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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Propagation Effects In Strong Pump-Weak Probe Coherent Interactions

F. P. Mattar

Published Nov 20, 1985• 1 citation
Publisher

Abstract

Analytic and numerical calculations for the propagational dependence of Rabi-Split resulting from a strong resonant pump and a coupled weak off-resonance probe are presented for a Lambda three-level atomic configuration. A semi-classical Maxwell-Bloch formulism was adopted for both the perturbational (using stationary phase and steepest descent asymptotic techniques) and the rigorous computational treatments. This calculation can be considered as a Double Self-Induced Transparency SIT' where the strong pump (multiple of 2n on-axis area) experiences coherent pulse break up, coherent self-focusing 2-4 and depletion as the weak probe (multiple of 0.02n area) cooperatively builds up. Different transition gain ratios (i.e., oscillator strength: p2w) are considered to insure that the weak probe does not get (a) delayed with respect to the pump or (b) get out of synchronization, and cease to overlap. The probe detuning can be as large as the input on-axis pump Rabi frequency. The interplay of nonlinear Raman gain action, dispersion and diffraction give rise concommitantly to a number of effects previously studied independently such as self-phase modulation, wave front encoding, transverse ring formation, self-focusing, quasi-trapping (when pump detuning is also allowed), and asymptotic three-level solitary waves.

