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arXiv:2512.09711

Dynamic stimulated emission for deterministic addition and subtraction of propagating photons

Haoyuan Luo, Parth S. Shah, Frank Yang, Mohammad Mirhosseini, Sahand Mahmoodian

quant-phSubmitted Dec 10, 2025• Announced Dec 11, 2025• 0 citations• Revised Sep 13, 2026 (v2)
v1 · Dec 10, 2025v2 · Sep 13, 2026
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Abstract

Photon subtraction and addition are essential non-Gaussian processes in quantum optics, where conventional methods using linear optics and number-resolving detection often suffer from low success probability. Here, we introduce the concept of \textit{dynamic stimulated emission}, whereby a quantum emitter undergoes stimulated emission with a time-dependent coupling. Despite interacting with a multimode photon field, we show that, for both two- and three-level emitters, their dynamics can mimic that of a single-mode Jaynes-Cummings model. This feature can be used to deterministically add or subtract a photon while maintaining a single propagating optical mode. We provide semi-analytic solutions to this problem for Fock states, enabling deterministic and unconditional photon addition and subtraction with fidelity ${\cal F}>0.996$. Our semi-analytic solutions are provided for both dynamically coupled two-level systems and for three-level systems whose dynamical coupling is controlled by a coherent laser drive. Moving beyond individual Fock states, we further showcase the ability to subtract and add single photons to photon-number superposition states. We show that Schr{ö}dinger cat states can be prepared from squeezed vacuum input via cascaded subtraction or cascaded addition. Finally, we show that our photon-addition process can be used to add a photon to any squeezed and displaced state with high success probability and fidelity ${\cal F}>0.99$, thereby potentially converting quantum emitters from single-photon sources to sources of single-photon-added Gaussian states without the need for inline squeezing. Our protocols provide a path towards integrating quantum emitters to construct efficient sources of single-mode non-Gaussian light beyond single photons.

