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Journal de physique

Relaxation nucléaire de 3He dans un champ magnétique inhomogène

Valérie Lefèvre-Seguin, Pierre-Jean Nacher, Franck Laloë

Published Jan 1, 1982• 0 citations
Publisher

Abstract

This article gives a theoretical study of the effects of weak magnetic field gradients on the spin relaxation of a dilute atomic gas. The theory is valid for low or moderate values of the field (the relevant correlation time of the gas is then the diffusion time across the container) as well as for high fields (the intercollision time then plays the most important role). Quantum effects due to particle indistinguishability are included. No consequences of the divergence of the atomic mean free path in a polarized gas at zero temperature are found, in contrast to the situation for viscosity and heat conductivity. On the other hand, substantial effects due to « identical spin rotation effects » are predicted.

DOI
10.1051/jphys:01982004305073700/pdf

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Relaxation nucléaire de 3He ↑ dans un champ magnétique inhomogène

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On présente dans cet article une étude théorique de la relaxation de spin d'un gaz atomique dilué, produite par un gradient de champ magnétique de faible intensité. La théorie est valide à la fois en champ faible ou modéré (cas où le temps de corrélation du gaz qui joue un rôle est le temps de diffusion dans son récipient) et en champ fort (c'est alors le temps entre collisions qui joue le rôle essentiel). Elle tient compte des effets quantiques d'indiscernabilité des atomes. Si les effets de divergence du libre parcours moyen dans un gaz polarisé à température nulle ne jouent ici aucun rôle, contrairement à ce qui se produit pour la viscosité par exemple, les effets de « rotation des spins identiques » peuvent être importants.

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The general results obtained in the preceding article are applied to the study of transport phenomena in a spin polarized gas at low temperatures, with particular emphasis on the particle indistinguishability effects in collisions. The effects of the nuclear orientation M are treated exactly (no M expansion). First, a simple theory of spin diffusion is presented and the response of the gas to a spin orientation gradient is calculated. The spin coherences and their evolution due to the « identical-spin rotation effect » are taken into account; it is found that they can play an important role, especially in the low temperature limit. The hydrodynamic equations of evolution of M are non-linear and anisotropic. Particle indistinguishability effects give an oscillatory character to the evolution of the transverse components of M (spin oscillations). Then, a more elaborate variational method is used to study the coupling between spin diffusion and heat conduction. This effect is, again, a sheer consequence of quantum interference phenomena introduced by particle indistinguishability. Finally, isotopic mixtures of 3He and 4He are considered In addition to coupling between isotopic diffusion and heat conduction, which exists for classical systems, quantum collision effects introduce a coupling between these two modes and spin diffusion.

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Longitudinal Relaxation Time in a Degenerate, Polarized Fermi Gas

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The longitudinal relaxation time T$\\sb1$ is calculated for a dilute Fermi gas. We include the possibility of arbitrary degrees of polarization P, and uniform external magnetic fields. At low temperatures T$\\sb1$ is proportional to T$\\sp{-2}$ for the unpolarized gas in agreement with earlier calculations. For a polarized system in zero applied field the separation between up and down Fermi spheres provides an open channel in phase space for spin flipping processes. As temperature is reduced to zero T$\\sb1$ levels off and approaches a constant value which depends sensitively on P, leading to much smaller values of T$\\sb1$ than in the unpolarized case. For relaxation in a uniform external field H, Zeeman energy conservation during spin flipping interactions essentially shifts the location of the T$\\sp{-2}$ behavior from zero polarization to the polarization P(H) which would be produced in equilibrium with the external field H. When the initial polarization of the system is different from P(H), T$\\sb1$ again approaches a constant value which is equally sensitive to the initial polarization as temperature is reduced to zero. We apply our calculations to the case of dilute $\\sp3$He-HeII solutions. We also consider the calculation of density dependent corrections to T$\\sb1$ for unpolarized, or weakly polarized $\\sp3$He-HeII using the long wavelength limit of the Bardeen-Baym-Pines interaction as a form for the spin independent part of the $\\sp3$He-$\\sp3$He interaction. Owing to the positive sign of the antisymmetric Landau parameter $\\rm F\\sbsp{o}{a}$ in dilute $\\sp3$He-HeII Fermi Liquid interactions act to screen the magnetic dipole interactions which cause relaxation. To lowest order in density we find that the relaxation rate 1/T$\\sb1$ is reduced by factor $\\rm (1 - 3F\\sbsp{o}{a})$ which compares favorably with recent calculations of T$\\sb1$ for pure $\\sp3$He.

