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Physical review. B, Condensed matter

Magnetotransport effects in paramagnetic gases

Eugene P. Bashkin

Published Dec 1, 1991• 6 citations
Publisher

Abstract

A theory of magnetotransport phenomena in low-density paramagnetic systems at low temperature is proposed. The main contentions are based on considering a dissipation mechanism due to the inelastic scattering of paramagnetic particles with transverse collective spin fluctuations. In the presence of an external magnetic field and in the low-momentum limit the corresponding cross section may be very large. Theoretical estimates are in good agreement with recent indirect measurements of intrabeam scattering for cooled H atoms. The extra scattering channel results in a drastic reduction in the mean free path and, consequently, a decrease in the thermal conductivity and viscosity, in contrast to previous theories. In the case of degenerate Fermi systems, the calculations yield quite different temperature dependencies compared with those given by the Fermi-liquid approach. Application of the theory to gaseous H\ensuremath{\downarrow}, $^{3}\mathrm{\ensuremath{\uparrow}}$, and dilute $^{3}\mathrm{\ensuremath{-}}^{4}$He mixtures are briefly discussed, and it is shown that the thermal conductivity and viscosity of gaseous H\ensuremath{\downarrow} under common conditions are expected to be roughly ${10}^{2}$ times less than the normal gas-kinetic values.

DOI
10.1103/physrevb.44.12440

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Longitudinal Relaxation Time in a Degenerate, Polarized Fermi Gas

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The longitudinal relaxation time T$\\sb1$ is calculated for a dilute Fermi gas. We include the possibility of arbitrary degrees of polarization P, and uniform external magnetic fields. At low temperatures T$\\sb1$ is proportional to T$\\sp{-2}$ for the unpolarized gas in agreement with earlier calculations. For a polarized system in zero applied field the separation between up and down Fermi spheres provides an open channel in phase space for spin flipping processes. As temperature is reduced to zero T$\\sb1$ levels off and approaches a constant value which depends sensitively on P, leading to much smaller values of T$\\sb1$ than in the unpolarized case. For relaxation in a uniform external field H, Zeeman energy conservation during spin flipping interactions essentially shifts the location of the T$\\sp{-2}$ behavior from zero polarization to the polarization P(H) which would be produced in equilibrium with the external field H. When the initial polarization of the system is different from P(H), T$\\sb1$ again approaches a constant value which is equally sensitive to the initial polarization as temperature is reduced to zero. We apply our calculations to the case of dilute $\\sp3$He-HeII solutions. We also consider the calculation of density dependent corrections to T$\\sb1$ for unpolarized, or weakly polarized $\\sp3$He-HeII using the long wavelength limit of the Bardeen-Baym-Pines interaction as a form for the spin independent part of the $\\sp3$He-$\\sp3$He interaction. Owing to the positive sign of the antisymmetric Landau parameter $\\rm F\\sbsp{o}{a}$ in dilute $\\sp3$He-HeII Fermi Liquid interactions act to screen the magnetic dipole interactions which cause relaxation. To lowest order in density we find that the relaxation rate 1/T$\\sb1$ is reduced by factor $\\rm (1 - 3F\\sbsp{o}{a})$ which compares favorably with recent calculations of T$\\sb1$ for pure $\\sp3$He.

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Relaxation nucléaire de 3He dans un champ magnétique inhomogène

Valérie Lefèvre-Seguin, Pierre-Jean Nacher, Franck Laloë

This article gives a theoretical study of the effects of weak magnetic field gradients on the spin relaxation of a dilute atomic gas. The theory is valid for low or moderate values of the field (the relevant correlation time of the gas is then the diffusion time across the container) as well as for high fields (the intercollision time then plays the most important role). Quantum effects due to particle indistinguishability are included. No consequences of the divergence of the atomic mean free path in a polarized gas at zero temperature are found, in contrast to the situation for viscosity and heat conductivity. On the other hand, substantial effects due to « identical spin rotation effects » are predicted.

