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Известия Российской академии наук Серия физическая

Spatial coherence of exciton-polaritoniс Bose‒Einstein condensates

N. V. Kuznetsova, Денис В. Макаров, Norayr Armenovich Asriyan, Andrei A. Elistratov, Yu. E. Lozovik

Published Jun 15, 2024• 0 citations
Publisher

Abstract

Dynamics of exciton-polariton Bose‒Einstein condensate in an optical microcavity is considered. A novel version of stochastic Gross‒Pitaevsky equation for description of condensate evolution under non-Markovian interaction with environment is proposed. Using the proposed version, analysis of condensate dynamics for various temperatures is carried out. The phase transition from a homogeneous to fragmented condensate state near temperature of 15 K is found. This phase transition is accompanied by drop of condensate density and decrease of correlation length. It is found that correlation length oscillates with time for the temperature of 10 K. The results obtained indicate the necessity to take into account non-Markovianity of condensate interaction with the excitonic reservoir.

DOI
10.31857/s0367676524060074

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Dynamics of exciton-polariton Bose‒Einstein condensate in an optical microcavity is considered. A novel version of stochastic Gross‒Pitaevsky equation for description of condensate evolution under non-Markovian interaction with environment is proposed. Using the proposed version, analysis of condensate dynamics for various temperatures is carried out. The phase transition from a homogeneous to fragmented condensate state near temperature of 15 K is found. This phase transition is accompanied by drop of condensate density and decrease of correlation length. It is found that correlation length oscillates with time for the temperature of 10 K. The results obtained indicate the necessity to take into account non-Markovianity of condensate interaction with the excitonic reservoir.
Abstract The dynamics of an exciton–polariton Bose–Einstein condensate in an optical microcavity was considered. A novel version of the stochastic Gross–Pitaevskii equation was proposed to describe the condensate evolution under the non-Markovian interaction with the environment. The proposed version was used to analyze the condensate dynamics at various temperatures. The phase transition from the homogeneous to the fragmented state of the condensate near a temperature of 15 K was detected. This phase transition is accompanied by a sharp drop in the condensate density and a decrease in the correlation length. It was found that, at a temperature of 10 K, the correlation length oscillates with time. The results obtained indicated the necessity to take into account the non-Markovianity of the condensate interaction with the excitonic reservoir.
Bose-Einstein condensate of exciton polaritons in a semiconductor microcavity is a macroscopically populated coherent quantum state subject to concurrent pumping and decay. Debates about the fundamental nature of the condensed phase in this open quantum system still persist. Here, we gain a new insight into the spontaneous condensation process by imaging long-lifetime exciton polaritons in a high-quality inorganic microcavity in the single-shot optical excitation regime, without averaging over multiple condensate realisations. In this highly non-stationary regime, a condensate is strongly influenced by the `hot' incoherent reservoir, and reservoir depletion is critical for the transition to the ground energy and momentum state. Condensates formed by more photonic exciton polaritons exhibit dramatic reservoir-induced density filamentation and shot-to-shot fluctuations. In contrast, condensates of more excitonic quasiparticles display smooth density and are second-order coherent. Our observations show that the single-shot measurements offer a unique opportunity to study formation of macroscopic phase coherence during a quantum phase transition in a solid state system.
We study the behavior of exciton polaritons in an optical microcavity with an embedded semiconductor quantum well. We use a two-component exciton-photon approach formulated in terms of path integral formalism. In order to describe spatial distributions of the exciton and photon condensate densities, the two coupled equations of the Gross-Pitaevskii type are derived. For a homogeneous system, we find the noncondensate photon and exciton spectra, calculate the coefficients of transformation from the exciton-photon basis to the lower-upper polariton basis, and obtain the exciton and photon occupation numbers of the lower and upper polariton branches for nonzero temperatures. For an inhomogeneous system, the set of coupled equations of the Bogoliubov--de Gennes type is derived. The equations govern the spectra and spatial distributions of noncondensate photons and excitons.
We study the relation between the models commonly used to describe the dynamics of nonresonantly pumped exciton-polariton condensates, namely the ones described by the complex Ginzburg-Landau equation, and by the open-dissipative Gross-Pitaevskii equation including a separate equation for the reservoir density. In particular, we focus on the validity of the adiabatic approximation and small density fluctuations approximation that allow one to reduce the coupled condensate-reservoir dynamics to a single partial differential equation. We find that the adiabatic approximation consists of three independent analytical conditions that have to be fulfilled simultaneously. By investigating stochastic versions of the two corresponding models, we verify that the breakdown of these approximations can lead to discrepancies in correlation lengths and distributions of fluctuations. Additionally, we consider the phase diffusion and number fluctuations of a condensate in a box, and show that self-consistent description requires treatment beyond the typical Bogoliubov approximation.