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arXiv:cond-mat/9406101 · Physical Review Letters

Low-Temperature Spin Diffusion in a Spin-Polarized Fermi Gas

Denis I. Golosov, Andrei E. Ruckenstein

Published Feb 27, 1995• 19 citations
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Abstract

We present a finite temperature calculation of the transverse spin-diffusion coefficient ${D}_{\ensuremath{\perp}}$ in a dilute degenerate Fermi gas, in the presence of a small external magnetic field $H$. While the longitudinal diffusion coefficient displays the conventional Fermi-liquid dependence, ${D}_{\ensuremath{\parallel}}\ensuremath{\propto}{T}^{\ensuremath{-}2}$, the behavior of ${D}_{\ensuremath{\perp}}$ shows three separate regimes: (a) ${D}_{\ensuremath{\perp}}\ensuremath{\sim}{H}^{\ensuremath{-}2}$ for $T\ensuremath{\ll}H$, (b) ${D}_{\ensuremath{\perp}}\ensuremath{\sim}{T}^{\ensuremath{-}2}$, $\frac{{D}_{\ensuremath{\perp}}}{{D}_{\ensuremath{\parallel}}}\ensuremath{\ne}1$ for $T\ensuremath{\gg}H$ and large spin-rotation parameter $\ensuremath{\xi}\ensuremath{\gg}1$, and (c) ${D}_{\ensuremath{\perp}}={D}_{\ensuremath{\parallel}}\ensuremath{\propto}{T}^{\ensuremath{-}2}$ for $T\ensuremath{\gg}H$ and $\ensuremath{\xi}\ensuremath{\ll}1$. Our results are qualitatively consistent with the experimental data in weakly spin-polarized $^{3}\mathrm{He}$ and $^{3}\mathrm{He}$- $^{4}\mathrm{He}$ mixtures.

