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arXiv:0709.2998 · Physical Review A

Cavity-assisted spontaneous emission as a single-photon source: Pulse shape and efficiency of one-photon Fock-state preparation

M. Khanbekyan, D.‐G. Welsch, C. Di Fidio, W. Vogel

Published Jul 15, 2008• 16 citations
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Abstract

Within the framework of exact quantum electrodynamics in dispersing and absorbing media, we have studied the quantum state of the radiation emitted from an initially in the upper state, prepared two-level atom in a high-$\mathit{Q}$ cavity, including the regime where the emitted photon belongs to a wave packet that simultaneously covers the areas inside and outside the cavity. For both continuing atom-field interaction and short-term atom-field interaction, we have determined the spatiotemporal shape of the excited outgoing wave packet and calculated the efficiency of the wave packet to carry a one-photon Fock state. Furthermore, we have made contact with quantum noise theories where the intracavity field and the field outside the cavity are regarded as approximately representing independent degrees of freedom such that two separate Hilbert spaces can be introduced.

DOI
10.1103/physreva.78.013822

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Within the framework of exact quantum electrodynamics in dispersing and absorbing media, we have studied the quantum state of the radiation emitted from an initially in the upper state, prepared two-level atom in a high-Q\mathit{Q}Q cavity, including the regime where the emitted photon belongs to a wave packet that simultaneously covers the areas inside and outside the cavity. For both continuing atom-field interaction and short-term atom-field interaction, we have determined the spatiotemporal shape of the excited outgoing wave packet and calculated the efficiency of the wave packet to carry a one-photon Fock state. Furthermore, we have made contact with quantum noise theories where the intracavity field and the field outside the cavity are regarded as approximately representing independent degrees of freedom such that two separate Hilbert spaces can be introduced.
Within the framework of quantum electrodynamics in dispersing and absorbing media, we have studied the quantum state of the radiation emitted from an initially in the upper state prepared two-level atom in a high-Q cavity, including the regime where the emitted photon belongs to a wave packet that simultaneously covers areas inside and outside the cavity. Furthermore, we have compared the results with those of quantum noise theory where the intracavity field and the field outside the cavity are regarded as approximately representing independent degrees of freedom such that two separate Hilbert spaces can be introduced.
Within the framework of exact quantum electrodynamics in dispersing and absorbing media, we have studied the emission from an initially in the upper state prepared emitter in a high-quality cavity in the case when there are two cavity modes that resonantly interact with the emitter. In the case when one of the modes is in resonance with the emitter transition and the other mode is tuned to the frequency equal to the Rabi splitting of the first mode, the effect of Rabi resonance is observed. In particular, the second mode exhibits a substantial increase of the one-photon Fock state efficiency and enhancement of the emission spectrum in comparison to the exact resonant case.
Stimulated Raman interaction of a classically pumped single three-level ΛΛΛ-type atom in a resonator cavity featuring both radiative and unwanted losses is studied. It is shown that in the regime of stimulated adiabatic Raman passage the excited outgoing wave packet of the cavity-assisted electromagnetic field can be prepared in a one-photon Fock state with high efficiency. In this regime, the spatio-temporal shape of the wave packet does not depend on the interaction shape of the pump field, provided that the interaction of the atom with the pump is time-delayed with respect to the interaction of the atom with the cavity-assisted field. Therefore, the scheme can be used to generate a sequence of identical radiation pulses each of almost one-photon Fock state. It is further shown that the spatio-temporal shape of the outgoing wave packet can be manipulated by controlling the time of interaction between the atom and the cavity-assisted electromagnetic field.
Rapid advances in quantum technology have made possible the control of quantum states of elementary material quantum systems, such as atoms or molecules, and of the electromagnetic radiation field resulting from spontaneous photon emission of their unstable excited states to such a level of precision that subtle quantum electrodynamical phenomena have become observable experimentally. Recent developments in the area of quantum information processing demonstrate that characteristic quantum electrodynamical effects can even be exploited for practical purposes provided the relevant electromagnetic field modes are controlled by appropriate cavities. A central problem in this context is the realization of an ideal transfer of quantum information between a state of a material quantum system and a quantum state of the electromagnetic radiation field which contains a small number or even a single photon only. Despite much recent work in cavity quantum electrodynamics, which has explored this problem successfully in cases in which the number of accessible electromagnetic field modes is strongly restricted by a cavity, currently still much less is known about ideal quantum state transfer between matter and few-photon quantum states of the electromagnetic field in the extreme opposite case of free space. In this contribution we review recent work which explores characteristic quantum electrodynamical phenomena governing the interaction of a material quantum system with the electromagnetic field in extreme many-mode cases which are close to cavity-free situations. For this purpose the simplest possible quantum electrodynamical situation, namely the interaction of a single material two-level system with the wave packet of a single optical photon, is investigated in free space and in situations in which a large cavity modifies the mode structure of the electromagnetic field modes. It is demonstrated that perfect excitation of an atom by a properly shaped single-photon wave packet is possible even in free space. In particular, it is demonstrated that perfect excitation of an atom can be achieved by a single optical photon which is prepared initially in an appropriate superposition of plane-wave modes, provided this photon is focused subsequently onto the absorbing atom by a parabolic cavity.
The radiation emitted by a classically pumped three-level $\mathrm{\ensuremath{\Lambda}}$-type emitter in a resonator cavity featuring both radiative and unwanted losses is studied. In particular, the efficiency of one-photon Fock state excitation of the outgoing wave packet and the spatiotemporal shape of the wave packet are investigated. It is shown that, for a given shape of the emitter-cavity interaction, adjusting the shape of the pump pulse renders it possible to generate the emission of one-photon Fock state wave packets of desired shape with high efficiency.
Over the last decades, quantum optics has evolved from high-quality-factor cavities in the early experiments toward new cavity designs involving leaky modes. Despite very reliable models, in the concepts of cavity quantum electrodynamics, photon leakage is most of the time treated phenomenologically. Here, we take a different approach, and starting from first principles, we define an inside-outside representation which is derived from the original true-mode representation, in which one can determine the effective Hamiltonian and Poynting vector. Unlike the phenomenological model, they allow a full description of a leaking single photon produced in the cavity and propagating in free space. This is applied for a laser-driven atom-cavity system. In addition, we propose an atom-cavity nonresonant scheme for single-photon generation, and we rigorously analyze the outgoing single photon in time and frequency domains for different coupling regimes. Finally, we introduce a particular coupling regime ensuring adiabatic elimination for which the pulse shape of the outgoing single photon is tailored using a specifically designed driving field envelope.