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Physica Scripta

Nonequilibrium spinor exciton-polariton condensates in a magnetic field

Ting-Wei Chen, Szu-Cheng Cheng

Published Feb 15, 2024• 1 citation
Publisher

Abstract

Abstract A complete-nonequilibrium model is proposed to investigate spinor exciton-polariton condensates (SEPCs) in a magnetic field. Due to the Zeeman splitting (ZS), the loss rates of two spin components in a magnetic field are distinct and affected by the magnetic field. Therefore, the individual spin component of a SEPC has its own threshold pump power. We investigate the ZS and degree of circular polarization of the SEPC as a function of the excitation power and magnetic field. Above both spin-dependent threshold pump powers, we find an increasing degree of circular polarization with the magnetic field and a quenching of the ZS below a critical strength of the magnetic field. The ZS of a SEPC shows a reverse sign and its magnitude is increasing significantly compared to the uncondensed exciton-polartion ZS. The effect of a magnetic field on excitation spectra of SEPCs are also investigated. We find that the excitation dispersions are Bogoliubov excitations if the pump power is low. The nonequilibrium fluctuations in a SEPC are reduced when a magnetic field is applied.

DOI
10.1088/1402-4896/ad29ca

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Abstract A complete-nonequilibrium model is proposed to investigate spinor exciton-polariton condensates (SEPCs) in a magnetic field. Due to the Zeeman splitting (ZS), the loss rates of two spin components in a magnetic field are distinct and affected by the magnetic field. Therefore, the individual spin component of a SEPC has its own threshold pump power. We investigate the ZS and degree of circular polarization of the SEPC as a function of the excitation power and magnetic field. Above both spin-dependent threshold pump powers, we find an increasing degree of circular polarization with the magnetic field and a quenching of the ZS below a critical strength of the magnetic field. The ZS of a SEPC shows a reverse sign and its magnitude is increasing significantly compared to the uncondensed exciton-polartion ZS. The effect of a magnetic field on excitation spectra of SEPCs are also investigated. We find that the excitation dispersions are Bogoliubov excitations if the pump power is low. The nonequilibrium fluctuations in a SEPC are reduced when a magnetic field is applied.
The effect of a magnetic field on a spinor exciton-polariton condensate has been investigated. A quenching of a polariton Zeeman splitting and an elliptical polarization of the condensate have been observed at low magnetic fields B<2 T. The effects are attributed to a competition between the magnetic field induced circular polarization buildup and the spin-anisotropic polariton-polariton interaction which favors a linear polarization. The sign of the circular polarization of the condensate emission at B<3 T is negative, suggesting that a dynamic condensation in the excited spin state rather than the ground spin state takes place in this magnetic field range. From about 2T on, the Zeeman splitting opens and from then on the slope of the circular polarization degree changes its sign. For magnetic fields larger than the 3 T, the upper spin state occupation is energetically suppressed and circularly polarized condensation takes place in the ground state.
The suppression of Zeeman energy splitting due to spin-dependent interactions (the spin Meissner effect) was predicted to occur within a Bose-Einstein condensate. We report a clear observation of this effect in semimagnetic microcavities which exhibit a giant Zeeman energy splitting between two spin-polarized polariton states as high as 2 meV and demonstrate that a partial suppression of the energy difference occurs already in the uncondensed phase in a striking similarity to the behavior of up-critical superconductors in the fluctuation-dominated regime. These observations are explained quantitatively by a kinetic model accounting for both the condensed and uncondensed polaritons and taking into account the nonequilibrium character of the system.
We theoretically investigate a spinor polariton condensate under nonresonant pumping, based on driven-dissipative Gross-Pitaevskii equations coupled to the rate equation of a spin-unpolarized reservoir. We find the homogeneous polariton condensate can transit from the spin-unpolarized phase, where it is linearly polarized, to the spin-polarized phase, where it is elliptically polarized, depending on the cross-spin versus same-spin interactions and the linear polarization splitting. In both phases, we study elementary excitations using Bogoliubov approach, in a regime where the decay rate of total exciton density in reservoir crosses over from the slow to the fast limit. Depending on reservoir parameters, the global-phase mode can be either diffusive or gapped. By contrast, the relative-phase mode always possesses a gapped energy, undamped in the spin-unpolarized phase but weakly damped in the spin-polarized phase. In the spin-unpolarized phase, both modes are linearly polarized despite pumping and decay. However, in the spin-polarized phase, the mode polarization can be significantly affected by the reservoir and depends strongly on the circular polarization degree of the condensate. Interestingly, we demonstrate that the ``ghost'' branch of the Bogoliubov spectrum of the relative-phase mode can be visualized in the photoluminescence emission, distinguishable from that of the global-phase mode and thus allowing for experimental observation, when the spinor polariton condensate is elliptically polarized.
Abstract The dependences of the exciton-polariton photoluminescence spectra on the intensity of optical excitation and external magnetic fields are investigated in cylindrical mesas based on high-quality microcavities. It was found that with an increase of the intensity of optical excitation above a certain threshold at sufficiently large magnetic field or with an increase of magnetic fields at constant optical excitation, the distribution of exciton-polaritons over Zeeman sublevels becomes substantially non-Boltzmannian.
We investigate the influence of transverse-electric–transverse-magnetic (TE–TM) splitting on the nonlinear response and bistability of resonantly driven spinor exciton-polaritons in a spatially homogeneous microcavity system. Using a coupled exciton–photon mean-field model, we find that TE–TM splitting significantly modifies the bistability threshold, hysteresis width, and spin composition of the steady states. In particular, TE–TM splitting counteracts the spin imbalance imposed by elliptically polarized pumping, leading to nearly equal populations of the two spin components and strongly suppressed degree of circular polarization in the steady state. The pump momentum plays a crucial role through its connection to the curvature of the lower polariton dispersion, resulting in distinct nonlinear regimes with different switching thresholds and dynamical responses. The intermediate branch within the hysteresis loop is unstable but may exhibit slow instability growth rates, giving rise to long-lived transient states. These results clarify how TE–TM splitting reshapes bistability and nonlinear spin dynamics in polariton systems and provide insight into the controlling polariton switching behavior through cavity anisotropy and pump parameters.