DOI
10.1103/physrevlett.74.1613

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We present a finite temperature calculation of the transverse spin-diffusion coefficient D\ensuremath⊥{D}_{\ensuremath{\perp}}D\ensuremath⊥​ in a dilute degenerate Fermi gas, in the presence of a small external magnetic field HHH. While the longitudinal diffusion coefficient displays the conventional Fermi-liquid dependence, D\ensuremath∥\ensuremath∝T\ensuremath−2{D}_{\ensuremath{\parallel}}\ensuremath{\propto}{T}^{\ensuremath{-}2}D\ensuremath∥​\ensuremath∝T\ensuremath−2, the behavior of D\ensuremath⊥{D}_{\ensuremath{\perp}}D\ensuremath⊥​ shows three separate regimes: (a) D\ensuremath⊥\ensuremath∼H\ensuremath−2{D}_{\ensuremath{\perp}}\ensuremath{\sim}{H}^{\ensuremath{-}2}D\ensuremath⊥​\ensuremath∼H\ensuremath−2 for T\ensuremath≪HT\ensuremath{\ll}HT\ensuremath≪H, (b) D\ensuremath⊥\ensuremath∼T\ensuremath−2{D}_{\ensuremath{\perp}}\ensuremath{\sim}{T}^{\ensuremath{-}2}D\ensuremath⊥​\ensuremath∼T\ensuremath−2, D\ensuremath⊥D\ensuremath∥\ensuremath≠1\frac{{D}_{\ensuremath{\perp}}}{{D}_{\ensuremath{\parallel}}}\ensuremath{\ne}1D\ensuremath∥​D\ensuremath⊥​​\ensuremath=1 for T\ensuremath≫HT\ensuremath{\gg}HT\ensuremath≫H and large spin-rotation parameter \ensuremathξ\ensuremath≫1\ensuremath{\xi}\ensuremath{\gg}1\ensuremathξ\ensuremath≫1, and (c) D\ensuremath⊥=D\ensuremath∥\ensuremath∝T\ensuremath−2{D}_{\ensuremath{\perp}}={D}_{\ensuremath{\parallel}}\ensuremath{\propto}{T}^{\ensuremath{-}2}D\ensuremath⊥​=D\ensuremath∥​\ensuremath∝T\ensuremath−2 for T\ensuremath≫HT\ensuremath{\gg}HT\ensuremath≫H and \ensuremathξ\ensuremath≪1\ensuremath{\xi}\ensuremath{\ll}1\ensuremathξ\ensuremath≪1. Our results are qualitatively consistent with the experimental data in weakly spin-polarized 3He^{3}\mathrm{He}3He and 3He^{3}\mathrm{He}3He- 4He^{4}\mathrm{He}4He mixtures.
We compute spin diffusion in a dilute Fermi gas at arbitrary temperature, polarization, and strong interaction in the normal phase using kinetic theory. While the longitudinal spin diffusivity ${D}_{\ensuremath{\parallel}}$ depends weakly on polarization and diverges for small temperatures, the transverse spin diffusivity ${D}_{\ensuremath{\perp}}$ has a strong polarization dependence and approaches a finite value for $T\ensuremath{\rightarrow}0$ in the Fermi liquid phase. For a 3D unitary Fermi gas at infinite scattering length, the diffusivities reach a minimum near the quantum limit of diffusion $\ensuremath{\hbar}/m$ in the quantum degenerate regime and are strongly suppressed by medium scattering, and we discuss the importance of the spin-rotation effect. In two dimensions, ${D}_{\ensuremath{\perp}}$ attains a minimum at strong coupling $\ensuremath{-}1\ensuremath{\lesssim}\mathrm{ln}({k}_{F}{a}_{2D})\ensuremath{\lesssim}1$ and reaches ${D}_{\ensuremath{\perp}}\ensuremath{\sim}0.2...\phantom{\rule{0.16em}{0ex}}0.3\phantom{\rule{0.16em}{0ex}}\ensuremath{\hbar}/m$ at large polarization. These values are consistent with recent measurements of two-dimensional ultracold atomic gases in the strong coupling regime.
We report measurements of the transverse-spin-diffusion coefficient ${\mathit{D}}_{\mathrm{\ensuremath{\perp}}}$ and the spin-rotation parameter \ensuremath{\Omega}${\mathrm{\ensuremath{\tau}}}_{\mathrm{\ensuremath{\perp}}}$ for two very dilute $^{3}\mathrm{\ensuremath{-}}^{4}$He mixtures (x3{\mathit{x}}_{3}x3​=1.82\ifmmode\times\else\texttimes\fi{}${10}^{\mathrm{\ensuremath{-}}3}$ and 6.26\ifmmode\times\else\texttimes\fi{}${10}^{\mathrm{\ensuremath{-}}4}$) spin polarized by an 8-T magnetic field. Brute-force spin polarization up to 40% was achieved at the lowest temperature, 6 mK. We find that \ensuremath{\Omega}${\mathrm{\ensuremath{\tau}}}_{\mathrm{\ensuremath{\perp}}}$ increases monotonically as the temperature is reduced through the Fermi temperature TF{\mathit{T}}_{\mathit{F}}TF​, in disagreement with the only previous experiment but in good agreement with recent theory. Unlike the earlier experiment, which measured spin echoes, the present experiments employed a spin-wave technique that avoids nonlinear excitation of the spin field. We compare our results with the recent calculations of Jeon and Mullin for spin transport in dilute gases with arbitrary polarization and degeneracy. The best fit to the data is obtained by scaling the quasiparticle interaction V(q) proposed by Ebner by a modest factor, 1.07. The corresponding s-wave scattering length is a=-1.21 \AA{}. Good agreement is found for \ensuremath{\Omega}${\mathrm{\ensuremath{\tau}}}_{\mathrm{\ensuremath{\perp}}}$(T) at both concentrations and all temperatures, and for ${\mathit{D}}_{\mathrm{\ensuremath{\perp}}}$/\ensuremath{\Omega}${\mathrm{\ensuremath{\tau}}}_{\mathrm{\ensuremath{\perp}}}$(T) apart from the lower concentration at T20 mK. The discrepancy in ${\mathit{D}}_{\mathrm{\ensuremath{\perp}}}$/\ensuremath{\Omega}${\mathrm{\ensuremath{\tau}}}_{\mathrm{\ensuremath{\perp}}}$ at the lowest temperatures and x3{\mathit{x}}_{3}x3​ could be explained by an unanticipated polarization dependence or by modification of the spin-wave boundary condition by processes occurring at the interface between the mixture and the silica cavity wall.