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Spin diffusion in Fermi gases

Georg M. Bruun

We examine spin diffusion in a two-component homogeneous Fermi gas in the normal phase. Using a variational approach, analytical results are presented for the spin diffusion coefficient and the related spin relaxation time as a function of temperature and interaction strength. For low temperatures, strong correlation effects are included through the Landau parameters, which we extract from Monte Carlo results. We show that the spin diffusion coefficient has a minimum for a temperature somewhat below the Fermi temperature with a value that approaches the quantum limit ∼ℏ/ m in the unitarity regime, where m is the particle mass. Finally, we derive a value for the low-temperature shear viscosity in the normal phase from the Landau parameters.

arXiv:1012.1607•New Journal of Physics•Mar 16, 2011•48 citations
This article gives a theoretical study of the effects of weak magnetic field gradients on the spin relaxation of a dilute atomic gas. The theory is valid for low or moderate values of the field (the relevant correlation time of the gas is then the diffusion time across the container) as well as for high fields (the intercollision time then plays the most important role). Quantum effects due to particle indistinguishability are included. No consequences of the divergence of the atomic mean free path in a polarized gas at zero temperature are found, in contrast to the situation for viscosity and heat conductivity. On the other hand, substantial effects due to « identical spin rotation effects » are predicted.
On présente dans cet article une étude théorique de la relaxation de spin d'un gaz atomique dilué, produite par un gradient de champ magnétique de faible intensité. La théorie est valide à la fois en champ faible ou modéré (cas où le temps de corrélation du gaz qui joue un rôle est le temps de diffusion dans son récipient) et en champ fort (c'est alors le temps entre collisions qui joue le rôle essentiel). Elle tient compte des effets quantiques d'indiscernabilité des atomes. Si les effets de divergence du libre parcours moyen dans un gaz polarisé à température nulle ne jouent ici aucun rôle, contrairement à ce qui se produit pour la viscosité par exemple, les effets de « rotation des spins identiques » peuvent être importants.
The general results obtained in the preceding article are applied to the study of transport phenomena in a spin polarized gas at low temperatures, with particular emphasis on the particle indistinguishability effects in collisions. The effects of the nuclear orientation M are treated exactly (no M expansion). First, a simple theory of spin diffusion is presented and the response of the gas to a spin orientation gradient is calculated. The spin coherences and their evolution due to the « identical-spin rotation effect » are taken into account; it is found that they can play an important role, especially in the low temperature limit. The hydrodynamic equations of evolution of M are non-linear and anisotropic. Particle indistinguishability effects give an oscillatory character to the evolution of the transverse components of M (spin oscillations). Then, a more elaborate variational method is used to study the coupling between spin diffusion and heat conduction. This effect is, again, a sheer consequence of quantum interference phenomena introduced by particle indistinguishability. Finally, isotopic mixtures of 3He and 4He are considered In addition to coupling between isotopic diffusion and heat conduction, which exists for classical systems, quantum collision effects introduce a coupling between these two modes and spin diffusion.
A theory of magnetotransport phenomena in low-density paramagnetic systems at low temperature is proposed. The main contentions are based on considering a dissipation mechanism due to the inelastic scattering of paramagnetic particles with transverse collective spin fluctuations. In the presence of an external magnetic field and in the low-momentum limit the corresponding cross section may be very large. Theoretical estimates are in good agreement with recent indirect measurements of intrabeam scattering for cooled H atoms. The extra scattering channel results in a drastic reduction in the mean free path and, consequently, a decrease in the thermal conductivity and viscosity, in contrast to previous theories. In the case of degenerate Fermi systems, the calculations yield quite different temperature dependencies compared with those given by the Fermi-liquid approach. Application of the theory to gaseous H\ensuremath{\downarrow}, $^{3}\mathrm{\ensuremath{\uparrow}}$, and dilute $^{3}\mathrm{\ensuremath{-}}^{4}$He mixtures are briefly discussed, and it is shown that the thermal conductivity and viscosity of gaseous H\ensuremath{\downarrow} under common conditions are expected to be roughly 102{10}^{2}102 times less than the normal gas-kinetic values.
