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arXiv:1806.04862 · OSA Continuum

Exact calculation of stimulated emission driven by pulsed light

Kevin A. Fischer

Published Oct 12, 2018• 11 citations

Abstract

Stimulated emission can be defined as the process when an incoming photon stimulates an additional quantum of energy from an atom into the same electromagnetic mode as the impinging photon. Hence, the two outgoing photons are identical. In a waveguide or free space, this intuition is typically found through Fermi's Golden rule, however, this does not properly account for the wave-like nature of the photons. Here, I present an exact solution to stimulated emission from a quantum two-level atom that properly accounts for the incoming and outgoing electromagnetic modes. This result is valid over a huge range of incident photon numbers. For a single incident photon, it shows how the photon must properly mode match the two-level system to cause stimulated emission. For a Fock state drive with large photon number, the exact solution shows how a two-level system Rabi oscillates with the traveling Fock mode as it passes by. I additionally use the same formalism to show that stimulated emission by a coherent pulse cannot be understood as an additional photon being emitted into the incident coherent state because the two-level system's state factorizes with the electromagnetic field's coherent state. Recent advances in superconducting circuits make them an ideal platform to test these predictions.

DOI: 10.1364/osac.1.000772

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Stimulated emission can be defined as the process when an incoming photon stimulates an additional quantum of energy from an atom into the same electromagnetic mode as the impinging photon. Hence, the two outgoing photons are identical. In a waveguide or free space, this intuition is typically found through Fermi's Golden rule, however, this does not properly account for the wave-like nature of the photons. Here, I present an exact solution to stimulated emission from a quantum two-level atom that properly accounts for the incoming and outgoing electromagnetic modes. This result is valid over a huge range of incident photon numbers. For a single incident photon, it shows how the photon must properly mode match the two-level system to cause stimulated emission. For a Fock state drive with large photon number, the exact solution shows how a two-level system Rabi oscillates with the traveling Fock mode as it passes by. I additionally use the same formalism to show that stimulated emission by a coherent pulse cannot be understood as an additional photon being emitted into the incident coherent state because the two-level system's state factorizes with the electromagnetic field's coherent state. Recent advances in superconducting circuits make them an ideal platform to test these predictions.

Usually it is assumed that the stimulated emission appears as a consequence of the Bose—Einstein statistics of photons and that to observe this effect at least two excitations have to be initially present in the atom—field system. That is, both the atom and the electromagnetic field have to be excited. In this paper we show that stimulated emission can appear exclusively as a consequence of quantum interference in a system with just a single excitation. Specifically, we consider a single two-level atom which is initially in its lower energy state and it interacts with a single-photon multi-mode wave packet. We show that for a proper choice of the photon-wave packet the atom can exhibit stimulated emission.

Photon statistics are obtained from exact closed-form solutions for both spontaneous and stimulated coherent emissions by a large number of two-level atoms in a Dicke state. Depending on the initial excitation level of the atoms, three types of photon statistics are obtained for the emitted radiation field. Moments of the photon number of the emitted field are calculated in the case of initial atomic coherent states as well as Dicke states, and in the case of n-photon stimulating pulses as well as coherent stimulating pulses. In the particular case of an initial "superradiant" Dicke state stimulated by a coherent-radiation field, the emitted radiation pulse is also fully coherent. In other cases the photon distributions undergo large fluctuations.

Photon subtraction and addition are essential non-Gaussian processes in quantum optics, where conventional methods using linear optics and number-resolving detection often suffer from low success probability. Here, we introduce the concept of \textit{dynamic stimulated emission}, whereby a quantum emitter undergoes stimulated emission with a time-dependent coupling. Despite interacting with a multimode photon field, we show that, for both two- and three-level emitters, their dynamics can mimic that of a single-mode Jaynes-Cummings model. This feature can be used to deterministically add or subtract a photon while maintaining a single propagating optical mode. We provide semi-analytic solutions to this problem for Fock states, enabling deterministic and unconditional photon addition and subtraction with fidelity

{\cal F}>0.996

. Our semi-analytic solutions are provided for both dynamically coupled two-level systems and for three-level systems whose dynamical coupling is controlled by a coherent laser drive. Moving beyond individual Fock states, we further showcase the ability to subtract and add single photons to photon-number superposition states. We show that Schr{ö}dinger cat states can be prepared from squeezed vacuum input via cascaded subtraction or cascaded addition. Finally, we show that our photon-addition process can be used to add a photon to any squeezed and displaced state with high success probability and fidelity

{\cal F}>0.99

, thereby potentially converting quantum emitters from single-photon sources to sources of single-photon-added Gaussian states without the need for inline squeezing. Our protocols provide a path towards integrating quantum emitters to construct efficient sources of single-mode non-Gaussian light beyond single photons.

We investigate the stimulated emission of superradiant atoms coupled to a waveguide induced by a coherent-state photon pulse. We provide an analytical result when a short

π

pulse is incident, which shows that the atoms emit photons coherently into the output pulse, which remains a coherent state in the short pulse limit. An incident pulse is amplified in phase-preserving manner, where noise is added almost entirely in the phase direction in phase space. This property improves the ratio of intensity signal to noise after the amplification for sufficiently short pulses. This is a unique feature different from general phase-preserving linear amplifiers, where the signal-to-noise ratio deteriorates in the amplification process. We also discuss the dependence of the photon-emission probability on pulse parameters, such as the pulse area and the duration.