabricate nano-SQUIDs which show critical current oscillations at temperatures up to 1.5 K and magnetic flux densities up to over 20 mT. These nano-SQUIDs exhibit flux modulation depths intermediate between all-Al and all-Nb devices, with some of the desirable characteristics of both. The suspended geometry is attractive for magnetic single nanoparticle measurements.