Journal de physique•Jan 1, 1982•0 citations
A theory of magnetotransport phenomena in low-density paramagnetic systems at low temperature is proposed. The main contentions are based on considering a dissipation mechanism due to the inelastic scattering of paramagnetic particles with transverse collective spin fluctuations. In the presence of an external magnetic field and in the low-momentum limit the corresponding cross section may be very large. Theoretical estimates are in good agreement with recent indirect measurements of intrabeam scattering for cooled H atoms. The extra scattering channel results in a drastic reduction in the mean free path and, consequently, a decrease in the thermal conductivity and viscosity, in contrast to previous theories. In the case of degenerate Fermi systems, the calculations yield quite different temperature dependencies compared with those given by the Fermi-liquid approach. Application of the theory to gaseous H\ensuremath{\downarrow}, 3\ensuremath↑^{3}\mathrm{\ensuremath{\uparrow}}3\ensuremath↑, and dilute 3\ensuremath−4^{3}\mathrm{\ensuremath{-}}^{4}3\ensuremath−4He mixtures are briefly discussed, and it is shown that the thermal conductivity and viscosity of gaseous H\ensuremath{\downarrow} under common conditions are expected to be roughly 102{10}^{2}102 times less than the normal gas-kinetic values.
We derive the linearized spin dynamics for paramagnetic quantum liquids. In these systems, the existence of quantum-mechanical exchange in the presence of (an externally induced) broken symmetry in spin space gives rise to a coherent precession of the spins damped by diffusion. Such collective oscillations occur as a result of the precession of the spin current about a macroscopic local exchange field generated either by an external polarizing magnetic field (as in dilute nondegenerate spin-polarized gases) or by the long-lived nonequilibrium polarization (as in degenerate Fermi liquids). We use a unified approach based on the Kadanoff-Baym formulation of the kinetic equations to describe these phenomena. The connection between strongly and weakly interacting paramagnetic systems is made obvious by considering two special cases: (1) a weakly interacting spin-polarized quantum gas and (2) a parametrization of strongly correlated degenerate Fermi liquids in terms a weakly interacting gas of ``quasiparticles.'' Transport coefficients are calculated with a novel method which may be generalizable to systems with no translational invariance.
We carried out experiments on a spin polarized 3He- 4He mixture with 3He concentration x 3 = 6.26 × 10−4, and on pure 3He liquid. Spin polarization affects the transport properties of these Fermi systems. The effect on momentum transport was studied by using a vibrating-wire viscometer to measure viscosity of the 3He-4He mixture over the temperature range 6.09 mK–100 mK in 7.96 T and 1.00 T magnetic fields. A large viscosity increase was observed upon application of the 7.96 T magnetic field for temperature T < TF(TF = 19.5 mK is the Fermi temperature). The observed viscosity is in very good agreement with theoretical calculations for a dilute Fermi gas by Jeon and Mullin [1988, 1989] and Mullin and Jeon [1992]. The polarization effect on spin transport was investigated by measuring the transverse diffusion coefficient D ⊥ in pure 3He liquid at saturated vapor pressure and at 15.85 bar over the temperature range 4.5 mK–159 mK in a 7.96 T magnetic field. We used a pulsed NMR spin echo technique in a field gradient of 16.0 G/cm to do the measurements and fits to the Leggett equations [1970] to obtain D⊥. For T < 20 mK, we found D⊥ is less than measured in earlier experiments at lower magnetic fields. D⊥ does not increase with decreasing temperature as 1/T2, but appears to approach a constant as T → 0 while it is expected that the longitudinal spin diffusion coefficient D∥ ∝ 1/ T2. This is called spin diffusion anisotropy and it was observed for the first time in our 3He liquid experiments. The anisotropy temperature we determined for 3He liquid was Ta = 16.4 ± 2.2 mK at saturated vapor pressure and in a 7.96 T magnetic field. The transverse spin diffusion in 3 He results agree qualitatively with theories proposed by Meyerovich and Musaeflan [1992, 1994]. They also agree qualitatively with theories proposed by Golosov and Ruckenstein [1995, 1998] by extrapolation of the dilute theory to a strongly interacting system.
