Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:1010.4661 · Physical Review A

Efficient excitation of a two-level atom by a single photon in a propagating mode

Yimin Wang, Jiří Minář, Lana Sheridan, Valerio Scarani

Published Jun 28, 2011• 122 citations
arXivHTMLPDF

Abstract

State mapping between atoms and photons, and photon-photon interactions play an important role in scalable quantum information processing. We consider the interaction of a two-level atom with a quantized propagating pulse in free space and study the probability ${P}_{e}(t)$ of finding the atom in the excited state at any time $t$. This probability is expected to depend on (i) the quantum state of the pulse field and (ii) the overlap between the pulse and the dipole pattern of the atomic spontaneous emission. We show that the second effect is captured by a single parameter $\ensuremath{\Lambda}\ensuremath{\in}[0,8\ensuremath{\pi}/3]$, obtained by weighting the dipole pattern with the numerical aperture. Then, ${P}_{e}(t)$ can be obtained by solving time-dependent Heisenberg-Langevin equations. We provide detailed solutions for both single-photon Fock state and coherent states and for various temporal shapes of the pulses.

DOI
10.1103/physreva.83.063842

Related papers

Excitation of two atoms by a propagating single photon pulse

Navneeth Ramakrishnan, Yimin Wang, Valerio Scarani

We describe the interaction of two two-level atoms in free space with propagating modes of the quantized electromagnetic field, using the time-dependent Heisenberg-Langevin method. For single- photon pulses, we consider the effect of the pulse's spatial and temporal profiles on the atomic excitation. In particular, we find the ideal shape for a pulse to put exactly one excitation in any desired state of the bi-atomic system. Furthermore, we analyze the differences in the atomic dynamics between the cases of Fock state pulses and coherent state pulses.

arXiv:1411.3445•Nov 13, 2014•0 citations

QUANTUM INFORMATION EXCHANGE BETWEEN PHOTONS AND ATOMS

Wang Yi-min

Quantum information processing tasks have been implemented in various physical platforms. In this thesis, we consider two specific implementations: Part I presents a detailed study of the interaction of a single atom with a light pulse. Part II examines the case of a quantum controlled-phase gate in circuit quantum electrodynamics in the ultrastrong coupling regime. They are both actively pursued by many research groups. In Part I, we first present the framework for a single two-level atom interacting with the quantized electromagnetic field. The effect of temporal and spectral properties of the pulses on atomic excitation is studied for both Fock state and coherent state pulse. The detailed analysis of atomic excited state population is provided for single photon pulse with various temporal shapes. The work is then extended to a more general case with two spatial-modes and multi-photon pulses. The difference between Fock state and coherent state pulse on atomic excitation is further investigated. We find that at few photon levels, the maximum atomic excitation probability is a monotonic function of photon number for the coherent state pulse, but not for the Fock state pulse. Furthermore, we show that the atomic dynamics can be controlled by the initial relative phase between the two counter-propagating coherent state pulses incident on the atom, which is not the case with two Fock state pulses. The theoretical prediction is then compared with an experiment, where a single trapped 87Rb atom interacts with coherent state pulses engineered in temporal shape of rising exponential and rectangular form. Next, we propose a quantum memory setup based on a single two-level atom in a half cavity with a moving mirror. The efficiency of the quantum storage process is studied analytically and

•Jan 1, 2013•0 citations

State-dependent atomic excitation by multiphoton pulses propagating along two spatial modes

Yimin Wang, Jiří Minář, Valerio Scarani

We investigate the dynamics of a single two-level atom, which interacts with pulses propagating in two spatial modes (right and left) and frequency continuum. Using Heisenberg equations of motion, we present the explicit analytical derivations and general formalisms for atomic excitation with two-spatial-mode multiphoton pulses in both the Fock and coherent states. Based on those formalisms, we show that perfect atomic excitation by a single-photon Fock state pulse can only be realized when it is rising exponentially shaped in the even mode, a balanced superposition of the two spatial modes. A single photon from a single spatial mode can only give half of the maximal atomic excitation probability. We also show that the maximum atomic excitation probability with multiphoton pulses in the even mode is a monotonic function of the average photon number for the coherent state, but not for the Fock states. Furthermore, we demonstrate that the atomic dynamics can be controlled by the initial relative phase between the two counterpropagating coherent state pulses incident on the atom, which is not the case with the two Fock state pulses.