DOI
10.1117/12.976172

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Analytic and numerical calculations for the propagational dependence of Rabi-Split resulting from a strong resonant pump and a coupled weak off-resonance probe are presented for a Lambda three-level atomic configuration. A semi-classical Maxwell-Bloch formulism was adopted for both the perturbational (using stationary phase and steepest descent asymptotic techniques) and the rigorous computational treatments. This calculation can be considered as a Double Self-Induced Transparency SIT' where the strong pump (multiple of 2n on-axis area) experiences coherent pulse break up, coherent self-focusing 2-4 and depletion as the weak probe (multiple of 0.02n area) cooperatively builds up. Different transition gain ratios (i.e., oscillator strength: p2w) are considered to insure that the weak probe does not get (a) delayed with respect to the pump or (b) get out of synchronization, and cease to overlap. The probe detuning can be as large as the input on-axis pump Rabi frequency. The interplay of nonlinear Raman gain action, dispersion and diffraction give rise concommitantly to a number of effects previously studied independently such as self-phase modulation, wave front encoding, transverse ring formation, self-focusing, quasi-trapping (when pump detuning is also allowed), and asymptotic three-level solitary waves.
In the domain of semiclassical formulation and for the Doppler-free atom–field interaction, we construct the optical Bloch equations involving an M-type six-level system coupled to two pump fields and a probe field. The response of the system is probed for different pump-induced transitions in double and triple-resonance situations. In order to obtain the coherent lineshapes (absorptive and dispersive), we use the usual perturbation method for obtaining the approximate analytical solutions to these coupled optical Bloch equations for the density matrix elements. The interferences between the probability amplitudes for different energy levels (dipole allowed and dipole forbidden) are taken care of. For off-resonance pump positions, the linewidths of the three probe transitions are insensitive to the pump Rabi frequencies. On the other hand, the shifts of the three resonance peaks are extremely sensitive to the pump Rabi frequencies. However, for on-resonance pump conditions, the sensitivities of pump Rabi frequencies on the linewidths of the resonance peaks and on the shifts of the resonance peak positions are opposite to those of their off-resonance counterparts. In particular, we have shown the asymmetric and symmetric Rabi splittings under different physical conditions, for non-zero and near-zero probe detuning, respectively. The Rabi splitting under triple-resonance conditions, significantly, modifies the dispersive lineshape at the centre of the absorption line. The two- and three-photon absorptions are also reported for different off-resonant pump positions.
The coherent frequency conversion between on-resonance pump and probe beams is examined in the physical situation where the medium nonlinearity balances the linear diffraction for each transition. Without diffraction neither soliton can occur. The paraxial-Maxwell Bloch formalism is adopted. To achieve optimally the energy transfer the pulse velocities must be equal to maintain maximum overlap throughout the propagation. The sequential evolution of probe soliton then pump soliton is reported in conjunction with pump depletion diffraction rigorously accounted for. Phase diagram of the pump and probe areas exhibit multi-value features.
A computer movie illustrating a rigorous multimode calculation of SF, St, Prb buildup in Raman studies is presented. This coherent copropagational study based on Maxwell-Bloch formalism1 includes phase and transverse variations, nonlinear asymmetric dispersion, pump spatial depletion, and time-dependent variations in population inversion density. Theλ scheme is selected so that the active transitions are optically thick for both the pump (α p l > 5) and the SF (α sf l > 35) pulses. This choice of Beer lengths, i.e., of oscillator strengths, insures that the two pulses never cease to overlap and optimizes the SF initially small signal growth. The pump interacts like a self-induced transparency while the SF, St, Prb evolves as a small-area in a two-level emitter which can be described as a nonlinear pendulum in the pane wave. For a given ratio of Beer lengths, distinct Fresnel numbers, atomic density numbers, small signal SF, St, Prb time-integrated energy stabilization or self-focusing may arise, as observed experimentally. For a sufficiently larger propagation distance, an asymptotic evolution of a quasisolitary nonhyperbolic-secant pulse of constant area is reported.
We study the interaction of the medium composed of three-level atoms in A configuration interacting with two laser fields: weak probe field and strong control field. The probe field enters the medium under a certain angle, and it is initially in the form of the spatial soliton, while the control field is periodically modulated. The system of optical Bloch equations is analytically solved in the stationary regime by the perturbation method in order to obtain linear and third-order nonlinear susceptibility of the medium with respect to the probe field. After a straightforward algebraic procedure, using the approximation of the slow-varying field envelope, the nonlinear Schrödinger equation for the probe field is obtained. It is numerically solved by applying the spectral Fourier split-step method. It is found that, for properly chosen values of the probe and control field detunings and control Rabi frequency, the probe field behaves as a solitary wave whose direction does not depend on the incident angle. Moreover, the regime consisting of Bloch-like oscillations can be identified. The simulation is performed by choosing the corresponding levels of Mg atoms.
This paper is devoted to understanding the temporal synchronization of the two-color superfluorescence output powers. Following McCall and Feld et al., the monochromatic superfluorescence can be described in terms of a semi-classical propagational model that shares the same equations as Self-Induced Transparency (SIT). Thus it became important to understand double SIT that was discovered by McCall and Hahn (MH) to correctly interpret co-propagating beams with coherent exchange of energy and nonlinear phase evolution. A further motivation would be to elucidate pump and Stokes synchronization as well as pump depletion effect on Stokes buildup in Raman forward amplifier. In this work, we describe how the diffraction affects the longitudinal and transverse reshaping associated affects the simultaneous resonant propagation of two different-wavelength optical pulses in a three-level medium. The pulse lengths are shorter than any of the relaxation times, thus, the interaction is coherent. The material response has an inertial characteristic, which precludes its description with two instantaneous susceptibilities, and requires instead the density matrix formulism. A semi-classical formulism, as introduced by Konopnicki and Eberly (KE), is adopted in which two paraxial Maxwell field equations are closely intertwined in the generalized three-level Bloch equations.
We treat theoretically the two-pulse plane-wave propagation problem associated with the stimulated Raman process. A strong pump pulse and a weak probe pulse interact self-consistently during mutual propagation through a medium in the three-level lambda configuration. We treat the pulse interaction fully coherently, but take initially incoherent mixed ground states to describe the medium. We present analytic pulse envelope solutions to the nonlinear evolution equations, and then test them numerically. We show that the entire process can be interpreted consistently as a three-regime evolution, in which the first and last regimes display behavior quantitatively the same as self-induced transparency. They are connected through a Raman transfer process in the intermediate regime.