We carried out experiments on a spin polarized 3He- 4He mixture with 3He concentration x 3 = 6.26 × 10−4, and on pure 3He liquid. Spin polarization affects the transport properties of these Fermi systems. The effect on momentum transport was studied by using a vibrating-wire viscometer to measure viscosity of the 3He-4He mixture over the temperature range 6.09 mK–100 mK in 7.96 T and 1.00 T magnetic fields. A large viscosity increase was observed upon application of the 7.96 T magnetic field for temperature T < TF(TF = 19.5 mK is the Fermi temperature). The observed viscosity is in very good agreement with theoretical calculations for a dilute Fermi gas by Jeon and Mullin [1988, 1989] and Mullin and Jeon [1992]. The polarization effect on spin transport was investigated by measuring the transverse diffusion coefficient D ⊥ in pure 3He liquid at saturated vapor pressure and at 15.85 bar over the temperature range 4.5 mK–159 mK in a 7.96 T magnetic field. We used a pulsed NMR spin echo technique in a field gradient of 16.0 G/cm to do the measurements and fits to the Leggett equations [1970] to obtain D⊥. For T < 20 mK, we found D⊥ is less than measured in earlier experiments at lower magnetic fields. D⊥ does not increase with decreasing temperature as 1/T2, but appears to approach a constant as T → 0 while it is expected that the longitudinal spin diffusion coefficient D∥ ∝ 1/ T2. This is called spin diffusion anisotropy and it was observed for the first time in our 3He liquid experiments. The anisotropy temperature we determined for 3He liquid was Ta = 16.4 ± 2.2 mK at saturated vapor pressure and in a 7.96 T magnetic field. The transverse spin diffusion in 3 He results agree qualitatively with theories proposed by Meyerovich and Musaeflan [1992, 1994]. They also agree qualitatively with theories proposed by Golosov and Ruckenstein [1995, 1998] by extrapolation of the dilute theory to a strongly interacting system.
The longitudinal relaxation time Tsb1\\sb1sb1 is calculated for a dilute Fermi gas. We include the possibility of arbitrary degrees of polarization P, and uniform external magnetic fields. At low temperatures Tsb1\\sb1sb1 is proportional to Tsp−2\\sp{-2}sp−2 for the unpolarized gas in agreement with earlier calculations. For a polarized system in zero applied field the separation between up and down Fermi spheres provides an open channel in phase space for spin flipping processes. As temperature is reduced to zero Tsb1\\sb1sb1 levels off and approaches a constant value which depends sensitively on P, leading to much smaller values of Tsb1\\sb1sb1 than in the unpolarized case. For relaxation in a uniform external field H, Zeeman energy conservation during spin flipping interactions essentially shifts the location of the Tsp−2\\sp{-2}sp−2 behavior from zero polarization to the polarization P(H) which would be produced in equilibrium with the external field H. When the initial polarization of the system is different from P(H), Tsb1\\sb1sb1 again approaches a constant value which is equally sensitive to the initial polarization as temperature is reduced to zero. We apply our calculations to the case of dilute sp3\\sp3sp3He-HeII solutions. We also consider the calculation of density dependent corrections to Tsb1\\sb1sb1 for unpolarized, or weakly polarized sp3\\sp3sp3He-HeII using the long wavelength limit of the Bardeen-Baym-Pines interaction as a form for the spin independent part of the sp3\\sp3sp3He-sp3\\sp3sp3He interaction. Owing to the positive sign of the antisymmetric Landau parameter rmFsbspoa\\rm F\\sbsp{o}{a}rmFsbspoa in dilute sp3\\sp3sp3He-HeII Fermi Liquid interactions act to screen the magnetic dipole interactions which cause relaxation. To lowest order in density we find that the relaxation rate 1/Tsb1\\sb1sb1 is reduced by factor rm(1−3Fsbspoa)\\rm (1 - 3F\\sbsp{o}{a})rm(1−3Fsbspoa) which compares favorably with recent calculations of Tsb1\\sb1sb1 for pure sp3\\sp3sp3He.
We examine spin diffusion in a two-component homogeneous Fermi gas in the normal phase. Using a variational approach, analytical results are presented for the spin diffusion coefficient and the related spin relaxation time as a function of temperature and interaction strength. For low temperatures, strong correlation effects are included through the Landau parameters, which we extract from Monte Carlo results. We show that the spin diffusion coefficient has a minimum for a temperature somewhat below the Fermi temperature with a value that approaches the quantum limit ∼ℏ/ m in the unitarity regime, where m is the particle mass. Finally, we derive a value for the low-temperature shear viscosity in the normal phase from the Landau parameters.