arXiv:1204.5265•Physical Review A•Aug 7, 2012•11 citations

Two-level-atom excitation probability for single- and N -photon wave packets

Hemlin Swaran Rag, Julio R. Gea-Banacloche

We study how the transient excitation probability of a two-level atom by a quantized field depends on the temporal profile of the incident pulse, in the presence of external losses, for both coherent and Fock states, and in two complementary limits: when the pulse contains only one photon (on average), and when the number of photons $N$ is large. For the latter case we derive analytical expressions for the scaling of the excitation probability with $N$ that can be easily evaluated for any pulse shape.

arXiv:1707.02351•Physical Review A•Sep 11, 2017•15 citations

Arbitrary control of the temporal waveform of photons during spontaneous emission

Carl Thomas, Rebecca Munk, Boris Blinov

Control of the temporal waveform of photons produced during spontaneous emission from single quantum emitters provides a crucial tool in the establishment of hybrid quantum systems, optimization of quantum state transfer protocols and mitigation of effects due interferometric instability for network architectures based on flying qubits. We describe a method to generate photons of any temporal waveform from emitters of any excited state lifetime, limited only by the timing resolution of control hardware. We show how the temporal waveform of photons can be controlled by deterministically varying the population of an excited state which undergoes spontaneous emission. Our broadly applicable approach has only two requirements for a candidate quantum emitter: modulation of the (1) amplitude and (2) relative phase of a field coupling a ground state to the excited manifold. We detail how to identify optimal excitation pulses by employing variational algorithms to feed back on atomic populations. Additionally, we develop Quantum Monte Carlo based tools to determine photon-number statistics and establish techniques to identify optimal excitation strengths and post-selection thresholds for photon generation protocols. We situate our work in the context of other prior research on bespoke single photon sources and networking including post-emission pulse shaping, temporal gating and cavity-based methods. In comparison, our free-space process has greater flexibility in producing any waveform, requires less infrastructure, and can be readily applied across a wide range of quantum emitters. We discuss the applications and limits of this technique, including how increasing photon emission probabilities affects achievable temporal-mode overlap fidelities between emitted and target photon waveforms.

physics.atom-phCross-listedarXiv:2511.23462•Physical Review A•Dec 1, 2025•0 citations

Cavity-assisted spontaneous emission as a single-photon source: Pulse shape and efficiency of one-photon Fock-state preparation

M. Khanbekyan, D.‐G. Welsch, C. Di Fidio +1 more

Within the framework of exact quantum electrodynamics in dispersing and absorbing media, we have studied the quantum state of the radiation emitted from an initially in the upper state, prepared two-level atom in a high-$\mathit{Q}$ cavity, including the regime where the emitted photon belongs to a wave packet that simultaneously covers the areas inside and outside the cavity. For both continuing atom-field interaction and short-term atom-field interaction, we have determined the spatiotemporal shape of the excited outgoing wave packet and calculated the efficiency of the wave packet to carry a one-photon Fock state. Furthermore, we have made contact with quantum noise theories where the intracavity field and the field outside the cavity are regarded as approximately representing independent degrees of freedom such that two separate Hilbert spaces can be introduced.