We compute spin diffusion in a dilute Fermi gas at arbitrary temperature, polarization, and strong interaction in the normal phase using kinetic theory. While the longitudinal spin diffusivity ${D}_{\ensuremath{\parallel}}$ depends weakly on polarization and diverges for small temperatures, the transverse spin diffusivity ${D}_{\ensuremath{\perp}}$ has a strong polarization dependence and approaches a finite value for $T\ensuremath{\rightarrow}0$ in the Fermi liquid phase. For a 3D unitary Fermi gas at infinite scattering length, the diffusivities reach a minimum near the quantum limit of diffusion $\ensuremath{\hbar}/m$ in the quantum degenerate regime and are strongly suppressed by medium scattering, and we discuss the importance of the spin-rotation effect. In two dimensions, ${D}_{\ensuremath{\perp}}$ attains a minimum at strong coupling $\ensuremath{-}1\ensuremath{\lesssim}\mathrm{ln}({k}_{F}{a}_{2D})\ensuremath{\lesssim}1$ and reaches ${D}_{\ensuremath{\perp}}\ensuremath{\sim}0.2...\phantom{\rule{0.16em}{0ex}}0.3\phantom{\rule{0.16em}{0ex}}\ensuremath{\hbar}/m$ at large polarization. These values are consistent with recent measurements of two-dimensional ultracold atomic gases in the strong coupling regime.
We present a finite temperature calculation of the transverse spin-diffusion coefficient ${D}_{\ensuremath{\perp}}$ in a dilute degenerate Fermi gas, in the presence of a small external magnetic field HHH. While the longitudinal diffusion coefficient displays the conventional Fermi-liquid dependence, ${D}_{\ensuremath{\parallel}}\ensuremath{\propto}{T}^{\ensuremath{-}2}$, the behavior of ${D}_{\ensuremath{\perp}}$ shows three separate regimes: (a) ${D}_{\ensuremath{\perp}}\ensuremath{\sim}{H}^{\ensuremath{-}2}$ for $T\ensuremath{\ll}H$, (b) ${D}_{\ensuremath{\perp}}\ensuremath{\sim}{T}^{\ensuremath{-}2}$, $\frac{{D}_{\ensuremath{\perp}}}{{D}_{\ensuremath{\parallel}}}\ensuremath{\ne}1$ for $T\ensuremath{\gg}H$ and large spin-rotation parameter $\ensuremath{\xi}\ensuremath{\gg}1$, and (c) ${D}_{\ensuremath{\perp}}={D}_{\ensuremath{\parallel}}\ensuremath{\propto}{T}^{\ensuremath{-}2}$ for $T\ensuremath{\gg}H$ and $\ensuremath{\xi}\ensuremath{\ll}1$. Our results are qualitatively consistent with the experimental data in weakly spin-polarized 3He^{3}\mathrm{He}3He and 3He^{3}\mathrm{He}3He- 4He^{4}\mathrm{He}4He mixtures.
The longitudinal relaxation time Tsb1\\sb1sb1 is calculated for a dilute Fermi gas. We include the possibility of arbitrary degrees of polarization P, and uniform external magnetic fields. At low temperatures Tsb1\\sb1sb1 is proportional to Tsp−2\\sp{-2}sp−2 for the unpolarized gas in agreement with earlier calculations. For a polarized system in zero applied field the separation between up and down Fermi spheres provides an open channel in phase space for spin flipping processes. As temperature is reduced to zero Tsb1\\sb1sb1 levels off and approaches a constant value which depends sensitively on P, leading to much smaller values of Tsb1\\sb1sb1 than in the unpolarized case. For relaxation in a uniform external field H, Zeeman energy conservation during spin flipping interactions essentially shifts the location of the Tsp−2\\sp{-2}sp−2 behavior from zero polarization to the polarization P(H) which would be produced in equilibrium with the external field H. When the initial polarization of the system is different from P(H), Tsb1\\sb1sb1 again approaches a constant value which is equally sensitive to the initial polarization as temperature is reduced to zero. We apply our calculations to the case of dilute sp3\\sp3sp3He-HeII solutions. We also consider the calculation of density dependent corrections to Tsb1\\sb1sb1 for unpolarized, or weakly polarized sp3\\sp3sp3He-HeII using the long wavelength limit of the Bardeen-Baym-Pines interaction as a form for the spin independent part of the sp3\\sp3sp3He-sp3\\sp3sp3He interaction. Owing to the positive sign of the antisymmetric Landau parameter rmFsbspoa\\rm F\\sbsp{o}{a}rmFsbspoa in dilute sp3\\sp3sp3He-HeII Fermi Liquid interactions act to screen the magnetic dipole interactions which cause relaxation. To lowest order in density we find that the relaxation rate 1/Tsb1\\sb1sb1 is reduced by factor rm(1−3Fsbspoa)\\rm (1 - 3F\\sbsp{o}{a})rm(1−3Fsbspoa) which compares favorably with recent calculations of Tsb1\\sb1sb1 for pure sp3\\sp3sp3He.
This article gives a theoretical study of the effects of weak magnetic field gradients on the spin relaxation of a dilute atomic gas. The theory is valid for low or moderate values of the field (the relevant correlation time of the gas is then the diffusion time across the container) as well as for high fields (the intercollision time then plays the most important role). Quantum effects due to particle indistinguishability are included. No consequences of the divergence of the atomic mean free path in a polarized gas at zero temperature are found, in contrast to the situation for viscosity and heat conductivity. On the other hand, substantial effects due to « identical spin rotation effects » are predicted.