Single-shot acquisition of the cross-correlation between two counterpropagating short pulses is demonstrated over 150 ps using sum-frequency generation in an SBN61 crystal with random ferroelectric domains, revealing the jitter between two laser systems.
We report what we call co- and counter propagating slow-light systems based on the high nonlinearity in Si lattice-shifted
photonic crystal waveguides (LSPCWs). The intense slow-light pulse, as a control pulse, efficiently generates
two-photon absorption and carrier plasma effects, which tunes the dispersion characteristics of the LSPCWs and
spectrum of copropagating or counter-propagating slow-light pulse, as a signal pulse. Using the control pulse, we
succeeded in experimentally demonstrating adiabatic wavelength conversion and its enhancement, delay tuning of up to
10 ps with a response time <10 ps, and temporal pulse compression of factor 9.9 in the signal pulse. Furthermore, we
discussed theoretically the collision and reflection of the signal pulse counterpropagating against the control pulse
through the photonic-bandgap shift, resulting in a large Doppler shift. Considering the detail of these phenomena, we
clarified the relation and difference between the adiabatic wavelength conversion, cross-phase modulation, and Doppler
shift, which have been unclear so far.
Single-shot photoelectron spectroscopy of nonresonant two-color two-photon ionization of He has been carried out using an intense free-electron laser (FEL) at 59.7 nm and a femtosecond UV laser at 268 nm. By shot-by-shot analysis of photoelectron spectra, the cross section for nonresonant two-color ionization of He is determined to be ${\ensuremath{\sigma}}^{(2)}=4.1(6)\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}52}$ cm4 s. The cross-correlation trace derived from the nonresonant signals shows that the temporal resolution of the system is 0.36(3) ps, which is mainly governed by the timing jitter between the FEL and UV laser pulses.