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Linear equations for the transverse spin dynamics in a weakly polarized degenerate Fermi liquid are derived from the Landau-Silin phenomenological kinetic equation with a general two-particle collision integral. Unlike a previous treatment where the Fermi velocity and density of states were taken to be constant independent of polarization we make no such assumption. The equations found describe the spin dynamics in a paramagnetic Fermi liquid with finite polarization as well in an itinerant ferromagnet. The results are confirmed by field theoretical calculations based on the integral equation for the vertex function. The transverse spin wave frequency in a polarized paramagnetic Fermi liquid is found to be proportional to k2{k}^{2}k2 with a complex diffusion coefficient such that the damping has a finite value proportional to the quasiparticles scattering rate at T=0T=0T=0. This behavior of a polarized Fermi liquid contrasts with the behavior of a Heisenberg ferromagnet in the hydrodynamic regime where the transverse spin-wave attenuation appears in terms proportional to k4{k}^{4}k4. The reactive part of the diffusion coefficient in a paramagnetic state at T=0T=0T=0 proves to be inversely proportional to the magnetization whereas in a ferromagnetic it is directly proportional to the magnetization. The dissipative part of the diffusion coefficient at T=0T=0T=0 in the paramagnetic state is polarization independent, whereas in the ferromagnetic state it is proportional to the square of the magnetization. Moreover, the spin wave spectrum in a ferromagnetic Fermi liquid proves to be unstable demonstrating the difficulty of applying a Fermi liquid description to itinerant ferromagnetism.
We have studied NMR spin echoes in 3He^{3}\mathrm{He}3He liquid in a magnetic field B0{\mathit{B}}_{0}B0​=8 T for temperatures T\ensuremath{\ge}4.5 mK. The data are analyzed in terms of the Leggett-Rice effect to obtain the transverse spin-diffusion coefficient ${\mathit{D}}_{\mathrm{\ensuremath{\perp}}}$(T). For T20 mK we find that ${\mathit{D}}_{\mathrm{\ensuremath{\perp}}}$ is less than measured in earlier experiments at lower B0{\mathit{B}}_{0}B0​. This phenomenon has been predicted for degenerate Fermi systems, due to the phase space created for quasiparticle scattering by spin polarization. The effect we have measured is more pronounced than suggested by scaling a dilute-gas theory result by a Fermi-liquid factor.
We carried out experiments on a spin polarized 3He- 4He mixture with 3He concentration x 3 = 6.26 × 10−4, and on pure 3He liquid. Spin polarization affects the transport properties of these Fermi systems. The effect on momentum transport was studied by using a vibrating-wire viscometer to measure viscosity of the 3He-4He mixture over the temperature range 6.09 mK–100 mK in 7.96 T and 1.00 T magnetic fields. A large viscosity increase was observed upon application of the 7.96 T magnetic field for temperature T < TF(TF = 19.5 mK is the Fermi temperature). The observed viscosity is in very good agreement with theoretical calculations for a dilute Fermi gas by Jeon and Mullin [1988, 1989] and Mullin and Jeon [1992]. The polarization effect on spin transport was investigated by measuring the transverse diffusion coefficient D ⊥ in pure 3He liquid at saturated vapor pressure and at 15.85 bar over the temperature range 4.5 mK–159 mK in a 7.96 T magnetic field. We used a pulsed NMR spin echo technique in a field gradient of 16.0 G/cm to do the measurements and fits to the Leggett equations [1970] to obtain D⊥. For T < 20 mK, we found D⊥ is less than measured in earlier experiments at lower magnetic fields. D⊥ does not increase with decreasing temperature as 1/T2, but appears to approach a constant as T → 0 while it is expected that the longitudinal spin diffusion coefficient D∥ ∝ 1/ T2. This is called spin diffusion anisotropy and it was observed for the first time in our 3He liquid experiments. The anisotropy temperature we determined for 3He liquid was Ta = 16.4 ± 2.2 mK at saturated vapor pressure and in a 7.96 T magnetic field. The transverse spin diffusion in 3 He results agree qualitatively with theories proposed by Meyerovich and Musaeflan [1992, 1994]. They also agree qualitatively with theories proposed by Golosov and Ruckenstein [1995, 1998] by extrapolation of the dilute theory to a strongly interacting system.