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arXiv:1108.0563 · Physical Review A

Interaction of a single-photon wave packet with an excited atom

P. V. Elyutin

Published Mar 16, 2012• 8 citations
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Abstract

The interaction of a single-photon wave packet with an initially excited two-level atom in free space is studied in semiclassical and quantum approaches. It is shown that the final state of the field does not contain doubly occupied modes. The process of the atom's transition to the ground state may be accelerated, decelerated, or even reversed by the incoming photon, depending on parameters. The spectrum of emitted radiation is close to the sum of the spectrum of the incoming single-photon wave packet and the natural line shape, with small and complicated deviations.

DOI
10.1103/physreva.85.033816

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The interaction of a single-photon wave packet with an initially excited two-level atom in free space is studied in semiclassical and quantum approaches. It is shown that the final state of the field does not contain doubly occupied modes. The process of the atom's transition to the ground state may be accelerated, decelerated, or even reversed by the incoming photon, depending on parameters. The spectrum of emitted radiation is close to the sum of the spectrum of the incoming single-photon wave packet and the natural line shape, with small and complicated deviations.
Rapid advances in quantum technology have made possible the control of quantum states of elementary material quantum systems, such as atoms or molecules, and of the electromagnetic radiation field resulting from spontaneous photon emission of their unstable excited states to such a level of precision that subtle quantum electrodynamical phenomena have become observable experimentally. Recent developments in the area of quantum information processing demonstrate that characteristic quantum electrodynamical effects can even be exploited for practical purposes provided the relevant electromagnetic field modes are controlled by appropriate cavities. A central problem in this context is the realization of an ideal transfer of quantum information between a state of a material quantum system and a quantum state of the electromagnetic radiation field which contains a small number or even a single photon only. Despite much recent work in cavity quantum electrodynamics, which has explored this problem successfully in cases in which the number of accessible electromagnetic field modes is strongly restricted by a cavity, currently still much less is known about ideal quantum state transfer between matter and few-photon quantum states of the electromagnetic field in the extreme opposite case of free space. In this contribution we review recent work which explores characteristic quantum electrodynamical phenomena governing the interaction of a material quantum system with the electromagnetic field in extreme many-mode cases which are close to cavity-free situations. For this purpose the simplest possible quantum electrodynamical situation, namely the interaction of a single material two-level system with the wave packet of a single optical photon, is investigated in free space and in situations in which a large cavity modifies the mode structure of the electromagnetic field modes. It is demonstrated that perfect excitation of an atom by a properly shaped single-photon wave packet is possible even in free space. In particular, it is demonstrated that perfect excitation of an atom can be achieved by a single optical photon which is prepared initially in an appropriate superposition of plane-wave modes, provided this photon is focused subsequently onto the absorbing atom by a parabolic cavity.
Usually it is assumed that the stimulated emission appears as a consequence of the Bose—Einstein statistics of photons and that to observe this effect at least two excitations have to be initially present in the atom—field system. That is, both the atom and the electromagnetic field have to be excited. In this paper we show that stimulated emission can appear exclusively as a consequence of quantum interference in a system with just a single excitation. Specifically, we consider a single two-level atom which is initially in its lower energy state and it interacts with a single-photon multi-mode wave packet. We show that for a proper choice of the photon-wave packet the atom can exhibit stimulated emission.
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State mapping between atoms and photons, and photon-photon interactions play an important role in scalable quantum information processing. We consider the interaction of a two-level atom with a quantized propagating pulse in free space and study the probability Pe(t){P}_{e}(t)Pe​(t) of finding the atom in the excited state at any time ttt. This probability is expected to depend on (i) the quantum state of the pulse field and (ii) the overlap between the pulse and the dipole pattern of the atomic spontaneous emission. We show that the second effect is captured by a single parameter $\ensuremath{\Lambda}\ensuremath{\in}[0,8\ensuremath{\pi}/3]$, obtained by weighting the dipole pattern with the numerical aperture. Then, Pe(t){P}_{e}(t)Pe​(t) can be obtained by solving time-dependent Heisenberg-Langevin equations. We provide detailed solutions for both single-photon Fock state and coherent states and for various temporal shapes of the pulses.
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