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Scientific Reports

Spatially structured multi-wave-mixing induced nonlinear absorption and gain in a semiconductor quantum well

Pradipta Panchadhyayee, Bibhas Kumar Dutta

Published Dec 26, 2022• 6 citations
Publisher

Abstract

We have studied two-dimensional absorption and gain spectrum in an asymmetric semiconductor triple-coupled-quantum-well (TCQW) nanostructure. Four subband transitions are coupled by using four coherent fields in a close-loop configuration to introduce cross-Kerr effect and four-wave-mixing (FWM) induced nonlinearity in achieving nonlinear absorption and gain profiles. Position-dependent absorption and gain are obtained by applying one, or two coherent fields in a variety of standing wave configurations including superposed field configuration in the standing-wave regime. In addition to the control parameters like Rabi frequency and detuning, the specialty of the model is to employ double-controlled spatial phase-coherence guided by the FWM-induced phase and the phases introduced by the standing wave formation. Our results highlight the high-precision electron localization in spatial domain. The evolution of spatially modulated gain without inversion may be a substitute for obtaining gain from a traditional quantum cascade laser. The importance of the present work is to find its application in designing electro-optic modulators in semiconductor nanostructures in near future.

DOI
10.1038/s41598-022-26140-y

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We have studied two-dimensional absorption and gain spectrum in an asymmetric semiconductor triple-coupled-quantum-well (TCQW) nanostructure. Four subband transitions are coupled by using four coherent fields in a close-loop configuration to introduce cross-Kerr effect and four-wave-mixing (FWM) induced nonlinearity in achieving nonlinear absorption and gain profiles. Position-dependent absorption and gain are obtained by applying one, or two coherent fields in a variety of standing wave configurations including superposed field configuration in the standing-wave regime. In addition to the control parameters like Rabi frequency and detuning, the specialty of the model is to employ double-controlled spatial phase-coherence guided by the FWM-induced phase and the phases introduced by the standing wave formation. Our results highlight the high-precision electron localization in spatial domain. The evolution of spatially modulated gain without inversion may be a substitute for obtaining gain from a traditional quantum cascade laser. The importance of the present work is to find its application in designing electro-optic modulators in semiconductor nanostructures in near future.
We propose a scheme to generate spatially dependent four-wave mixing (FWM) in an asymmetric semiconductor three-coupled-quantum-well nanostructure. By adjusting the detuning of the control field, one can effectively manipulate the FWM output field. Specifically, the vortex phase of the FWM field can be modulated. The detailed explanations based on the dispersion relation are given, which are in good agreement with our results. Furthermore, we perform the interference between the FWM field and the same-frequency Gaussian beam. Our results show that the interference patterns can also be modulated via the detuning of the control field, which may provide a way to observe helical phase modulation via the intensity measurement. This work may be useful for investigating the nonlinear optical phenomena based on orbital angular momentum light.
We propose an atomic model in close-loop configuration, which exhibits controllable symmetric and asymmetric evolution of significantly enhanced diffraction peaks of the weak probe beam in an opto-atomic grating at far-field regime. Such results are obtained by the linear and nonlinear modulation of the intensities of the diffraction peaks as a result of multi-wave-mixing-induced modification of spatially modulated coherence in a closed four-level atomic system. Novelty of the results lies in predicting the diffraction pattern with uniform peak height due to the dominance of the amplitude part of the grating-transfer-function at the condition of exact atom-field resonance, which is unique to the present model. Efficacy of the present scheme is to apply it in producing nonlinear light generated by four-wave-mixing-induced control of spatially modulated coherence effect. The work also finds its importance for its applicability in the field of all-optical devices.
We propose a multi-field-coupled atomic model that exhibits controllable symmetricsymmetricsymmetric and asymmetricasymmetricasymmetric evolution of significantly enhanced diffraction peaks in an opto-atomic grating at far-field regime. Such results are obtained by the linear and nonlinear modulation of the intensities of the diffraction peaks as a result of multi-wave-mixing-induced modification of spatially modulated coherence in a closed four-level atomic system. Novelty of the results lies in predicting super symmetric alignment of the diffraction peaks due to the dominance of the amplitude part of the grating-transfer-function at the condition of exact atom-field resonance, which is unique to the present model. Efficacy of the present scheme is to apply it in producing nonlinear light generated by four-wave-mixing-induced control of spatially modulated coherence effect. The work also finds its importance for its applicability in the field of high-precision atomic lithography.
Abstract In this article, we present an alternative excitation scheme for the study of optical responses of the probe field in a five-level semiconductor coupled quantum wells (CQWs). It is shown that in the linear case, our study reveals the formation of double and triple electromagnetically induced transparency (EIT) windows for the suitable values of Rabi-frequency of the control fields, while the linear dispersion is also tuned from anomalous to normal and vice versa within small range of detuning. Interestingly, we find that by properly adjusting the appropriate values of control field detunings, the behaviour of optical absorption and transparency is found to be asymmetric in nature. In addition, we also found that due to quantum coherence, nonlinear dispersion, specifically Kerr nonlinearity is dramatically enhanced with nearly vanishing linear absorption under EIT. The Kerr nonlinearity in the present scheme is identified to be very large ( ∼10−13 m2 V−2\:\sim{10}^{-13}\:{m}^{2}\:{V}^{-2}∼10−13m2V−2) in the mid IR range ( λ p=4.74  μ m\:{\lambda\:}_{p}=4.74\:\:\mu\:mλp​=4.74μm), which can be very useful for the investigation of several nonlinear phenomena at low light intensity in CQWs. The results of the investigations may have potential applications in optical switching devices at low powers, quantum information processing and many more in solid-state laser based system.
A four level ladder scheme is employed for the realization of slow light large Kerr nonlinear indices in an asymmetric semiconductor three-coupled-quantum-well (TCQW) structure based on intersubband transitions. It is shown that a giant Kerr nonlinearity accompanied with negligible loss can be achieved by properly tuning the intensity of the control fields. A dressed state analysis is given to explain the origin of such a transparency based on slow light enhanced Kerr nonlinearity in this solid medium. In addition, we show that the three-photon detuning plays the important role in enhancing the third-order nonlinearity of the TCQW medium, and may provide new possibilities for technological applications in nonlinear optics and optical switching.
We investigate the two-dimensional (2D) position-dependent probe absorption in a triple semiconductor quantum well (SQW) structure driven coherently by two orthogonal standing-wave fields. Under weak probe field approximation and utilizing the density matrix approach, an analytical solution is presented for the probe linear susceptibility which clarifies directly the spatial-dependent nature of the probe absorption. Then, the distribution of probe absorption in 2D is numerically explored. It is found that 2D absorption spectra are very sensitive to the intensity and frequency detuning of standing-wave fields which can result in various 2D localization structures in one period of standing waves in the x – y plane.