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Photon subtraction and addition are essential non-Gaussian processes in quantum optics, where conventional methods using linear optics and number-resolving detection often suffer from low success probability. Here, we introduce the concept of \textit{dynamic stimulated emission}, whereby a quantum emitter undergoes stimulated emission with a time-dependent coupling. Despite interacting with a multimode photon field, we show that, for both two- and three-level emitters, their dynamics can mimic that of a single-mode Jaynes-Cummings model. This feature can be used to deterministically add or subtract a photon while maintaining a single propagating optical mode. We provide semi-analytic solutions to this problem for Fock states, enabling deterministic and unconditional photon addition and subtraction with fidelity F>0.996{\cal F}>0.996F>0.996. Our semi-analytic solutions are provided for both dynamically coupled two-level systems and for three-level systems whose dynamical coupling is controlled by a coherent laser drive. Moving beyond individual Fock states, we further showcase the ability to subtract and add single photons to photon-number superposition states. We show that Schr{ö}dinger cat states can be prepared from squeezed vacuum input via cascaded subtraction or cascaded addition. Finally, we show that our photon-addition process can be used to add a photon to any squeezed and displaced state with high success probability and fidelity F>0.99{\cal F}>0.99F>0.99, thereby potentially converting quantum emitters from single-photon sources to sources of single-photon-added Gaussian states without the need for inline squeezing. Our protocols provide a path towards integrating quantum emitters to construct efficient sources of single-mode non-Gaussian light beyond single photons.
Abstract We explore a recently demonstrated deterministic photon subtraction scheme, based on single-photon Raman interaction with a Λ-type three-level atom, as a tool for manipulating quantum state of few-photon light pulses. We establish a comprehensive theoretical framework using input–output formalism and quantum regression theorem, enabling calculation of the first order autocorrelation matrices of the output light and identification of the temporal modes present in the generated light via their eigendecomposition. By modeling the entire system as a quantum network consisting multiple virtual cavities and a lambda-type emitter cascaded in two parallel guided modes of opposite propagation directions, we extract the quantum state occupying the modes of interest. For both squeezed vacuum and coherent light input pulses, the Wigner function of the output light after photon subtraction clearly reveals its non-Gaussian character. Furthermore, we propose a measurement-based scheme on the subtracted photon which can lead to conditional generation of quantum states resembling Schrodinger’s kitten state directly from coherent input light with fidelities above 99%. This result is particularly nothworthy, as coherent pulses, unlike the squeezed vacuum inputs commonly used in previous studies, are readily available in most experimental setups.
Coherent manipulation of quantum states of light is key to photonic quantum information processing. In this Letter, we show that a passive two-level nonlinearity suffices to implement non-Gaussian quantum operations on propagating field modes. In particular, the collective light-matter interaction can efficiently extract a single photon from a multiphoton input wave packet to an orthogonal temporal mode. We accurately describe the single-photon subtraction process by elements of an intuitive quantum-trajectory model. By employing this process, quantum information protocols gain orders of magnitude improved efficiency over heralded schemes with linear optics. The reverse process can be used to add photons one by one to a single wave packet mode and compose arbitrarily large Fock states with a finite total success probability >96.7%.
The nature of a quantum network, in particular in the continuous variable regime, is governed not only by the light quantum state but also by the measurement process. It can then be chosen after the light source has been generated. Multimode entanglement is not anymore an intrinsic property of the source but a complex interplay between source, measurement and eventually post processing. This new avenue paves the way for adaptive and scalable quantum information processing. However, to reach this ambitious goal, multimode degaussification has to be implemented. Single-photon subtraction and addition have proved to be such key operations, but are usually performed with linear optics elements on single-mode resources. We present a device able to perform mode dependant non Gaussian operation on a spectrally multimode squeezed vacuum states. Sum frequency generation between the state and a bright control beam whose spectrum has been engineered through ultrafast pulse-shaping is performed. The detection of a single converted photon heralds the success of the operation. The resulting multimode quantum state is analysed with standard homodyne detection whose local oscillator spectrum is independently engineered. The device can be characterized through quantum process tomography using weak multimode coherent states as inputs. Its single-mode character can be quantified and its inherent subtraction modes can be measured. The ability to simultaneously control the state engineering and its detection ensures both flexibility and scalability in the production of highly entangled non-Gaussian quantum states.
In atomic-scale or quantum physics, an electromagnetic field is composed of photons, optical packets so small that a typical laser pointer with 1mW of power emits billions of them each second. Being able to take away or add a single photon in a light field at will would be useful for accurate engineering of quantum states. Such pure single photons are ideal for carrying and manipulating information in emerging quantum technologies, but generating them still is very challenging. In quantum physics, subtraction or addition of a photon is not a deterministic process. Instead, the probability is proportional to the number of photons originally in the electromagnetic field. This is described by the equation â|n〉 = √ n|n − 1〉 and â†|n〉 = √ n+ 1|n + 1〉, where â and ↠are annihilation and creation operators, respectively, representing the action of subtracting and adding a photon in a field composed of n photons.1 Such single-photon operations were limited to pure theoretical discussions until 2004, when Grangier and coworkers found a simple way to subtract a photon2 from a field. Passing through a beam splitter of high transmittivity, some photons can be split from the initial field. A ‘click’ detected in the photodetector in the reflected channel means one photon has been subtracted from the field: see Figure 1(a). When the initial field is composed of a small number of photons, the effect is dramatic and may even completely change the characteristics of the field. For example, let us take an initial single-mode squeezed state generated by ‘degenerate’ parametric down-conversion, which is an optical nonlinear process that converts a pump photon into two twin photons with half the pump photon energy. (This state is well known for its quantum noise squeezed into one quadrature at the expense of expanded noise in the other quadrature.) In order to visualize the noise properties and characteristics of the squeezed state, a probability-like function, such Figure 1. Setups to subtract (a) and add (b) a single photon from/to a light field. ρin and ρout denote the density operators of the input and output fields; BS is a low-reflectivity beam splitter; PDC is a nonlinear crystal where parametric down-conversion takes place; â and ↠denote on/off photodetectors.
The ability to control light at the single photon level is essential for fully harnessing the power of quantum information theory, and precision measurements. In this thesis, we study two phenomena which can help us to create, and shape light at the smallest scale. In the first part of the thesis, we explore deterministic single photon subtraction based upon single photon Raman interaction of a single three-level Λ-type quantum emitter in a bi-modal cavity or coupled with a chiral waveguide. We study the effect of photon subtraction from different types of optical inputs –- continuous-wave or pulsed coherent states and Fock states, and dependence of the fidelity of subtraction upon key system parameters. We also discuss the suitability and prospects of using different emitter-waveguide systems reported in literature to successfully extract a single photon from an optical input. We find that a quantum dot coupled with a photonic crystal waveguide with high group index could subtract photons with fidelity close to unity. Moreover, we explore how such a SPRINT-based single photon subtraction process can be used to create non-Gaussian states with negative values of Wigner distribution, and negative conditional entropies. Such states can be used as quantum resources in various fields of quantum information theory. Finally, as an interesting example, we also discuss how this mechanism can also be used to create non-classical Fock states of arbitrary photon number. \nIn the second part of this thesis, we study how to shape the emission from a single solid-state quantum emitter, in particular an NV⁻ center in diamond, using two dimensional patterns with sub-wavelength features. We propose a pattern etched on the surface of a diamond sample that enhances the NV's emission in a particular direction, and maximizes coupling with a waveguide substantially far away from the diamond-air interface. Our proposed structure was designed using the adjoint optimization technique, which significantly reduces the amount of computational resources compared to brute-force methods to design an optical element with desired properties. Our structure exhibits a higher directionality of emission compared to other nanophotonic structures reported in the literature -- solid immersion lenses, nanopillars, and bull's eye structures. Finally, we also discuss in details the steps pertaining to setting up a confocal microscope in our laboratory for imaging NV centers, and characterizing our proposed device.
Optical Schrödinger cat states are non-Gaussian states with applications in quantum technologies, such as for building error-correcting states in quantum computing. Yet the efficient generation of high-fidelity optical Schrödinger cat states is an outstanding problem in quantum optics. Here, we propose using squeezed superpositions of zero and two photons, ∣θ⟩=cos⁡(θ/2)∣0⟩+sin⁡(θ/2)∣2⟩|θ\rangle = \cos{(θ/2)}|0\rangle + \sin{(θ/2)}|2\rangle∣θ⟩=cos(θ/2)∣0⟩+sin(θ/2)∣2⟩, as ingredients for protocols to efficiently generate high-fidelity cat states. We present a protocol using linear optics with success probability P≳50%P\gtrsim 50\%P≳50% that can generate cat states of size ∣α∣2=5|α|^2=5∣α∣2=5 with fidelity F>0.99F>0.99F>0.99. The protocol relies only on detecting single photons and is remarkably tolerant of loss, with 2%2\%2% detection loss still achieving F>0.98F>0.98F>0.98 for cats with ∣α∣2=5|α|^2=5∣α∣2=5. We also show that squeezed θθθ states are ideal candidates for nonlinear photon subtraction using a two-level system with near deterministic success probability and fidelity F>0.98F>0.98F>0.98 for cat states of size ∣α∣2=5|α|^2=5∣α∣2=5. Schemes for generating θθθ states using quantum emitters are also presented. Our protocols can be implemented with current state-of-the-art quantum optics experiments.