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Journal of Modern Optics

Stimulated emission via quantum interference: Scattering of one-photon packets on an atom in a ground state

G. Drobný, Martti Havukainen, V. Bu[zcirc]ek

Published Apr 1, 2000• 15 citations
Publisher

Abstract

Usually it is assumed that the stimulated emission appears as a consequence of the Bose—Einstein statistics of photons and that to observe this effect at least two excitations have to be initially present in the atom—field system. That is, both the atom and the electromagnetic field have to be excited. In this paper we show that stimulated emission can appear exclusively as a consequence of quantum interference in a system with just a single excitation. Specifically, we consider a single two-level atom which is initially in its lower energy state and it interacts with a single-photon multi-mode wave packet. We show that for a proper choice of the photon-wave packet the atom can exhibit stimulated emission.

DOI
10.1080/09500340008235095

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Usually it is assumed that the stimulated emission appears as a consequence of the Bose—Einstein statistics of photons and that to observe this effect at least two excitations have to be initially present in the atom—field system. That is, both the atom and the electromagnetic field have to be excited. In this paper we show that stimulated emission can appear exclusively as a consequence of quantum interference in a system with just a single excitation. Specifically, we consider a single two-level atom which is initially in its lower energy state and it interacts with a single-photon multi-mode wave packet. We show that for a proper choice of the photon-wave packet the atom can exhibit stimulated emission.
Stimulated emission can be defined as the process when an incoming photon stimulates an additional quantum of energy from an atom into the same electromagnetic mode as the impinging photon. Hence, the two outgoing photons are identical. In a waveguide or free space, this intuition is typically found through Fermi's Golden rule, however, this does not properly account for the wave-like nature of the photons. Here, I present an exact solution to stimulated emission from a quantum two-level atom that properly accounts for the incoming and outgoing electromagnetic modes. This result is valid over a huge range of incident photon numbers. For a single incident photon, it shows how the photon must properly mode match the two-level system to cause stimulated emission. For a Fock state drive with large photon number, the exact solution shows how a two-level system Rabi oscillates with the traveling Fock mode as it passes by. I additionally use the same formalism to show that stimulated emission by a coherent pulse cannot be understood as an additional photon being emitted into the incident coherent state because the two-level system's state factorizes with the electromagnetic field's coherent state. Recent advances in superconducting circuits make them an ideal platform to test these predictions.
The interaction of a single-photon wave packet with an initially excited two-level atom in free space is studied in semiclassical and quantum approaches. It is shown that the final state of the field does not contain doubly occupied modes. The process of the atom's transition to the ground state may be accelerated, decelerated, or even reversed by the incoming photon, depending on parameters. The spectrum of emitted radiation is close to the sum of the spectrum of the incoming single-photon wave packet and the natural line shape, with small and complicated deviations.
We theoretically investigate signatures of stimulated emission at the single-photon level for a two-level atom interacting with a one-dimensional light field. We consider the transient regime where the atom is initially excited, and the steady-state regime where the atom is continuously driven with an external pump. The influence of pure dephasing is studied, clearly showing that these effects can be evidenced with state-of-the-art solid-state devices. We finally propose a scheme to demonstrate the stimulation of one optical transition by monitoring another one, in three-level one-dimensional atoms.
In this contribution we investigate quantum electrodynamical many-mode aspects by exploring the simplest possible situation in this context, namely the interaction of a single atom, modeled by a simple two-level system, with many-mode one-photon quantum states of the electromagnetic field. In particular, we concentrate on the question how the engineering of electromagnetic field modes influences the atom-field interaction. An interesting problem in this context is the engineering of ideal one-photon multi-mode quantum states which may excite a single atom perfectly [M. Stobińska, G. Alber, and G. Leuchs, EPL {\bf 86}, 14007 (2009)]. For purposes of quantum information processing such one-photon multi-mode states are particularly well suited for transmitting quantum information and for storing it in a material memory again.
We investigate (non-relativistic) atomic systems interacting with quantum electromagnetic field (QEF). The resulting model describes spontaneous emission of light from a two-level atom surrounded by various initial states of the QEF. We assume that the quantum field interacts with the atom via the standard, minimal-coupling Hamiltonian, with the A2 term neglected. We also assume that there will appear at most single excitations (photons). By conducting the analysis on a general level we allow for an arbitrary initial state of the QEF (which can be for instance: the vacuum, the ground state in a cavity, or the squeezed state). We derive a Volterra-type equation which governs the time evolution of the amplitude of the excited state. The two-point function of the initial state of the QEF, integrated with a combination of atomic wavefunctions, forms the kernel of this equation.