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Measurement

Suppression of spin-exchange relaxation in Bell-Bloom magnetometer

Chi Fang, Liwei Jiang, Jiali Liu, Yuanqiang Chen, Jun Zhu, Qi Shao, Yuntian Zou, Min Xiang, Wei Quan

Published Sep 10, 2024• 12 citations
Publisher
DOI
10.1016/j.measurement.2024.115695

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Spin-exchange collisions in hot vapors are generally regarded as a decoherence mechanism. In contrast, we show that linear and nonlinear spin-exchange coupling can lead to the generation of atomic coherence in a Bell-Bloom magnetometer. In particular, we theoretically and experimentally demonstrate that nonlinear spin-exchange coupling, acting in an analogous way to a wave-mixing mechanism, can create additional modes of coherent excitation which inherit the magnetic properties of the natural Larmor coherence. The generated coherences further couple via linear spin-exchange interaction, leading to an increase of the natural coherence lifetime of the system. Notably, the measurements are performed in a low-density caesium vapor and for nonzero magnetic field, outside the standard conditions for collisional coherence transfer. The strategies discussed are important for the development of spin-exchange coupling into a resource for an improved measurement platform based on room-temperature alkali-metal vapors.
The Bell-Bloom-type optically pumped atomic magnetometers are well suited for weak geomagnetic field detection. However, conventional single-beam pumping introduces an atomic spin polarization gradient, which limits the measurement accuracy and sensitivity. To address this issue, this paper proposes and experimentally demonstrates a Bell-Bloom-type rubidium FID magnetometer scheme integrating orthogonally polarized counter-propagating pumping and multi-pass probe detection. This design homogenizes the atomic spin polarization distribution and suppresses light shifts and power broadening effects induced by the pump beam. Meanwhile, the five-pass probe configuration significantly enhances the signal amplitude. Experimental results reveal that, compared with the traditional single-beam pumping and single-pass detection scheme, the proposed magnetometer achieves a remarkable improvement in magnetic field measurement accuracy, and the magnetic field sensitivity is improved from 18.9 pT/\sqrt{Hz} to 3.1 pT/\sqrt{Hz}. This work provides an effective technical approach and reference for optimizing the performance of atomic magnetometers and extending their applications in integrated arrays.