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International Meeting on Instabilities and Dynamics of Lasers and Nonlinear Optical Systems

Transverse Effects Self-Action Instabilities in the Simultaneous Propagation of Short Different-Wavelength Pulses in Three-Level Absorbers†

F.P. Mattarff, George R. Harrison, J. P. Babuel-Peyrissac, J. P. Marinier, C. Bardin

Published Jan 1, 1985• 0 citations
Publisher

Abstract

This paper is devoted to understanding the temporal synchronization of the two-color superfluorescence output powers. Following McCall and Feld et al., the monochromatic superfluorescence can be described in terms of a semi-classical propagational model that shares the same equations as Self-Induced Transparency (SIT). Thus it became important to understand double SIT that was discovered by McCall and Hahn (MH) to correctly interpret co-propagating beams with coherent exchange of energy and nonlinear phase evolution. A further motivation would be to elucidate pump and Stokes synchronization as well as pump depletion effect on Stokes buildup in Raman forward amplifier. In this work, we describe how the diffraction affects the longitudinal and transverse reshaping associated affects the simultaneous resonant propagation of two different-wavelength optical pulses in a three-level medium. The pulse lengths are shorter than any of the relaxation times, thus, the interaction is coherent. The material response has an inertial characteristic, which precludes its description with two instantaneous susceptibilities, and requires instead the density matrix formulism. A semi-classical formulism, as introduced by Konopnicki and Eberly (KE), is adopted in which two paraxial Maxwell field equations are closely intertwined in the generalized three-level Bloch equations.

DOI
10.1364/idlnos.1985.wd36

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This paper is devoted to understanding the temporal synchronization of the two-color superfluorescence output powers. Following McCall and Feld et al., the monochromatic superfluorescence can be described in terms of a semi-classical propagational model that shares the same equations as Self-Induced Transparency (SIT). Thus it became important to understand double SIT that was discovered by McCall and Hahn (MH) to correctly interpret co-propagating beams with coherent exchange of energy and nonlinear phase evolution. A further motivation would be to elucidate pump and Stokes synchronization as well as pump depletion effect on Stokes buildup in Raman forward amplifier. In this work, we describe how the diffraction affects the longitudinal and transverse reshaping associated affects the simultaneous resonant propagation of two different-wavelength optical pulses in a three-level medium. The pulse lengths are shorter than any of the relaxation times, thus, the interaction is coherent. The material response has an inertial characteristic, which precludes its description with two instantaneous susceptibilities, and requires instead the density matrix formulism. A semi-classical formulism, as introduced by Konopnicki and Eberly (KE), is adopted in which two paraxial Maxwell field equations are closely intertwined in the generalized three-level Bloch equations.
The phenomenon that describes the effect of a coherent medium response to an incident electric field, to which the medium is totally transparent and which undergoes lossless propagation, is known as self-induced transparency (SIT). SIT was first discovered by McCall and Hahn (1969) in the case of nondegenerate two-level atoms. Special solutions for the two-level system were found by Lamb (1971), while the initial value problem for the propagation of a pulse through a resonant two-level optical medium was solved by Inverse Scattering Transform (IST) in [1, 2]. It is possible to formulate the SIT equations in the framework of the IST also in the case of a three-level system, as in [3]. While the associated scattering problem is the same as for the coupled nonlinear Schrödinger equation, the time evolution depends on asymptotic values of the material polarizability envelopes and is highly non-trivial. This talk will address the solution of the initial value problem for the SIT equations for three level systems, for generic preparation of the medium, and
Using proven computational methods developed to efficiently treat transverse and longitudinal dynamic reshaping associated with single-stream propagation effects in cooperative light-matter interactions, a realistic superfluorescence (SF) theory was constructed in close collaboration with experimentalists. A semi-classical model based on the Maxwell-Bloch equa-tions (which rigorously encompasses diffraction, transverse density variations and inhomoge-neous broadening) is used. Furthermore, the medium initiation is stimulated by a coherent pulse of an area θ0 which varies radially, propagates along the rod axis and tips the indi-vidual Bloch vectors over an angle θ0 from its upright position. This effective initiation is treated in using either (a) an homogeneous average tipping angle or (b) instantaneous longitudinal and transverse fluctuations. The Cs datas are correctly simulated for the first time.* Important remark At this time, I wish to express my appreciation and give credit to Gibbs, McCall and Feld for their many contributions in the form of numerous relevant discussions, preparatory ana-lytical work and help in selecting details of realistic models based on their close contact with laboratory results. In addition, Dr Gibbs' participation in carrying the calculations accelerated the rate of progress in my research. Let me take this occasion to thank Dr. Gibbs, Dr. McCall and Dr. Feld for their energetic and enthousiastic collaboration.
A computer movie illustrating a rigorous multimode calculation of SF, St, Prb buildup in Raman studies is presented. This coherent copropagational study based on Maxwell-Bloch formalism1 includes phase and transverse variations, nonlinear asymmetric dispersion, pump spatial depletion, and time-dependent variations in population inversion density. Theλ scheme is selected so that the active transitions are optically thick for both the pump (α p l > 5) and the SF (α sf l > 35) pulses. This choice of Beer lengths, i.e., of oscillator strengths, insures that the two pulses never cease to overlap and optimizes the SF initially small signal growth. The pump interacts like a self-induced transparency while the SF, St, Prb evolves as a small-area in a two-level emitter which can be described as a nonlinear pendulum in the pane wave. For a given ratio of Beer lengths, distinct Fresnel numbers, atomic density numbers, small signal SF, St, Prb time-integrated energy stabilization or self-focusing may arise, as observed experimentally. For a sufficiently larger propagation distance, an asymptotic evolution of a quasisolitary nonhyperbolic-secant pulse of constant area is reported.
The coherent propagation of two optical short pulses through a resonant medium consisting of two three-level atoms in the configuration is investigated. A self-consisting analytical solution without steady state or adiabatic approximations is presented. The electric field in the model studied consists of two co-propagating plane waves, each of which is in near resonance with a transition in the absorber. The density matrix of two three level atoms is studied. Also, the reduced density matrices are stated. The present approach for the semiclassical treatment of resonant coherent interactions in three-level atoms represents a generalization of the Maxwell- Bloch equations for a two-level system. The Maxwell-Bloch equations reduced to the non-linear pendulum equation. The solution shows that the two pulses can propagate simultaneously without loss under some conditions about the pulses and the medium. The propagation of the two pulses through the medium without any constrains approves the self -induced transparency (SIT) phenomenon.
Analytic and numerical calculations for the propagational dependence of Rabi-Split resulting from a strong resonant pump and a coupled weak off-resonance probe are presented for a Lambda three-level atomic configuration. A semi-classical Maxwell-Bloch formulism was adopted for both the perturbational (using stationary phase and steepest descent asymptotic techniques) and the rigorous computational treatments. This calculation can be considered as a Double Self-Induced Transparency SIT' where the strong pump (multiple of 2n on-axis area) experiences coherent pulse break up, coherent self-focusing 2-4 and depletion as the weak probe (multiple of 0.02n area) cooperatively builds up. Different transition gain ratios (i.e., oscillator strength: p2w) are considered to insure that the weak probe does not get (a) delayed with respect to the pump or (b) get out of synchronization, and cease to overlap. The probe detuning can be as large as the input on-axis pump Rabi frequency. The interplay of nonlinear Raman gain action, dispersion and diffraction give rise concommitantly to a number of effects previously studied independently such as self-phase modulation, wave front encoding, transverse ring formation, self-focusing, quasi-trapping (when pump detuning is also allowed), and asymptotic three-level solitary waves.