arXiv:0709.2998•Physical Review A•Jul 15, 2008•16 citations
State mapping between atoms and photons, and photon-photon interactions play an important role in scalable quantum information processing. We consider the interaction of a two-level atom with a quantized propagating pulse in free space and study the probability Pe(t){P}_{e}(t)Pe​(t) of finding the atom in the excited state at any time ttt. This probability is expected to depend on (i) the quantum state of the pulse field and (ii) the overlap between the pulse and the dipole pattern of the atomic spontaneous emission. We show that the second effect is captured by a single parameter \ensuremathΛ\ensuremath∈[0,8\ensuremathπ/3]\ensuremath{\Lambda}\ensuremath{\in}[0,8\ensuremath{\pi}/3]\ensuremathΛ\ensuremath∈[0,8\ensuremathπ/3], obtained by weighting the dipole pattern with the numerical aperture. Then, Pe(t){P}_{e}(t)Pe​(t) can be obtained by solving time-dependent Heisenberg-Langevin equations. We provide detailed solutions for both single-photon Fock state and coherent states and for various temporal shapes of the pulses.
We describe the interaction of two two-level atoms in free space with propagating modes of the quantized electromagnetic field, using the time-dependent Heisenberg-Langevin method. For single- photon pulses, we consider the effect of the pulse's spatial and temporal profiles on the atomic excitation. In particular, we find the ideal shape for a pulse to put exactly one excitation in any desired state of the bi-atomic system. Furthermore, we analyze the differences in the atomic dynamics between the cases of Fock state pulses and coherent state pulses.
Quantum information processing tasks have been implemented in various physical platforms. In this thesis, we consider two specific implementations: Part I presents a detailed study of the interaction of a single atom with a light pulse. Part II examines the case of a quantum controlled-phase gate in circuit quantum electrodynamics in the ultrastrong coupling regime. They are both actively pursued by many research groups. In Part I, we first present the framework for a single two-level atom interacting with the quantized electromagnetic field. The effect of temporal and spectral properties of the pulses on atomic excitation is studied for both Fock state and coherent state pulse. The detailed analysis of atomic excited state population is provided for single photon pulse with various temporal shapes. The work is then extended to a more general case with two spatial-modes and multi-photon pulses. The difference between Fock state and coherent state pulse on atomic excitation is further investigated. We find that at few photon levels, the maximum atomic excitation probability is a monotonic function of photon number for the coherent state pulse, but not for the Fock state pulse. Furthermore, we show that the atomic dynamics can be controlled by the initial relative phase between the two counter-propagating coherent state pulses incident on the atom, which is not the case with two Fock state pulses. The theoretical prediction is then compared with an experiment, where a single trapped 87Rb atom interacts with coherent state pulses engineered in temporal shape of rising exponential and rectangular form. Next, we propose a quantum memory setup based on a single two-level atom in a half cavity with a moving mirror. The efficiency of the quantum storage process is studied analytically and
We investigate the dynamics of a single two-level atom, which interacts with pulses propagating in two spatial modes (right and left) and frequency continuum. Using Heisenberg equations of motion, we present the explicit analytical derivations and general formalisms for atomic excitation with two-spatial-mode multiphoton pulses in both the Fock and coherent states. Based on those formalisms, we show that perfect atomic excitation by a single-photon Fock state pulse can only be realized when it is rising exponentially shaped in the even mode, a balanced superposition of the two spatial modes. A single photon from a single spatial mode can only give half of the maximal atomic excitation probability. We also show that the maximum atomic excitation probability with multiphoton pulses in the even mode is a monotonic function of the average photon number for the coherent state, but not for the Fock states. Furthermore, we demonstrate that the atomic dynamics can be controlled by the initial relative phase between the two counterpropagating coherent state pulses incident on the atom, which is not the case with the two Fock state pulses.
We study how the transient excitation probability of a two-level atom by a quantized field depends on the temporal profile of the incident pulse, in the presence of external losses, for both coherent and Fock states, and in two complementary limits: when the pulse contains only one photon (on average), and when the number of photons NNN is large. For the latter case we derive analytical expressions for the scaling of the excitation probability with NNN that can be easily evaluated for any pulse shape.
Control of the temporal waveform of photons produced during spontaneous emission from single quantum emitters provides a crucial tool in the establishment of hybrid quantum systems, optimization of quantum state transfer protocols and mitigation of effects due interferometric instability for network architectures based on flying qubits. We describe a method to generate photons of any temporal waveform from emitters of any excited state lifetime, limited only by the timing resolution of control hardware. We show how the temporal waveform of photons can be controlled by deterministically varying the population of an excited state which undergoes spontaneous emission. Our broadly applicable approach has only two requirements for a candidate quantum emitter: modulation of the (1) amplitude and (2) relative phase of a field coupling a ground state to the excited manifold. We detail how to identify optimal excitation pulses by employing variational algorithms to feed back on atomic populations. Additionally, we develop Quantum Monte Carlo based tools to determine photon-number statistics and establish techniques to identify optimal excitation strengths and post-selection thresholds for photon generation protocols. We situate our work in the context of other prior research on bespoke single photon sources and networking including post-emission pulse shaping, temporal gating and cavity-based methods. In comparison, our free-space process has greater flexibility in producing any waveform, requires less infrastructure, and can be readily applied across a wide range of quantum emitters. We discuss the applications and limits of this technique, including how increasing photon emission probabilities affects achievable temporal-mode overlap fidelities between emitted and target photon waveforms.
Within the framework of exact quantum electrodynamics in dispersing and absorbing media, we have studied the quantum state of the radiation emitted from an initially in the upper state, prepared two-level atom in a high-Q\mathit{Q}Q cavity, including the regime where the emitted photon belongs to a wave packet that simultaneously covers the areas inside and outside the cavity. For both continuing atom-field interaction and short-term atom-field interaction, we have determined the spatiotemporal shape of the excited outgoing wave packet and calculated the efficiency of the wave packet to carry a one-photon Fock state. Furthermore, we have made contact with quantum noise theories where the intracavity field and the field outside the cavity are regarded as approximately representing independent degrees of freedom such that two separate Hilbert spaces can be introduced.